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Journal of the Optical Society of America B

Study of the effect of repump laser on atomic line filter

Ayan Ray, Md. Sabir Ali, Alok Chakrabarti

Published Aug 16, 2013• 8 citations
Publisher

Abstract

The improvement in the performance of an atomic line filter (ALF) under the action of a repump laser is reported in the current experimental work. We address the issue of repumping by including an additional laser coupling the 5S1/2(F=1)→5P3/2(F′′=2,1,0) hyperfine levels whereas the optical filter action is exhibited through a pump–probe laser-induced excited state absorption {5S1/2(F=2)→5P3/2(F′=3)→5D3/2(F′′=3)} of the Rb87 atom. It is found that the application of the repump mechanism considerably influences the characterizing parameters (i.e., transmittance and width) of the ALF. To optimize the performance of the ALF, it is required to carefully choose the detuning and intensity of the repump laser for a fixed set of pump–probe combination. For this purpose, the effect of systematic change in detuning and intensity of the repump laser on the ALF signal is studied in detail. For example, it is experimentally found that ALF considerably benefits (∼30%) in transmittance from selective repumping of atoms. It is to be noted that, unlike earlier reports, where the frequency scale of the filter is calibrated with Faby–Perot etalons of comparatively larger free spectral range, the marking is done here with the help of double resonance optical pumping (DROP) signals. The DROP signals, which originate from two-photon coupling within the 5S→5P→5D hyperfine domain, also act as an indicator of the existing “Radiation Trapping” process in the cascade medium. The current study may help in improving the performance of narrow-bandwidth ALF, which is useful for free space optical communication systems and laser spectroscopy.

DOI
10.1364/josab.30.002436

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Physica Scripta•Mar 18, 2024•0 citations
The improvement in the performance of an atomic line filter (ALF) under the action of a repump laser is reported in the current experimental work. We address the issue of repumping by including an additional laser coupling the 5S1/2(F=1)→5P3/2(F′′=2,1,0) hyperfine levels whereas the optical filter action is exhibited through a pump–probe laser-induced excited state absorption {5S1/2(F=2)→5P3/2(F′=3)→5D3/2(F′′=3)} of the Rb87 atom. It is found that the application of the repump mechanism considerably influences the characterizing parameters (i.e., transmittance and width) of the ALF. To optimize the performance of the ALF, it is required to carefully choose the detuning and intensity of the repump laser for a fixed set of pump–probe combination. For this purpose, the effect of systematic change in detuning and intensity of the repump laser on the ALF signal is studied in detail. For example, it is experimentally found that ALF considerably benefits (∼30%) in transmittance from selective repumping of atoms. It is to be noted that, unlike earlier reports, where the frequency scale of the filter is calibrated with Faby–Perot etalons of comparatively larger free spectral range, the marking is done here with the help of double resonance optical pumping (DROP) signals. The DROP signals, which originate from two-photon coupling within the 5S→5P→5D hyperfine domain, also act as an indicator of the existing “Radiation Trapping” process in the cascade medium. The current study may help in improving the performance of narrow-bandwidth ALF, which is useful for free space optical communication systems and laser spectroscopy.
We have studied double-resonance optical pumping (DROP) as a function of the polarization combination of lasers, laser power, and the alignment of lasers in the 5S1/2-5P3/2-D3/2,5/2 ladder-type system of Rb87 atoms. By considering the two-photon transition probability and optical pumping effects, the changes in the relative magnitude of the DROP hyperfine structures as a function of the polarization combination of the lasers were analyzed theoretically. The theoretical results are in good agreement with the experimental results. Owing to the low optical pumping effect in the cycling transition, we could see the dependence of the spectrum on the laser power in the 5P3/2-4D5/2 transition distinctly. Also, the spectral linewidths as a function of the alignment between the lasers were measured 12.2 MHz for copropagating beams and 6.9 MHz for counterpropagating beams.
An ongoing spectroscopic investigation of atomic rubidium utilizes a two-photon, single-laser excitation process. Transitions accessible with our tunable laser include 5P1/2 (F ′ ) ← 5S1/2 (F) and 5P3/2 (F ′ ) ← 5S1/2 (F). The laser is split into a pump and probe beam to allow for Doppler-free measurements of transitions between hyperfine levels. The pump and probe beams are overlapped in a counter-propagating geometry and the laser frequency scans over a transition. Absorption, fluorescence and polarization spectroscopy techniques are applied to this basic experimental setup. The temperature of the vapor cell and the power of the pump and probe beams have been varied to explore line broadening effects and signal-to-noise of each technique. This humble setup will hopefully grow into a more robust experimental arrangement in which double resonance, two-laser excitations are used to explore hyperfine state changing collisions between rubidium atoms and noble gas atoms. Rb-noble gas collisions can transfer population between hyperfine levels, such as 5P3/2 (F ′ = 3) Collision ←− 5P3/2 (F ′ = 2), and the probe beam couples 7S1/2 (F ′′ = 2) ← 5P3/2 (F ′ = 3). Polarization spectroscopy signal depends on the rate of population transfer due to the collision as well as maintaining the orientation created by the pump laser. Fluorescence spectroscopy relies only on transfer of population due to the collision. Comparison of these techniques yields information regarding the change of the magnetic sublevels, mF , during hyperfine state changing collisions.
We have investigated the optical pumping effects of single-resonance optical pumping (SROP) and double-resonance optical pumping (DROP) in the ladder-type electromagnetically induced transparency (EIT) of the 5S1/2–5P3/2–5D3/2 transition of 87Rb atoms. In the 5S1/2(F = 2)–5P3/2(F' = 3)–5D3/2(F'' = 2, 3) transition with the single-resonance cycling 5S1/2(F = 2)–5P3/2(F' = 3) transition, we observed the transmittance spectrum due to DROP and EIT. Based on our experimental results investigated according to the laser power (the probe and the coupling) and the coupling laser detuning, we revealed that DROP was significant for the transmittance spectrum. Particularly, in the 5S1/2(F = 2)–5P3/2(F' = 1, 2)–5D3/2(F'' = 1) transition without a cycling transition, we observed the two-photon absorption due to two-photon atomic coherence, when the probe laser power was weak and the coupling laser power was strong.
For the experimental implementation of an optically pumped atomic magnetometer, the magnetic resonance signal with a narrow linewidth and a high signal-to-noise ratio (SNR) is required for achieving a high sensitivity. Using 795-nm laser as both the pumping and the probe laser, we compare the magnetic resonance signals from different rubidium atomic vapor cells and investigate the variations of magnetic resonance signals with temperature. Optimized magnetic resonance signal is achieved with a paraffin-coated rubidium atomic vapor cell. Then the 780-nm laser at rubidium D2 line is introduced as a repumping laser, and we explore the changes of linewidth and SNR of the magnetic resonance signal under different power of the pumping laser and the repumping laser. Owing to the 780-nm repumping laser beam, the signal amplitude of rubidium-85 magnetic resonance signal is improved remarkably because more rubidium-85 atoms are spin- polarized by the 795-nm pumping laser beam. At the same time, the linewidth of rubidium-85 magnetic resonance signal is roughly not broadened anymore. We realize a closed-loop optically pumped rubidium-85 atomic magnetometer with a bandwidth of ~1.2 kHz, and the sensitivity is calibrated to be ~245.5 pT/Hz1/2 only with the 795-nm pumping laser beam. Owing to the employment of the 780-nm repumping laser beam, the sensitivity is improved to be ~26.4 pT/Hz1/2 which is improved roughly by one order of magnitude. We also calibrate the measurement accuracy and deviation of a commercial fluxgate magnetometer by using the enhanced rubidium magnetic resonance signal.
The major efforts of this project were: (1) to reassess the technical merits of a Tantalum atomic line filter (ALF) employing a low vapor density T1C1 and (2) to measure the excited state cesium trapping lifetimes and to derive the self quenching cross sections of excited state cesium atoms. These two separate efforts address alternative approaches to the implementation of an ALF based on metastable T1 atoms, T1 sub m, whose absorption wavelength (535 nm) matches the frequency doubled Nd:Bel laser. The first approach uses photodissociation to produce T1 sub m directly from T1C1. The second approach involves resonantly pumping the Cs in a T1-Cs mixture and collisionally transferring energy to the T1 to sustain the required density of T1 sub m.
Abstract In this work, we report experimental studies on coherence in a medium exhibiting DROP (Double Resonance Optical Pumping)-FWM (Four Wave Mixing). Here 5S1/2(F) → 5P3/2(F/) → 5D (F//) two photon transition of hot 87Rb atoms is used. The 5S→5P connection is modified by introducing an additional beam phase coupled to the original beam linking F = 2 → F/ transition. The frequency of the additional beam is offset from that of the original beam by ≈ +10Γ (Γ is natural linewidth). Such a two-beam configuration in F→F/ manifold effectively satisfies conditions of Vee (V) linkage or degenerate two-level connection (DTLC), depending on the detuning of the 780nm laser. This transformation profoundly affects the behavior of the ensuing Ladder (Ξ) system. While the (I) Ξ +V condition is favorable for Electromagnetically Induced Transparency (EIT), the (ii) Ξ + DTLC brings in the effect of Electromagnetically Induced Absorption (EIA). The EIT-dominated situation is helpful for FWM to take place, and the EIA effect augments the stronger presence of DROP. This condition is verified by monitoring the blue fluorescence emanating from the 5D→6P3/2→5S1/2 decay route. The DROP effect follows the Amplified Spontaneous Emission (ASE) pattern in the media. The origin of blue photons is also due to FWM under EIT conditions. In the case of EIA, the dominant condition increment in blue fluorescence is due to increased stimulated emission. The blue photons mainly contributed by (i) FWM and (ii) increased participation of stimulated emission are directional in nature and phase coherent.