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Acta Physica Sinica

Control of population and atomic coherence by adiabatic rapid passage

Yanwei Zhou, Ye Cun-Yun, Qiang Lin, Yuzhu Wang

Published Jan 1, 2005• 2 citations
Publisher

Abstract

Robust control of atomic coherence and population transfer among Zeeman sublevel s in the ground states of atom is investigated theoretically using adiabatic rap id passage on a nanosecond time scale. It is shown that a slight change in the p ump pulse time delay relative to the Stokes pulse leads to a significant modific ation of atomic coherence and population transfer. This coherence control of qua ntum state and population is presented by numerical simulations based on self-co nsistent set of density matrix equations and Maxwell equations.

DOI
10.7498/aps.54.2799

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Robust control of atomic coherence and population transfer among Zeeman sublevel s in the ground states of atom is investigated theoretically using adiabatic rap id passage on a nanosecond time scale. It is shown that a slight change in the p ump pulse time delay relative to the Stokes pulse leads to a significant modific ation of atomic coherence and population transfer. This coherence control of qua ntum state and population is presented by numerical simulations based on self-co nsistent set of density matrix equations and Maxwell equations.
Robust control of atomic coherence and population transfer among Zeeman sublevels in the ground states of rubidium atom is investigated using adiabatic rapid passage in a nanosecond time scale, which is smaller than the lifetime of first excited Rb. It is shown that a slight change in the pump pulse time delay relative to the Stokes pulse leads to a significant modification of atomic coherence and population transfer, consequently having remarkable impacts on the generation of coherent anti-Stokes Raman scattering (CARS) signal and probe pulse absorption. This coherent control of quantum state and population is presented by numerical simulations based on self-consistent set of density matrix equations and Maxwell equations as well as experimental demonstration in rubidium atom with different atomic densities. Experimental observations are in good agreement with numerical calculations.
It introduced several methods to transfer population,including two-level system and three-level system, and gave some comparisons on transfer efficiency and transfer velocity of them in theory. It is shown that population transfer by coherent pulse sequence is better than incoherence one. Numerical simulation results showed that when using Stimulated Raman Adiabatic Rapid Passage (STIRAP), in which the pump laser pulse fully overlaps the Stokes pulse with the Stokes preceding the pump, population can be transferred completely and rapidly. Robust control of population transfer among Zeeman sublevels in the ground states of three-level system is investigated using adiabatic rapid passage in theory. The laser pulse widths are supposed to be short compared to the lifetime of the excited level, which means adiabatic. We demonstrated that techniques of STIRAP can be found to optimize population transfer in the ground states of three-level Λ system.
This paper reviews some basic techniques and theories for laser-induced incoherent population transfer schemes and resonant coherent excitation. By numerical simulations based on self-consistent set of density matrix equations and Maxwell equations, the authors have found this control can be achievable with great robustness and efficiency in nanosecond time scale using two pulses with proper selection of sequence timing to prepare the state for coherence superposition and population transfer with effective suppression of spontaneous emission.
Two approaches of achieving population transfer and coherence are investigated for the three-level Λ system in the adiabatic limit. The effects of the laser pulse sequence on the population transfer efficiency and coherence are studied. Coherent control of quantum state and population is studied by numerical simulation based on self-consistent set of density matrix equations. It can be seen that the counterintuitive pulse sequence is more efficient in population transfer and coherence than the intuitive one.
Coherent population transfer in an atom using a sequence of adiabatic rapid passages through single-photon resonances is well-known, but it requires that the frequency sweep match the changing frequencies of the atomic transitions. The same population transfer can be effected via a single multiphoton adiabatic rapid passage, which requires only a small frequency sweep, if it is possible to select the desired multiphoton transition from the many possible transitions. Here we report the observation of population transfer between Rydberg states by high order multiphoton adiabatic rapid passage.
We review and compare recent experiments and theoretical models demonstrating complete population transfer to selected states in atoms and molecules using (1) Stimulated Raman Adiabatic Rapid Passage (STIRAP) with temporally delayed but partially overlapping time dependent fundamental and Stokes fields and (2) Chirped Adiabatic Passage (CHIRAP) using frequency chirped field with the frequency swept through the resonance frequency of transitions. The transfer efficiency in these processes is unity when the adiabatic criteria are satisfied. Alignment and orientation of the initial and terminals levels of the transitions can be obtained using these methods. The dynamics involve the atomic or molecular internal angular momentum states because the Rabi frequencies for the transitions depend on the magnetic quantum numbers of the states. Full wavefunction and density matrix (necessary when spontaneous emission of the excited states plays a role) calculations are presented and adiabatic-following wavefunction and density matrix descriptions are advanced to explain unexpected experimental results.