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arXiv:cond-mat/0404122 · Physical Review B

Regular and singular Fermi-liquid fixed points in quantum impurity models

Pankaj Mehta, Natan Andrei, Piers Coleman, L. Borda, Gergely Zaránd

Published Jul 14, 2005• 77 citations
arXivHTMLPDF

Abstract

We show that the traditional classification of quantum inpurity models based on thermodynamics is insufficient to probe the nature of their low-energy dynamics. We propose an analysis based on scattering theory, dividing Fermi liquids into regular Fermi liquids and singular Fermi liquids. In both cases electrons at the Fermi energy scatter elastically off the impurity, but in the case of regular Fermi liquids the scattering has analytical properties in the vicinity of the Fermi energy, while for singular Fermi liquids it does not, resulting in a breakdown of Nozi\`eres' Fermi-liquid picture and singular thermodynamic behavior. Using the Bethe ansatz and numerical renormalization group, we show that the ordinary Kondo model is a regular Fermi liquid whereas the underscreened Kondo model is a a singular Fermi liquid. Conventional regular Fermi liquid behavior is reestablished in an external magnetic field $H$, but with a density of states which diverges as $1∕H$. Our results may be relevant for the recently observed field-tuned quantum criticality in heavy electron materials.

DOI
10.1103/physrevb.72.014430

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We show that the traditional classification of quantum inpurity models based on thermodynamics is insufficient to probe the nature of their low-energy dynamics. We propose an analysis based on scattering theory, dividing Fermi liquids into regular Fermi liquids and singular Fermi liquids. In both cases electrons at the Fermi energy scatter elastically off the impurity, but in the case of regular Fermi liquids the scattering has analytical properties in the vicinity of the Fermi energy, while for singular Fermi liquids it does not, resulting in a breakdown of Nozi`eres' Fermi-liquid picture and singular thermodynamic behavior. Using the Bethe ansatz and numerical renormalization group, we show that the ordinary Kondo model is a regular Fermi liquid whereas the underscreened Kondo model is a a singular Fermi liquid. Conventional regular Fermi liquid behavior is reestablished in an external magnetic field HHH, but with a density of states which diverges as 1∕H1∕H1∕H. Our results may be relevant for the recently observed field-tuned quantum criticality in heavy electron materials.
We generalize Nozi\`eres' Fermi-liquid theory for the low-energy behavior of the Kondo model to that of the single-impurity Anderson model. In addition to the electrons' phase shift at the Fermi energy, the low-energy Fermi-liquid theory is characterized by four Fermi-liquid parameters: the two given by Nozi\`eres that enter to first order in the excitation energy, and two additional ones that enter to second order and are needed away from particle-hole symmetry. We express all four parameters in terms of zero-temperature physical observables, namely the local charge and spin susceptibilities and their derivatives with respect to the local level position. We determine these in terms of the bare parameters of the Anderson model using Bethe ansatz and numerical renormalization group (NRG) calculations. Our low-energy Fermi-liquid theory applies throughout the crossover from the strong-coupling Kondo regime via the mixed-valence regime to the empty-orbital regime. From the Fermi-liquid theory, we determine the conductance through a quantum dot symmetrically coupled to two leads in the regime of small magnetic field, low temperature, and small bias voltage, and compute the coefficients of the $\ensuremath{\sim}{B}^{2}, \ensuremath{\sim}{T}^{2}$, and $\ensuremath{\sim}{V}^{2}$ terms exactly in terms of the Fermi-liquid parameters. The coefficients of T2,V2{T}^{2}, {V}^{2}T2,V2, and B2{B}^{2}B2 are found to change sign during the Kondo to empty-orbital crossover. The crossover becomes universal in the limit that the local interaction is much larger than the level width. For completeness, we also compute the shot noise and discuss the resulting Fano factor.
Despite the fact that the low energy behavior of the basic Kondo model cannot be studied perturbatively it was eventually shown by Wilson, Anderson, Nozieres and others to have a simple "local Fermi liquid theory" description. That is, electronic degrees of freedom become effectively non-interacting in the zero energy limit. However, generalized versions of the Kondo model involving more than one channel or impurity may exhibit low energy behavior of a less trivial sort which can, nonetheless, be solved exactly using either Bethe ansatz or conformal field theory and bosonization techniques. Now the low energy limit exhibits interacting many body behavior. For example, processes in which a single electron scatters off the impurity into a multi electron-hole state have a non-vanishing (and sometimes large) amplitude at zero energy. This corresponds to a rare solveable example of non-Fermi liquid behavior. Essential features of these phenomena are reviewed.
We give a Hamiltonian-based interpretation of microscopic Fermi liquid theory within a renormalization group framework. The Fermi liquid fixed-point Hamiltonian with its leading-order corrections is identified and we show that the mean field calculations for this model correspond to the Landau phenomenological approach. This is illustrated first of all for the Kondo and Anderson models of magnetic impurities which display Fermi liquid behaviour at low temperatures. We then show how these results can be deduced by a reorganization of perturbation theory, in close parallel to that for the renormalized φ4 field theory. The Fermi liquid results follow from the two lowest order diagrams of the renormalized perturbation expansion. The calculations for the impurity models are simpler than for the general case because the self-energy depends on frequency only. We show, however, that a similar renormalized expansion can be derived also for the case of a translationally invariant system. The parameters specifying the Fermi liquid fixed-point Hamiltonian are related to the renormalized vertices appearing in the perturbation theory. The collective zero sound modes appear in the quasiparticle-quasihole ladder sum of the renormalized perturbation expansion. The renormalized perturbation expansion can in principle be used beyond the Fermi liquid regime to higher temperatures. This approach should be particularly useful for heavy fermions and other strongly correlated electron systems, where the renormalization of the single-particle excitations are particularly large. We briefly look at the breakdown of Fermi liquid theory from a renormalized perturbation theory point of view. We show how a modified version of the approach can be used in some situations, such as the spinless Luttinger model, where Fermi liquid theory is not applicable. Other examples of systems where the Fermi liquid theory breaks down are also briefly discussed.
In this work we consider several exactly solvable models of magnetic impurities in critical quantum antiferromagnetic spin chains and multichannel Kondo impurities. Their ground-state properties are studied, and the finite set of nonlinear integral equations which exactly describe the thermodynamics of the models is constructed. We obtain several analytical low-energy expressions for the temperature, magnetic field, and frequency dependences of important characteristics of exactly solvable disordered quantum spin models and disordered multichannel Kondo impurities with essential many-body interactions. We show that the only low-energy parameter that gets renormalized is the velocity of the low-lying excitations (or the effective crossover scale connected with each impurity); the others appear to be universal. In our study several kinds of strong disorder important for experiments were used. Some of them produce low divergences in certain characteristics of our strongly disordered critical systems (compared with finite values for the homogeneous case or a single impurity). For weak disorder, or for narrow distributions of the local Kondo temperatures, our exact results reveal the presence of Kondo screening of disordered ensembles of magnetic impurities by low-lying excitations of the host. We point out that our results qualitatively coincide with the data of experiments on real disordered quasi-one-dimensional antiferromagnetic systems and with the similar behavior of some heavy metallic alloys.
We discuss the two-channel Kondo problem with a pseudogap density of states $\ensuremath{\rho}(\ensuremath{\omega})\ensuremath{\propto}{|\ensuremath{\omega}|}^{r}$ of the bath fermions. Combining both analytical and numerical renormalization group techniques, we characterize the impurity phases and quantum phase transitions of the relevant Kondo and Anderson models. The line of stable points, corresponding to the overscreened non-Fermi-liquid behavior of the metallic r=0r=0r=0 case, is replaced by a stable particle-hole-symmetric intermediate-coupling fixed point for $0<r<{r}_{\mathrm{max}}\ensuremath{\approx}0.23$. For r>rmaxr>{r}_{\mathrm{max}}r>rmax​, this non-Fermi-liquid phase disappears, and instead a critical fixed point with an emergent spin-channel symmetry appears, controlling the quantum phase transition between two phases with stable spin and channel moments, respectively. We propose low-energy field theories to describe the quantum phase transitions, all being formulated in fermionic variables. We employ $\ensuremath{\epsilon}$ expansion techniques to calculate critical properties near the critical dimensions r=0r=0r=0 and 1, the latter being potentially relevant for two-channel Kondo impurities in neutral graphene. We find the analytical results to be in excellent agreement with those obtained from applying Wilson's numerical renormalization group technique.
The Luttinger Theorem, which relates the electron density to the volume of the Fermi surface in an itinerant electron system, is taken to be one of the essential features of a Fermi liquid. The microscopic derivation of this result depends on the vanishing of a certain integral, the Luttinger integral I L , which is also the basis of the Friedel sum rule for impurity models, relating the impurity occupation number to the scattering phase shift of the conduction electrons. It is known that non-zero values of I L with I L = ± π /2, occur in impurity models classified as singular Fermi liquids. Here we show the same values, I L = ± π /2, occur in an impurity model in phases with regular low energy Fermi liquid behavior. Consequently the Luttinger integral can be taken to characterize these phases, and the quantum critical points separating them interpreted as topological.