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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Ultrafast Uniformed Quantum Manipulation with Chirped Pulses in InAs Quantum Dot Ensemble with Resonator

Yushiro Takahashi, Kotaro Miyauchi, Yutaro Kinoshita, Kouichi Akahane, Junko Ishi‐Hayase

Published Jun 26, 2023• 0 citations
Publisher

Abstract

An exciton in a quantum dot (QD) strongly couples to light, allowing the ultrafast manipulation of the quantum states on the order of femtoseconds [1]. Since a QD exciton can be regarded as a two-level system, the excitonic state can be manipulated coherently via Rabi oscillations depending on the electric field of the excitation pulse and the resonant frequency of the QD exciton. However, uniformly manipulating the exciton ensemble in a large number of QDs using ultrashort pulses is quite difficult due to the inhomogeneous distributions of the excitonic resonant frequency and the laser intensity for each QD. Adiabatic rapid passage (ARP) has been demonstrated to overcome this problem because it provides a quantum manipulation technique robust over the inhomogeneities [2], [3] by using chirped pulses (CP) instead of using Fourier transform-limited pulses (TLP). While ARP has been studied extensively in two-level systems with inhomogeneous linewidths up to GHz, it has not been rarely applied to two-level systems with THz inhomogeneous linewidths such as QDs. In this work, we experimentally demonstrate the ultrafast coherent transfer of the exciton population via ARP in two kinds of QD samples; 150-layer stacked InAs QDs and 50-layer stacked InAs QDs embedded in a resonator (Fig. 1(a)).

DOI
10.1109/cleo/europe-eqec57999.2023.10231847

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An exciton in a quantum dot (QD) strongly couples to light, allowing the ultrafast manipulation of the quantum states on the order of femtoseconds [1]. Since a QD exciton can be regarded as a two-level system, the excitonic state can be manipulated coherently via Rabi oscillations depending on the electric field of the excitation pulse and the resonant frequency of the QD exciton. However, uniformly manipulating the exciton ensemble in a large number of QDs using ultrashort pulses is quite difficult due to the inhomogeneous distributions of the excitonic resonant frequency and the laser intensity for each QD. Adiabatic rapid passage (ARP) has been demonstrated to overcome this problem because it provides a quantum manipulation technique robust over the inhomogeneities [2], [3] by using chirped pulses (CP) instead of using Fourier transform-limited pulses (TLP). While ARP has been studied extensively in two-level systems with inhomogeneous linewidths up to GHz, it has not been rarely applied to two-level systems with THz inhomogeneous linewidths such as QDs. In this work, we experimentally demonstrate the ultrafast coherent transfer of the exciton population via ARP in two kinds of QD samples; 150-layer stacked InAs QDs and 50-layer stacked InAs QDs embedded in a resonator (Fig. 1(a)).
Photon echo (PE) techniques offer a promising approach to optical quantum memory, yet their implementation in conventional platforms, such as rare-earth-ion-doped crystals, is hindered by limited bandwidths. Semiconductor quantum dot (QD) ensembles, featuring THz-scale inhomogeneous broadening and sub-picosecond dynamics, provide an attractive alternative for ultrafast applications. However, achieving coherent control across such broad spectral ranges remains challenging due to detuning and spatial field inhomogeneities, which reduce PE efficiency. In this work, we demonstrate that chirped rephasing pulses satisfying adiabatic conditions enable robust adiabatic rapid passage (ARP) across an inhomogeneously broadened InAs QD ensemble. This approach achieves uniform population inversion and broadband rephasing, overcoming the limitations of transform-limited excitation. Experimentally, we observe a 3.2-fold enhancement of the PE signal in dense, self-assembled InAs QDs operating at telecom wavelengths. Numerical simulations based on a two-level model reproduce the experimentally observed ARP-induced enhancement, validating the underlying physical mechanism. These results establish ARP as an effective and scalable method for coherent control in THz-broadened QD ensembles, opening a pathway toward ultrafast and broadband optical quantum memory and communication in the telecom band.
We demonstrate electrically controlled robust state preparation of an exciton qubit by rapid adiabatic passage with Fourier-limited laser pulses. In our approach, resonant ps laser pulses are applied to generate excitonic population in a quantum dot, whereas synchronously applied ps electric transients provide a controlled sweep of the exciton transition energy. The ps electric transients applied to the quantum dot in a diode structure result in ultrafast Stark shifts of the exciton energy on time scales below the decoherence time of the exciton. We experimentally demonstrate that the tailored electric chirp of the exciton energy leads to a controlled rapid adiabatic passage, which results in a robust state preparation of the exciton. Our experimental results are confirmed by a theoretical analysis of the chirped coherent manipulation of the exciton two level system. Our approach toward optoelectronic quantum control paves the way for broader applications that require a scalable control of functional coherent systems.
In quantum information technology, it is necessary to develop a light-matter quantum interface that transfers and stores quantum information. As a bandwidth of quantum entangled photon pairs used for quantum information increases, a quantum interface with broad bandwidth will be required. The combination of quantum dot (QD) ensemble and photon echo (PE) method is one of promising methods for broadband quantum interface. Since the bandwidth of the quantum interface using this method is limited only by the inhomogeneous width of the QDs, it is possible to implement a quantum interface with the bandwidth of 10 THz at telecommunication wavelength. However, in the PE method, the spatial inhomogeneousity of the laser intensity and the inhomogeneousity of the resonance frequency of the QDs result in the uniform quantum control of excitons in QDs. As a result, the regeneration efficiency of the PE light is significantly deteriorated. To solve this problem, it is effective to introduce a quantum control method using chirped pulses (Adaptive Rapid Passages; ARPs) which is robust to inhomogeneousities. In this study, we demonstrate that the regeneration efficiency of PE in inhomogeneous QDs can be improved by ARPs using femtosecond pulses. By performing numerical simulation and optical experiments, it was found that the regeneration efficiency improves as the chirp amount and the pulse area increase, and saturates at a certain condition.
Two quantum control spectroscopic techniques were applied to study InAs quantum dot (QD) devices, which contain different strain-reducing layers. By adaptively control light matter interaction, a delayed resonant response from the InAs QDs was found to be encoded into the optimal phase profile of ultrafast optical pulse used. We verified the delayed resonant response to originate from excitons coupled to acoustic phonons of InAs QDs with two-dimensional coherent spectroscopy. Our study yields valuable dynamical information that can deepen our understanding of the coherent coupling process of exciton in the quantum-confined systems.