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Physica Scripta

Interference via dephasing effect in upper coupled three-level atoms

Sankar Davuluri, Shi‐Yao Zhu

Published Dec 18, 2015• 5 citations
Publisher

Abstract

Abstract Stark splitting and quantum interference effects in the absorption spectrum of a probe field in coherently driven closed upper coupled three level atomic schemes ( and upper-cascade), which are created by a strong driving field are studied using the dressed state representation. In the dressed representation, the absorption due to the Stark splitting can be separated from the absorption due to the interference effects. We explicitly show the presence of both destructive and constructive interference in upper coupled three level atomic schemes. The interference in these atomic schemes is due to the coupling of the two dressed states by the same vacuum modes and the probe. We show that the dephasing rates can change the nature of the interference from constructive to destructive and vice versa, resulting in increased or decreased resonant absorption of the probe field.

DOI
10.1088/0031-8949/91/1/013008

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Abstract Stark splitting and quantum interference effects in the absorption spectrum of a probe field in coherently driven closed upper coupled three level atomic schemes ( and upper-cascade), which are created by a strong driving field are studied using the dressed state representation. In the dressed representation, the absorption due to the Stark splitting can be separated from the absorption due to the interference effects. We explicitly show the presence of both destructive and constructive interference in upper coupled three level atomic schemes. The interference in these atomic schemes is due to the coupling of the two dressed states by the same vacuum modes and the probe. We show that the dephasing rates can change the nature of the interference from constructive to destructive and vice versa, resulting in increased or decreased resonant absorption of the probe field.
We observed quantum interference effects in steady-state optical absorption in a VVV-type three-level system of Pr3+:YAlO3{\mathrm{Pr}}^{3+}:{\mathrm{YAlO}}_{3}Pr3+:YAlO3​ where a hyperfine transition between two upper levels was homogeneously broadened by pure dephasing. This VVV-type system was excited by a single driving radio-frequency (rf) field and two probe laser fields (quantum-beat scheme). The probe absorption was constructively or destructively affected by the phase of the driving rf field. In contrast, under two-laser excitation without application of the rf, no absorption change due to electromagnetically induced transparency (EIT) was observed. A comparison of observations and theoretical predictions revealed that the quantum-beat scheme generates quantum interference even when the dephasing rate between the two upper levels is comparable with the Rabi frequency of the probe laser, and completely destroys EIT.
We examine the absorption of a weak probe beam by a laser driven V-type atom with a pair of closely lying excited levels, where both the driving and probe lasers interact simultaneously with the two transitions. The effects of quantum interference among decay channels on the absorption spectra are also investigated. We introduce dipole moments in the dressed-state representation and the Hamiltonian in terms of the dressed states describing the interaction between the probe and the atom. In the degenerate case, features similar to that of a driven two-level atomic system are found due to some dark transitions in the spontaneous emission and the fact that the probe beam only detects certain transitions. In the nondegenerate case, the absorption spectrum is strongly influenced by the degree of quantum interference, resulting in different line shapes for emission peaks, absorption peaks, and dispersionlike profiles. The effect of probe polarization on the absorption spectrum is also investigated.
In this paper we reveal that the constructive interference of atomic coherence on absorption leads to electromagnetically induced absorption,which is in sharp contrast to the case in which destructive interference of atomic coherence gives rise to electromagnetically induced transparency. A four-level atomic system is employed in which three transitions are in N configuration and the middle transition is used as a probe transition. In the dressed states representation the probe transition is split into four transitions that are coupled to each other. The coupling originates from the spontaneous emission of the atomic medium and the spontaneous transfer from excited state coherence to ground state coherence. The former leads to couplings between all transitions with the same sign and to the absorption reduction. The latter results in couplings,of which t wo terms have positive sign and another two have negative sign. It is due to the couplings with positive and negative signs that significant modification of the contribution of dressed coherence to absorption occurs,i.e., absorption inhibition is changed to absorption enhancement.
The quantum correlation in dephasing decay can be realized, when the energy fluctuations of transition frequencies are synchronized. The correlation in the three-level atom systems will enhance the interference in the absorption and change the nature of the interference, from destructive to constructive in cascade low-driving three-level atom and from constructive to destructive in V-type three-level atom. The quantum correlation is observed by properly introducing the collision or time-dependent magnetic field through the increase or decrease of the resonant absorption.
In this paper we present a detailed treatment of the ac Stark effect of a three-level atom driven by two strong laser fields in a cascade scheme. We consider two situations where there is a weak laser field probing a new transition starting from one of the three levels to a fourth level. In one case the initial level of the probed transition is the ground state and in the other case the initial level is the intermediate state. For both situations we derive an analytical expression for the absorptive and dispersive responses of the weak probe field and present the spectrum obtained from numerical calculation. The general feature of the spectrum has a three-peak structure. The positions and relative intensities of the three spectral components are affected strongly by the driving field intensities and detunings. An account of the spectrum is given in terms of the dressed-state formalism.
We study the effect of quantum interference on the population distribution and absorptive properties of a V-type three-level atom driven by two lasers of unequal intensities and different angular frequencies. Three coupling configurations of the lasers to the atom are analysed: (a) both lasers coupled to the same atomic transition, (b) each laser coupled to different atomic transition and (c) each laser coupled to both atomic transitions. Dressed states for the three coupling configurations are identified, and the population distribution and absorptive properties of the weaker field are interpreted in terms of transition dipole moments and transition frequencies among these dressed states. In particular, we find that in the first two cases there is no population inversion between the bare atomic states, but the population can be trapped in a superposition of the dressed states induced by quantum interference and the stronger field. We show, that the trapping of the population, which results from the cancellation of transition dipole moments, does not prevent the weaker field to be coupled to the cancelled (dark) transitions. As a result, the weaker field can be strongly amplified on transparent transitions. In the case of each laser coupled to both atomic transitions the population can be trapped in a linear superposition of the excited bare atomic states leaving the ground state unpopulated in the steady state. Moreover, we find that the absorption rate of the weaker field depends on the detuning of the strong field from the atomic resonances and the splitting between the atomic excited states. When the strong field is resonant to one of the atomic transitions a quasi-trapping effect appears in one of the dressed states. In the quasi-trapping situation all the transition dipole moments are different from zero, which allows the weaker field to be amplified on the inverted transitions. When the strong field is tuned halfway between the atomic excited states, the population is completely trapped in one of the dressed states and no amplification is found for the weaker field.