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IEEE Transactions on Instrumentation and Measurement

Measuring Spin Polarization of a Spin-Exchange Relaxation-Free Atomic Magnetometer at Extremely Large Optical Depths

Yanning Ma, Jixi Lu, Ke Yang, Zixuan Wang, Yaoguo Wang, Bowen Sun, Yueyang Zhai, Bangcheng Han

Published Jan 1, 2022• 8 citations
Publisher

Abstract

This paper presents a method for measuring the spin polarization of spin-exchange relaxation-free (SERF) atomic magnetometers at extremely large optical depths. Owing to the slowing-down effect, the spin polarization can be extracted by measuring the slowing-down factor extracted from the precession frequency. However, this technique is limited by a significant error in the regime of extremely large optical depths, where the pump beam intensity for achieving the optimized spin polarization of alkali atoms is significantly increased. We observed that the instantaneous precession frequency measured in the regime where the spin-exchange rate is not much larger than the Larmor frequency was no longer a constant but varied with the pump beam intensity. Thus, a method for measuring spin polarization based on the ratio of the precession frequency to the measured instantaneous precession frequency is proposed. Based on the proposed method, the spin polarization at a temperature of 473K and optical depth of 64 is measured. The measurement results were accordant with theoretical analysis. The expanded uncertainties of the experimental results varied between 1.8% and 9.6%. The proposed method is also applicable to other atomic devices operated in the SERF regime with extremely large optical depths, such as co-magnetometers and atomic spin gyroscopes.

DOI
10.1109/tim.2022.3207824

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This paper presents a method for measuring the spin polarization of spin-exchange relaxation-free (SERF) atomic magnetometers at extremely large optical depths. Owing to the slowing-down effect, the spin polarization can be extracted by measuring the slowing-down factor extracted from the precession frequency. However, this technique is limited by a significant error in the regime of extremely large optical depths, where the pump beam intensity for achieving the optimized spin polarization of alkali atoms is significantly increased. We observed that the instantaneous precession frequency measured in the regime where the spin-exchange rate is not much larger than the Larmor frequency was no longer a constant but varied with the pump beam intensity. Thus, a method for measuring spin polarization based on the ratio of the precession frequency to the measured instantaneous precession frequency is proposed. Based on the proposed method, the spin polarization at a temperature of 473K and optical depth of 64 is measured. The measurement results were accordant with theoretical analysis. The expanded uncertainties of the experimental results varied between 1.8% and 9.6%. The proposed method is also applicable to other atomic devices operated in the SERF regime with extremely large optical depths, such as co-magnetometers and atomic spin gyroscopes.
A novel method to determine the spin polarization and its distribution for a spin-exchange relaxation-free (SERF) atomic magnetometer are proposed in this paper. The Larmor precession frequency is measured using the fast Fourier transform (FFT) analysis result of the transient response of the magnetometer under the excitation of a series of the step-changed magnetic field. The spin polarization is extracted from the slow-down factor of the precession frequency. The variation of the spin polarization with different pump light intensities and the distribution of the spin polarization along the direction of the pump light are analyzed, and the experimental results are well consistent with the theoretical predictions. The expanded uncertainties of the experimental results vary from 2% to 11% with the increase of the spin polarization and the reason for this variation is analyzed. The advantage of this method is that it allows the accurate measurement of the spin polarization in the pump beam direction within the SERF regime operating state, and it is unaffected by the large optical depth of the vapor cell.
Spin-exchange-relaxation-free (SERF) atomic magnetometer is the most sensitive magnetic detector in the world at present due to the fact that the broadening of spin-exchange collision is eliminated by operating at high alkali-mental density and low magnetic field. On that condition, the precession frequency of high-density alkali vapor becomes a constant fractional value of Larmor frequency, and the width of magnetic-resonance line gets narrower. This paper analyzes the principle of SERF regime and proposes an innovation based on measuring the slowing-down Larmor frequency directly instead of the complicated conventional method based on the width of magnetic resonance line. We calculated and simulated the slowing-down precession frequency and linewidth of magnetic resonance on certain conditions. The experimental results have verified that the method is valid to identify the regime of SERF of atomic magnetometer via detecting the slowing-down precession frequency.
It is demonstrated that a spin-exchange relaxation-free (SERF) atomic magnetometer can be used for scalar measurements with no additional hardware. Because of relaxation processes, an ensemble of alkali atoms needs a constant supply of polarized photons by a pump beam to maintain a polarized state. If the pump beam is shuttered off, the system decays to its equilibrium state. For a low enough relaxation rate and with a magnetic field present, the system will exhibit oscillations at its natural frequencies. In a SERF magnetometer, it happens at the Zeeman resonance frequency of the atoms (Larmor frequency). Thus, shuttering off the pump beam reveals oscillations at the Larmor frequency. From this frequency, one can deduce the scalar value of the applied magnetic field. As a result, all-optical scalar measurements can be performed. At the same time, either one or two vector components of the applied field can be measured by using one or two orthogonal probe beams, respectively. In a low-polarization SERF regime, the ground state can be well described by the Bloch equations for the electron spin polarization. By solving the time-dependent Bloch equations [neglecting the diffusion term and assuming that the nuclear slowing-down factor q(P) is constant], the oscillation frequency of the system is obtained. From this frequency, the scalar value of the applied magnetic field is derived. It is shown that applied fields down to 1 nT can be measured with a 0.1% relative uncertainty. Fields down to 50 pT can be measured with a 10% relative uncertainty. The time dependence acquired in the “off” periods is strongly correlated with the Zeeman sublevels population of the atomic ground state and reveals its spin dynamics.
The measurement of atomic spin polarization distribution in spin-exchange relaxation free (SERF) magnetometer is an important topic for improving the sensitivity and consistency of multi-channel magnetic field measurement applications. A novel spin polarization spatial distribution measurement method is presented based on the transient response of the magnetometer after modulating the pumped light with a chopper. Polarization is obtained by a slow-down factor based on the fast spin-exchange interaction effects. Longitudinal and transverse polarization distributions are measured simultaneously without interrupting the operation of the SERF status. Under different oscillating magnetic fields, the spin polarization is measured at the cell centroid. Residual magnetic field inside the magnetometer is obtained from the linear relationship between the precession frequency and the oscillating magnetic field. The one-dimensional polarization distributions in the x, y, and z axes are measured using a digital micromirror device with a resolution of 0.25 cm. The measurement results conform to the Lambert-Bier absorption law and the Gaussian distribution law. Furthermore, 7 × 7 two-dimensional spatial distribution measurements of polarization on the xy and yz planes are performed. Nonuniformity of 1.04 in the xy plane and 1.82 in the yz plane in the built magnetometer. Compared with other measurement methods, the distribution measurement method proposed is independent of optical depth and suitable for low polarization and high polarization applications. Based on the results of the proposed measurement method of spin polarization spatial distribution, further compensation can improve the application consistency of multi-channel magnetic field measurements and improve the sensitivity of single-channel differential measurements.
Spin-exchange relaxation-free (SERF) atomic magnetometers seem to be the state-of-the-art magnetic sensors today as they have achieved a sensitivity of femtotesla in the elimination of broadening contribution of spin-exchange collisions operated in the mode of SERF regime. In order to extend the practicability of SERF atomic magnetometry in superb performances in a movable platform, ensuring and testing the working status of alkali atoms are of great importance. Given the fact that in the premise of SERF regime, the linewidth of magnetic resonance would be narrowing down and the precession frequency would become a constant fractional value of the Larmor frequency for alkali atoms, we measure the gyromagnetic ratio of weakly polarized alkali-metal vapor by yielding the damped oscillating curves and fitting measured increments of frequency and magnetic field to identify the working regime of alkali atoms in a fast and straightforward manner. The experimental results have good agreements with theoretical analysis and simulation, and the whole measurement process lasts milliseconds with relatively measured error ±1% in the temperature range of T = 156 °C-184 °C. To testify the validity of the innovation, magnetic resonance line is obtained in the same condition proffering the width comparative with the outcome from simulation, indicating the spin-exchange broadening has been eliminated, presenting the same conclusion with innovation, and providing systematic sensitivity 30 fT/Hz1/2.
In this paper, we experimentally study transient dynamics of spin polarized atoms in the spin-exchange-relaxation-free (SERF) regime with a single-beam configuration. We pumped atoms with a weak detuning pumping beam, along with a sequence of magnetic field pulses orthogonal to the pumping beam were applied. The dynamics of atomic spin, which experiences Larmor precession under the perturbation of magnetic field, is detected by the transmitted pumping beam. Benefited from the long coherence time of atomic spin in the SERF regime, the dependence of precession frequency and decay rate, which is equal to the magnetic resonance linewidth of atomic spin, on magnetic fields is studied with the transient dynamics of atomic spin in the limit of low spin polarization. Moreover, we demonstrate that coil constants can be calibrated by analyzing the precession frequency of the transient dynamics of atomic spin. And the experimental results show that the coil constants are 114.25 ± 0.02 nT/mA and 114.12 ± 0.04 nT/mA in x- and y-axis, respectively. This method is particularly applicable to study the atomic spin dynamics and calibrate the coil constant in situ of a miniature single-beam SERF magnetometer.