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Physica status solidi. C, Conferences and critical reviews/Physica status solidi. C, Current topics in solid state physics

Cover Picture: Phys. Status Solidi C 9/2013

Published Sep 1, 2013• 0 citations
Publisher

Abstract

The interest in the optical control of exciton states in a quantum dot (QD) has been stimulated by recent experiments, where the QD was controlled either by means of Rabi oscillations or by using chirped laser pulses exploiting the adiabatic rapid passage (ARP). On pp. 1210–1213, Gawarecki and coworkers investigate the exciton dynamics in a quantum dot adiabatically controlled by a frequency-swept (chirped), linearly polarized laser pulse in the presence of carrier–phonon coupling. The final occupation of the exciton state is limited both due to phonon-induced transitions between the adiabatic spectral branches and because of phonon-assisted transitions to the biexciton state. When the biexciton shift is large enough, the quantum dot can be modeled as a two-level system, which corresponds to excitation with circularly polarized light. For this case the authors compare the results obtained from three different simulation methods, namely time-convolutionless method (TCL), correlation expansion (CE) and path integrals (PI). The results obtained from CE and PI show very good agreement, even at T = 50 K. The TCL agrees perfectly with the other two methods at low temperatures and agrees reasonably at moderate temperatures, but at high temperatures a mismatch of up to 30% was found.

DOI
10.1002/pssc.201390012

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The interest in the optical control of exciton states in a quantum dot (QD) has been stimulated by recent experiments, where the QD was controlled either by means of Rabi oscillations or by using chirped laser pulses exploiting the adiabatic rapid passage (ARP). On pp. 1210–1213, Gawarecki and coworkers investigate the exciton dynamics in a quantum dot adiabatically controlled by a frequency-swept (chirped), linearly polarized laser pulse in the presence of carrier–phonon coupling. The final occupation of the exciton state is limited both due to phonon-induced transitions between the adiabatic spectral branches and because of phonon-assisted transitions to the biexciton state. When the biexciton shift is large enough, the quantum dot can be modeled as a two-level system, which corresponds to excitation with circularly polarized light. For this case the authors compare the results obtained from three different simulation methods, namely time-convolutionless method (TCL), correlation expansion (CE) and path integrals (PI). The results obtained from CE and PI show very good agreement, even at T = 50 K. The TCL agrees perfectly with the other two methods at low temperatures and agrees reasonably at moderate temperatures, but at high temperatures a mismatch of up to 30% was found.
Abstract We study the evolution of a quantum dot controlled by a frequency‐swept (chirped), linearly polarized laser pulse in the presence of carrier‐phonon coupling. The final occupation of the exciton state is limited both due to phonon‐induced transitions between the adiabatic spectral branches and because of phonon‐assisted transitions to the biexcitostate. When the biexciton shift is large enough, the quantum dot can be modeled as a two‐level system, which corresponds to excitation with circularly polarized light. For this case, we compare different methods of simulations: (i) a time convolutionless method, (ii) correlation expansion and (iii) path integrals. We show that results obtained from these methods agree perfectly at temperatur. (© 2013 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps and moderate pulse areas.
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, then the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps, and moderate pulse areas.
An exciton in a quantum dot (QD) strongly couples to light, allowing the ultrafast manipulation of the quantum states on the order of femtoseconds [1]. Since a QD exciton can be regarded as a two-level system, the excitonic state can be manipulated coherently via Rabi oscillations depending on the electric field of the excitation pulse and the resonant frequency of the QD exciton. However, uniformly manipulating the exciton ensemble in a large number of QDs using ultrashort pulses is quite difficult due to the inhomogeneous distributions of the excitonic resonant frequency and the laser intensity for each QD. Adiabatic rapid passage (ARP) has been demonstrated to overcome this problem because it provides a quantum manipulation technique robust over the inhomogeneities [2], [3] by using chirped pulses (CP) instead of using Fourier transform-limited pulses (TLP). While ARP has been studied extensively in two-level systems with inhomogeneous linewidths up to GHz, it has not been rarely applied to two-level systems with THz inhomogeneous linewidths such as QDs. In this work, we experimentally demonstrate the ultrafast coherent transfer of the exciton population via ARP in two kinds of QD samples; 150-layer stacked InAs QDs and 50-layer stacked InAs QDs embedded in a resonator (Fig. 1(a)).
The energy states in semiconductor quantum dots are discrete as in atoms, and quantum states can be coherently controlled with resonant laser pulses. Long coherence times allow the observation of Rabi-flopping of a single dipole transition in a solid state device, for which occupancy of the upper state depends sensitively on the dipole moment and the excitation laser power. We report on the robust preparation of a quantum state using an optical technique that exploits rapid adiabatic passage from the ground to an excited state through excitation with laser pulses whose frequency is swept through the resonance.
The energy states in semiconductor quantum dots are discrete as in atoms, and quantum states can be coherently controlled with resonant laser pulses. Long coherence times allow the observation of Rabi flopping of a single dipole transition in a solid state device, for which occupancy of the upper state depends sensitively on the dipole moment and the excitation laser power. We report on the robust population inversion in a single quantum dot using an optical technique that exploits rapid adiabatic passage from the ground to an excited state through excitation with laser pulses whose frequency is swept through the resonance. This observation in photoluminescence experiments is made possible by introducing a novel optical detection scheme for the resonant electron hole pair (exciton) generation.