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Journal of the Optical Society of America B

Double-resonance optical pumping of Rb atoms

Han Seb Moon, Lim Lee, Jung Bog Kim

Published Aug 7, 2007• 47 citations
Publisher

Abstract

We have studied double-resonance optical pumping (DROP) as a function of the polarization combination of lasers, laser power, and the alignment of lasers in the 5S1/2-5P3/2-D3/2,5/2 ladder-type system of Rb87 atoms. By considering the two-photon transition probability and optical pumping effects, the changes in the relative magnitude of the DROP hyperfine structures as a function of the polarization combination of the lasers were analyzed theoretically. The theoretical results are in good agreement with the experimental results. Owing to the low optical pumping effect in the cycling transition, we could see the dependence of the spectrum on the laser power in the 5P3/2-4D5/2 transition distinctly. Also, the spectral linewidths as a function of the alignment between the lasers were measured 12.2 MHz for copropagating beams and 6.9 MHz for counterpropagating beams.

DOI
10.1364/josab.24.002157

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Double-resonance optical-pumping spectra of rubidium 5S 1/2 - 5P 3/2 - 4D 3/2 transitions and frequency stabilization of 1.5-micrometer laser

Jing Gao, 王杰 Wang Jie, Baodong Yang +2 more

We demonstrate the spectra of 87Rb 5S1/2 - 5P3/2 - 4D3/2 transitions by utilizing the double-resonance optical-pumping (DROP) and optical-optical double-resonance (OODR) techniques, respectively. The DROP spectrum, compared with the traditional OODR spectrum, show a much better signal-to-noise ratio (SNR). Paying special attention to the influence of alignment of lasers where the coupling and probe beams are counter-propagation and co-propagation on DROP spectrum, so as to further narrow the spectral width by means of electromagnetically induced transparency (EIT). When -the frequency of 1.5μm fiber-pigtailed butterfly-type distributed-feedback (DFB) diode laser is stabilized to the DROP spectrum of 87Rb 5P3/2 - 4D3/2 transition, the preliminary result of residual frequency jitter after stabilization is ~ ±1.3 MHz within 60 s.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Oct 8, 2010•3 citations
We have studied double-resonance optical pumping (DROP) as a function of the polarization combination of lasers, laser power, and the alignment of lasers in the 5S1/2-5P3/2-D3/2,5/2 ladder-type system of Rb87 atoms. By considering the two-photon transition probability and optical pumping effects, the changes in the relative magnitude of the DROP hyperfine structures as a function of the polarization combination of the lasers were analyzed theoretically. The theoretical results are in good agreement with the experimental results. Owing to the low optical pumping effect in the cycling transition, we could see the dependence of the spectrum on the laser power in the 5P3/2-4D5/2 transition distinctly. Also, the spectral linewidths as a function of the alignment between the lasers were measured 12.2 MHz for copropagating beams and 6.9 MHz for counterpropagating beams.
The polarization dependence of double-resonance optical pumping (DROP) in the ladder-type electromagnetically induced transparency (EIT) of the $5{S}_{1/2}\ensuremath{-}5{P}_{3/2}\ensuremath{-}5{D}_{5/2}$ transition of 87{}^{87}87Rb atoms is studied. The transmittance spectra in the $5{S}_{1/2}(F=2)\ensuremath{-}5{P}_{3/2}({F}^{\ensuremath{'}}=3)\ensuremath{-}5{D}_{5/2}({F}^{\ensuremath{'}\ensuremath{'}}=2,3,4)$ transition were observed as caused by EIT, DROP, and saturation effects in the various polarization combinations between the probe and coupling lasers. The features of the double-structure transmittance spectra in the $5{S}_{1/2}(F=2)\ensuremath{-}5{P}_{3/2}({F}^{\ensuremath{'}}=3)\ensuremath{-}5{D}_{5/2}({F}^{\ensuremath{'}\ensuremath{'}}=4)$ cycling transition were attributed to the difference in saturation effect according to the transition routes between the Zeeman sublevels and the EIT according to the two-photon transition probability.
We have investigated the optical pumping effects of single-resonance optical pumping (SROP) and double-resonance optical pumping (DROP) in the ladder-type electromagnetically induced transparency (EIT) of the 5S1/2–5P3/2–5D3/2 transition of 87Rb atoms. In the 5S1/2(F = 2)–5P3/2(F' = 3)–5D3/2(F'' = 2, 3) transition with the single-resonance cycling 5S1/2(F = 2)–5P3/2(F' = 3) transition, we observed the transmittance spectrum due to DROP and EIT. Based on our experimental results investigated according to the laser power (the probe and the coupling) and the coupling laser detuning, we revealed that DROP was significant for the transmittance spectrum. Particularly, in the 5S1/2(F = 2)–5P3/2(F' = 1, 2)–5D3/2(F'' = 1) transition without a cycling transition, we observed the two-photon absorption due to two-photon atomic coherence, when the probe laser power was weak and the coupling laser power was strong.
We present the double resonance optical pumping (DROP) effect of ladder-type electromagnetically induced transparency (EIT) in the 5S1/2-5P3/2-5D5/2 transition of 87Rb atoms. When many atoms of the ladder-type atomic system are simultaneously resonant with the two laser fields, the population of one ground state can be optically pumped into another ground state through intermediate states and excited states. In this paper, we reveal that most previous results for the ladder-type EIT include the DROP effect. When the probe laser is very weak and the coupling laser is strong, we can observe the double structure transmittance spectrum, a narrow spectrum due to the EIT and a broad spectrum due to the DROP, in the 5S1/2(F=2)-5P3/2(F'=3)-5D5/2(F"=4) cycling transition.
우리는 87Rb^{87}Rb87Rb 원자의 5S1/2−5P3/2−4D3/2,  5/25S_{1/2}-5P_{3/2}-4D_{3/2,\;5/2}5S1/2​−5P3/2​−4D3/2,5/2​ 전이선을 이용하여 레이저의 세기, 편광조합, 그리고 정렬상태에 따른 이중공명광펌핑(double resonance optical pumping; DROP) 스펙트럼을 조사하였다. 5P3/2−4D5/25P_{3/2}-4D_{5/2}5P3/2​−4D5/2​ 전이선에서 레이저의 세기에 따른 초미세 구조간의 DROP 신호의 변화가 크게 나타났고, 그 원인은 순환전이선의 낮은 광펌핑 효율 때문이었다. 두 레이저의 편광조합을 달리 했을 때 이중공명의 전이율이 변하고, 이러한 효과가DROP스펙트럼의 변화로 나타났다. 또한 두 레이저가 같은 방향으로 진행하는 경우와 반대 방향으로 진행하는 경우를 비교했을 때, 스펙트럼의 선폭은 각각 12.2 MHz 와 6.9 MHz로 측정되었다. We present the double resonance optical pumping(DROP) spectra according to the laser power, the polarization combination of lasers, and the alignment of lasers in the transition 5P3/2−4D5/2  and  5P3/2−4D5/25P_{3/2}-4D_{5/2}\;and\;5P_{3/2}-4D_{5/2}5P3/2​−4D5/2​and5P3/2​−4D5/2​ of 87Rb.^{87}Rb.87Rb. We observed obviously changing DROP spectrum according to the laser power in the transition 5P3/2−4D5/25P_{3/2}-4D_{5/2}5P3/2​−4D5/2​ involved the cycling transition. The laser power effects are attributed to the low optical-pumping-effect in the cycling transition. We observed changing DROP spectrum depending on the polarizations of the lasers. The laser polarization effects are attributed to the changing transition probability according to the polarizations of lasers. We compared the co-propagation with the counter-propagation and the spectral linewidths were 12.2 MHz and 6.9 MHz, respectively.
The frequency stabilization of a laser diode in the 1.3 microm region using double resonance optical pumping (DROP) spectrum in the 5P(3/2)-6S(1/2) transition of (87)Rb atoms is demonstrated. The signal-to-noise ratio of the DROP spectrum is approximately ten times higher than that of the previous optical-optical double resonance spectrum. The spectral linewidth of the DROP measures 8.4 MHz. When the frequency of a 1.367 microm laser diode is stabilized to the DROP spectrum, the frequency stability is 9 x 10(-12) after 100 s. Also, the wavelength of the frequency-stabilized laser locked to the 5P(3/2)-6S(1/2) transition using a wavelength meter is measured.
We demonstrate the spectra of 87Rb 5S1/2 - 5P3/2 - 4D3/2 transitions by utilizing the double-resonance optical-pumping (DROP) and optical-optical double-resonance (OODR) techniques, respectively. The DROP spectrum, compared with the traditional OODR spectrum, show a much better signal-to-noise ratio (SNR). Paying special attention to the influence of alignment of lasers where the coupling and probe beams are counter-propagation and co-propagation on DROP spectrum, so as to further narrow the spectral width by means of electromagnetically induced transparency (EIT). When -the frequency of 1.5μm fiber-pigtailed butterfly-type distributed-feedback (DFB) diode laser is stabilized to the DROP spectrum of 87Rb 5P3/2 - 4D3/2 transition, the preliminary result of residual frequency jitter after stabilization is ~ ±1.3 MHz within 60 s.