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Proceedings of IEEE Sensors/Proceedings of IEEE Sensors ...

A fast determination method for identifying the spin exchange relaxation free regime of atomic magnetometer

Yanzhang Wang, Xue Zhang, Jianan Qin, Chen Chen

Published Oct 1, 2016• 1 citation
Publisher

Abstract

Spin-exchange-relaxation-free (SERF) atomic magnetometer is the most sensitive magnetic detector in the world at present due to the fact that the broadening of spin-exchange collision is eliminated by operating at high alkali-mental density and low magnetic field. On that condition, the precession frequency of high-density alkali vapor becomes a constant fractional value of Larmor frequency, and the width of magnetic-resonance line gets narrower. This paper analyzes the principle of SERF regime and proposes an innovation based on measuring the slowing-down Larmor frequency directly instead of the complicated conventional method based on the width of magnetic resonance line. We calculated and simulated the slowing-down precession frequency and linewidth of magnetic resonance on certain conditions. The experimental results have verified that the method is valid to identify the regime of SERF of atomic magnetometer via detecting the slowing-down precession frequency.

DOI
10.1109/icsens.2016.7808790

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Spin-exchange-relaxation-free (SERF) atomic magnetometer is the most sensitive magnetic detector in the world at present due to the fact that the broadening of spin-exchange collision is eliminated by operating at high alkali-mental density and low magnetic field. On that condition, the precession frequency of high-density alkali vapor becomes a constant fractional value of Larmor frequency, and the width of magnetic-resonance line gets narrower. This paper analyzes the principle of SERF regime and proposes an innovation based on measuring the slowing-down Larmor frequency directly instead of the complicated conventional method based on the width of magnetic resonance line. We calculated and simulated the slowing-down precession frequency and linewidth of magnetic resonance on certain conditions. The experimental results have verified that the method is valid to identify the regime of SERF of atomic magnetometer via detecting the slowing-down precession frequency.
Spin-exchange relaxation-free (SERF) atomic magnetometers seem to be the state-of-the-art magnetic sensors today as they have achieved a sensitivity of femtotesla in the elimination of broadening contribution of spin-exchange collisions operated in the mode of SERF regime. In order to extend the practicability of SERF atomic magnetometry in superb performances in a movable platform, ensuring and testing the working status of alkali atoms are of great importance. Given the fact that in the premise of SERF regime, the linewidth of magnetic resonance would be narrowing down and the precession frequency would become a constant fractional value of the Larmor frequency for alkali atoms, we measure the gyromagnetic ratio of weakly polarized alkali-metal vapor by yielding the damped oscillating curves and fitting measured increments of frequency and magnetic field to identify the working regime of alkali atoms in a fast and straightforward manner. The experimental results have good agreements with theoretical analysis and simulation, and the whole measurement process lasts milliseconds with relatively measured error ±1% in the temperature range of T = 156 °C-184 °C. To testify the validity of the innovation, magnetic resonance line is obtained in the same condition proffering the width comparative with the outcome from simulation, indicating the spin-exchange broadening has been eliminated, presenting the same conclusion with innovation, and providing systematic sensitivity 30 fT/Hz1/2.
A novel method to determine the spin polarization and its distribution for a spin-exchange relaxation-free (SERF) atomic magnetometer are proposed in this paper. The Larmor precession frequency is measured using the fast Fourier transform (FFT) analysis result of the transient response of the magnetometer under the excitation of a series of the step-changed magnetic field. The spin polarization is extracted from the slow-down factor of the precession frequency. The variation of the spin polarization with different pump light intensities and the distribution of the spin polarization along the direction of the pump light are analyzed, and the experimental results are well consistent with the theoretical predictions. The expanded uncertainties of the experimental results vary from 2% to 11% with the increase of the spin polarization and the reason for this variation is analyzed. The advantage of this method is that it allows the accurate measurement of the spin polarization in the pump beam direction within the SERF regime operating state, and it is unaffected by the large optical depth of the vapor cell.
The spin-exchange relaxation-free (SERF) atomic magnetometer (AM) has vital importance in advanced research and has been widely applied in different fields. To improve the sensitivity and robustness of SERF magnetometers, understanding the relaxation mechanism is a significant approach. By controlling the amplitude and direction of external magnetic fields, and switching statuses of the pump and probe laser beam, we measured both the transverse and longitudinal relaxation rate in two experimental methods, respectively, and obtained the Larmor precession frequency, the spin-exchange relaxation rate, the spin-destruction relaxation rate, and the relaxation rate due to collisions between atoms and vapor cell walls. All experimental results are verified with the theoretical calculations. The final longitudinal relaxation rate of our magnetometer is 53 Hz. Furthermore, we measured the sensitivity of our SERF magnetometer reaching 5 fT/Hz1/2 from 5 to 70 Hz after differential measurement with the 3-dB bandwidth of 70 Hz. Our work helps to improve the detection capability of SERF magnetometers, providing performance assurance for searching for exotic spin-dependent interactions and applications, including magnetoencephalograms and magnetocardiograms.
This paper presents a method for measuring the spin polarization of spin-exchange relaxation-free (SERF) atomic magnetometers at extremely large optical depths. Owing to the slowing-down effect, the spin polarization can be extracted by measuring the slowing-down factor extracted from the precession frequency. However, this technique is limited by a significant error in the regime of extremely large optical depths, where the pump beam intensity for achieving the optimized spin polarization of alkali atoms is significantly increased. We observed that the instantaneous precession frequency measured in the regime where the spin-exchange rate is not much larger than the Larmor frequency was no longer a constant but varied with the pump beam intensity. Thus, a method for measuring spin polarization based on the ratio of the precession frequency to the measured instantaneous precession frequency is proposed. Based on the proposed method, the spin polarization at a temperature of 473K and optical depth of 64 is measured. The measurement results were accordant with theoretical analysis. The expanded uncertainties of the experimental results varied between 1.8% and 9.6%. The proposed method is also applicable to other atomic devices operated in the SERF regime with extremely large optical depths, such as co-magnetometers and atomic spin gyroscopes.
Abstract A single-beam spin-exchange relaxation-free (SERF) atomic magnetometer can extract vector magnetic field information by detecting the transmission intensity of a resonant circularly polarized pumping beam, which depends sensitively on the atomic density of the alkali metal. We present a novel scheme to determine atomic density based on zero-field magnetic resonance. The resonance linewidth under different transverse DC magnetic fields is fitted by means of a quadratic function. The atomic density can be extracted from the quadratic coefficients of the fitted function. The experimental results indicate that the deviation of measured density is less than two times compared with the theoretical values between 378 K and 403 K. Furthermore, the influence of modulation field on resonance linewidth is investigated experimentally and theoretically. A miniature single-beam SERF atomic magnetometer with a sensor head volume of only 16.2 cm 3 and the measuring sensitivity of 40 fT/ Hz 1/2 has been achieved. These results should be beneficial for guiding the development of a chip-scale atomic magnetometer with high sensitivity and spatial resolution for bio-magnetic field imaging applications.
In this paper, we experimentally study transient dynamics of spin polarized atoms in the spin-exchange-relaxation-free (SERF) regime with a single-beam configuration. We pumped atoms with a weak detuning pumping beam, along with a sequence of magnetic field pulses orthogonal to the pumping beam were applied. The dynamics of atomic spin, which experiences Larmor precession under the perturbation of magnetic field, is detected by the transmitted pumping beam. Benefited from the long coherence time of atomic spin in the SERF regime, the dependence of precession frequency and decay rate, which is equal to the magnetic resonance linewidth of atomic spin, on magnetic fields is studied with the transient dynamics of atomic spin in the limit of low spin polarization. Moreover, we demonstrate that coil constants can be calibrated by analyzing the precession frequency of the transient dynamics of atomic spin. And the experimental results show that the coil constants are 114.25 ± 0.02 nT/mA and 114.12 ± 0.04 nT/mA in x- and y-axis, respectively. This method is particularly applicable to study the atomic spin dynamics and calibrate the coil constant in situ of a miniature single-beam SERF magnetometer.