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International Journal of Modern Physics Conference Series

Coherent population trapping in small- and chip-scale 87Rb vapor cells with buffer gas

Ермак Сергей Викторович, V. V. Semenov, Mikhail V. Petrenko, Пятышев Евгений Нилович

Published Jan 1, 2016• 3 citations
Publisher

Abstract

The characteristics of coherent population trapping (CPT) signal were investigated in small-size glass vapor cells containing [Formula: see text]Rb and Ne buffer gas with narrow line-width laser pumping on D2 line. The parameters of CPT signals were measured using small-size vapor cells with Ne buffer gas pressure in the range of 200–400 Torr, cell temperature in the range of 65–120 [Formula: see text]C and the values of laser pumping power of 30–400 [Formula: see text]W/cm2. Optimal conditions, under which the minimal value of short-term instability of resonance line is achieved, were obtained in experiments. Orientation frequency shifts of CPT resonance using glass [Formula: see text]Rb vapor cells containing buffer gas and anti-relaxation coating were compared. CPT signals using vapor cells based on integrated technologies containing [Formula: see text]Rb in atmosphere of Ne were also investigated. The CPT signals with typical line widths of 2–3 kHz and signal-to-noise ratio of 1500 in 1 Hz bandwidth are observed, which allows one to provide relative frequency instability of 10[Formula: see text] at 100 s.

DOI
10.1142/s2010194516601381

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Journal of the Optical Society of America B•Apr 4, 2018•11 citations
The characteristics of coherent population trapping (CPT) signal were investigated in small-size glass vapor cells containing [Formula: see text]Rb and Ne buffer gas with narrow line-width laser pumping on D2 line. The parameters of CPT signals were measured using small-size vapor cells with Ne buffer gas pressure in the range of 200–400 Torr, cell temperature in the range of 65–120 [Formula: see text]C and the values of laser pumping power of 30–400 [Formula: see text]W/cm2. Optimal conditions, under which the minimal value of short-term instability of resonance line is achieved, were obtained in experiments. Orientation frequency shifts of CPT resonance using glass [Formula: see text]Rb vapor cells containing buffer gas and anti-relaxation coating were compared. CPT signals using vapor cells based on integrated technologies containing [Formula: see text]Rb in atmosphere of Ne were also investigated. The CPT signals with typical line widths of 2–3 kHz and signal-to-noise ratio of 1500 in 1 Hz bandwidth are observed, which allows one to provide relative frequency instability of 10[Formula: see text] at 100 s.
Characteristics of CPT (coherent population trapping) signal are investigated in small-size glass vapor cells containing 87 Rb and Ne buffer gas with narrow linewidth laser pumping on D 2 line. Parameters of CPT absorption signals are measured using small-size vapor cells with Ne buffer gas pressure in range of 200-400 Torr, cell temperature in range of 65-120 °C and values of laser pumping power of 30-400 μW/cm 2 . Optimum conditions, under which the minimal value of short-term instability of resonance line is achieved, are obtained in experiments. CPT signals using vapor cells based on integrated technologies containing 87 Rb in atmosphere of Ne are also investigated. The CPT signals with typical linewidths of 2-3 kHz and signal-to-noise ratio of 1500 in 1 Hz bandwidth are observed, which allows one to provide relative frequency instability of 10 -11 at 100 s.
Coherent population trapping (CPT) on 87 Rb atoms in neon atmosphere has been studied in small-size glass absorption cells under conditions of pumping with narrow-band laser radiation at the D 2 line of the main doublet. Parameters of the absorption signal have been measured in 3-mm-diameter cells at buffer gas (Ne) pressures varied within 200–400 Torr, cell temperatures within 65–120°C, and pumping radiation power densities within 30–400 μW/cm 2 . Optimum values of the buffer gas pressures, cell temperature, and pumping power are determined at which the short-term instability of the resonance line is at minimum. Orientational shifts of the CPT resonance signal in gas-filled cells and small-size cells with antirelaxation coating have been compared.
We report the characterization of dark line resonances observed in Cs vapor microcells filled with a unique neon (Ne) buffer gas. The impact on the coherent population trapping (CPT) resonance of some critical external parameters such as laser intensity, cell temperature, and microwave power is studied. We show the suppression of the first-order light shift by proper choice of the microwave power. The temperature dependence of the Cs ground state hyperfine resonance frequency is shown to be canceled in the 77–80 °C range for various Ne buffer gas pressures. The necessity to adjust the Ne buffer gas pressure or the cell dimensions to optimize the CPT signal height at the frequency inversion temperature is pointed out. Based on such Cs–Ne microcells, we preliminary demonstrate a 852 nm vertical cavity surface emitted laser (VCSEL)-modulated based CPT atomic clock exhibiting a short term fractional frequency instability σy(τ)=1.5×10−10τ−1/2 until 30 s. These results, similar to those published in the literature by others groups, prove the potential of our original microcell technology in view of the development of high-performance chip scale atomic clocks.
Controlling buffer-gas conditions in vapor cells is essential for frequency stabilization and atomic-clock performance. This study investigated the dependence of coherent population trapping (CPT) signal characteristics on nitrogen (N 2{}_{2}2​ ) buffer-gas pressure in micro-fabricated vapor cells containing natural-abundance rubidium (Rb) generated from Rb azide (RbN 3{}_{3}3​ ) for chip-scale atomic clocks. A wafer-level fabrication method enabling individual control of N2 pressure was developed by inkjet patterning of RbN3 and subsequent krypton fluoride (KrF) excimer laser decomposition. An increasing N2 pressure was found to reduce the CPT linewidth and cause a significant decrease in the signal amplitude, which resulted in monotonic degradation in the CPT figure of merit with higher pressures. A CPT-based laser frequency stabilization method that locked the laser wavelength to the CPT resonance peak yielded significantly larger signal amplitudes than a conventional absorption-based method in the low-pressure regime below 8 kPa. These results show that CPT performance in micro-fabricated Rb vapor cells is more restricted by the signal amplitude rather than the linewidth. They also offer practical buffer-gas design guidelines for enhancing short-term frequency stability in chip-scale atomic clocks.
This work presents a study of the short-term stability properties of Rb atomic clocks based on coherent population trapping (CPT) under dynamic excitation of a CPT resonance in cells without buffer gas. It is demonstrated that in an optical cell with anti-relaxation coating of its inner walls, the best stability is achieved at the scanning frequency of the frequency difference of the bichromatic pump field equal to 2 kHz at the resonance width of 450 Hz. In cells without a wall coating, the optimal scanning frequency range is found to be 1.2–2.8 kHz at the resonance width of 29 kHz. Examination of the slope of the stabilization system’s discriminant curve at zero error signal for buffer-gas-free cells uncovered an amount of correlation between the discriminant curve slope and atomic clock stability. It is demonstrated that the highest stability of atomic clocks in dynamic excitation mode is achieved at a ratio of scanning frequency and amplitude around 1.
Pulsed coherent population trapping (CPT) spectroscopy is applied in buffer-gas filled Cs–Ne vapor microfabricated cells. The properties of the Ramsey-CPT clock transition central fringe (linewidth, signal amplitude, and contrast) are studied versus several experimental parameters, including the Ramsey sequence and the input laser intensity, and are compared to those obtained in the conventional continuous (CW) interrogation mode. In the pulsed case and for short Ramsey-free evolution times TR, the central fringe linewidth is found to exhibit a small but visible power broadening and is measured to be narrower than the value of 1/(2TR) that is reached for long TR. The microwave hyperfine coherence lifetime T2 in the Cs–Ne microcells is measured to be in the 50–500 μs range. Its dependence to the buffer gas pressure or cell temperature is briefly studied.