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Physical Review Letters

ac Stark Splitting and Quantum Interference with Intersubband Transitions in Quantum Wells

J. F. Dynes, Mark D. Frogley, Mattias Beck, Jérôme Faist, Chris C. Phillips

Published Apr 22, 2005• 218 citations
Publisher

Abstract

Resonant optical coupling experiments have demonstrated coherent quantum interference between the Stark-split "dressed states" of a synthesized 3-level electronic system in a semiconductor quantum well. Analysis of the dephasing mechanisms reveals dipole selection rules closely analogous to those seen in atomic spectroscopy experiments. In this respect, these systems behave as "artificial atoms" for the purposes of observing a range of nonclassical coherent optical effects. The prospects for exploiting them for scalable quantum information processing applications are more promising than previous dephasing models would have predicted.

DOI
10.1103/physrevlett.94.157403

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Resonant optical coupling experiments have demonstrated coherent quantum interference between the Stark-split "dressed states" of a synthesized 3-level electronic system in a semiconductor quantum well. Analysis of the dephasing mechanisms reveals dipole selection rules closely analogous to those seen in atomic spectroscopy experiments. In this respect, these systems behave as "artificial atoms" for the purposes of observing a range of nonclassical coherent optical effects. The prospects for exploiting them for scalable quantum information processing applications are more promising than previous dephasing models would have predicted.
Abstract Stark splitting and quantum interference effects in the absorption spectrum of a probe field in coherently driven closed upper coupled three level atomic schemes ( and upper-cascade), which are created by a strong driving field are studied using the dressed state representation. In the dressed representation, the absorption due to the Stark splitting can be separated from the absorption due to the interference effects. We explicitly show the presence of both destructive and constructive interference in upper coupled three level atomic schemes. The interference in these atomic schemes is due to the coupling of the two dressed states by the same vacuum modes and the probe. We show that the dephasing rates can change the nature of the interference from constructive to destructive and vice versa, resulting in increased or decreased resonant absorption of the probe field.
Summary form only given. In the excitonic ac Stark shift in quantum wells the excitonic absorption line is blueshifted by shining on the sample an intense laser pulse, whose frequency is lower than the exciton transition frequency. The effect is bigger when the laser spectrum approaches the resonance with the excitonic absorption. But if the laser and excitonic absorption spectra sensibly overlap, a great amount of electronic population is excited and consequently the Coulomb nonlinearities due to the interaction between excited carries or excitons dramatically increase. One prominent effect under these conditions is the excitation- induced dephasing which can destroy the coherence of the electronic system and therefore the coupling between excitons and light, which is inherently coherent. Some evidence for the resonant Stark effect was already reported, but the direct observation of the spectral splitting was still missing. This observation demonstrates that the coherent exciton light coupling in semiconductors can be strong enough to survive the fast dephasing, and that therefore an efficient ultrafast manipulation of the exciton absorption in the coherent transient is possible. In order to magnify the ac Stark effect and its visibility a special sample was designed: a single In/sub 0.04/Ga/sub 0.96/As quantum well is grown on the top of an AlAs/AlGaAs distributed Bragg reflector; two /spl lambda//2 spacers separate the quantum well from the mirror and from the air. In this configuration the light field incident on the sample and the one reflected by the mirror constructively interfere at the quantum well position, giving a high effective absorption.
We report the measurement of the transient intersubband absorption in a coupled quantum well semiconductor structure. Pulsed interband excitation is used to prepare a coherent population in the two lowest states of a three level system of electronic subbands. The time-dependent absorption to the upper state is probed by midinfrared time-domain spectroscopy. For certain pump–probe delay times we observe in the intersubband absorption spectra typical signatures of quantum interference: regions with reduced or enhanced absorption.
We report the observation of tunneling induced transparency in asymmetric double quantum well structures. Resonant tunneling through a thin barrier is used to coherently couple the two upper states in a three level system of electronic subbands in a GaAs/AlGaAs structure. This creates Fano-type interferences for the collective intersubband excitations in the absorption from the ground state, analogous to electromagnetically induced transparency (EIT) in atomic systems. We observe a 50% reduction in absorption between the subband resonances which can be explained by taking into account the coherent coupling of the upper states. We analyze the bias dependent absorption spectra and determine the relevant lifetime broadening and dephasing rates for the transitions.
The coherent optical response of high quality microcavities containing quantum wells is investigated. The dynamics of the ac Stark effect is investigated by degenerate pump–probe experiments, by exciting the quantum well excitons at various intensities and detunings. The evolution from a simple dynamical excitonic Stark shift to a splitting is clearly observed, even when the excitation is degenerate with the continuum states. The experimental results agree well with the predictions of a theoretical model based on the semiconductor Maxwell-Bloch equations.
This paper presents the current results of field-induced quantum interference in semiconductor quantum wells. Three-level systems with two conduction subbands in single and double quantum wells coupled by a resonant field are studied. We investigate effects of the Coulomb and field-induced electronic renormalizations of the energy subbands and steady eigenstates of electrons. The random-phase and ladder approximations have been used to calculate the linear interband and intersubband optical absorptions and refractive indices. The effect of collective dipole moment on the nonlinear susceptibility has been incorporated into the study by using a local-field approach. Lasing without population inversion, electromagnetically induced transparency, and enhanced nonlinearity with reduced absorption inside the intersubband-coupled single quantum well and dc-field coupled double quantum wells are found.