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Microfabricated Atomic Clocks at NIST

Svenja A. Knappe, Peter D. D. Schwindt, Vladislav P. Gerginov, Vishal Shah, Leo W. Hollberg, John E. Kitching, Li‐Anne Liew, John Moreland

Published Dec 1, 2004• 3 citations
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Abstract

This paper presents the latest progress in the development, fabrication, and characterization of microfabricated atomic frequency references at NIST. With volumes below 10 mm3 the physics packages contain the complete integrated assembly for probing the ground-state hyperfine splitting frequency of the alkali atoms by coherent population trapping (CPT). This technique allows for a simple and compact device containing a vertical-cavity surface-emitting laser (VCSEL), optics to shape the laser beam, a vapor cell containing the atoms, and a detector. We present an improved technique for microfabricating the miniature alkali vapor cells. When integrated into a CPT clock, a clear reduction of long-term frequency drifts is observed. This leads to a fractional frequency instability of less than 10-11 at one hour of integration, a more than one order of magnitude improvement over previous results. We identify the remaining sensitivities of the clock frequency to environmental influences and propose ways to reduce them.

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Applied Sciences•Jan 3, 2022•20 citations
This paper presents the latest progress in the development, fabrication, and characterization of microfabricated atomic frequency references at NIST. With volumes below 10 mm3 the physics packages contain the complete integrated assembly for probing the ground-state hyperfine splitting frequency of the alkali atoms by coherent population trapping (CPT). This technique allows for a simple and compact device containing a vertical-cavity surface-emitting laser (VCSEL), optics to shape the laser beam, a vapor cell containing the atoms, and a detector. We present an improved technique for microfabricating the miniature alkali vapor cells. When integrated into a CPT clock, a clear reduction of long-term frequency drifts is observed. This leads to a fractional frequency instability of less than 10-11 at one hour of integration, a more than one order of magnitude improvement over previous results. We identify the remaining sensitivities of the clock frequency to environmental influences and propose ways to reduce them.
A novel technique for microfabricating alkali atom vapor cells is described in which alkali atoms are evaporated into a micromachined cell cavity through a glass nozzle. A cell of interior volume 1 mm3, containing 87Rb and a buffer gas, was made in this way and integrated into an atomic clock based on coherent population trapping. A fractional frequency instability of 6 x 10(-12) at 1000 s of integration was measured. The long-term drift of the F=1, mF=0-->F=2, mF=0 hyperfine frequency of atoms in these cells is below 5 x 10(-11)/day.
Coherent population trapping (CPT) resonances usually exhibit contrasts below 10% when interrogated with frequency modulated lasers. We discuss a relatively simple way to increase the resonance contrast to nearly 100% generating an additional light field through a nonlinear four-wave mixing interaction in the atomic vapor.1 A similar method can also be used to create a beat signal at the CPT resonance frequency that can injection-lock a low-power microwave oscillator at 3.4 GHz directly to the atomic resonance.2 This could lead to chip-scale atomic clocks (CSACs) with improved performance. Furthermore, we introduce a miniature microfabricated saturated absorption spectrometer3 that produces a signal for locking a laser frequency to optical transitions in alkali atoms. The Rb absorption spectra are comparable to signals obtained with standard table-top setups, although the rubidium vapor cell has an interior volume of only 1 mm3 and the volume of the entire spectrometer is around 0.1 cm3.
The spectroscopic technique of coherent population trapping (CPT) enables an all-optical interrogation of the groundstate hyperfine splitting of cesium (or rubidium), compared to the optical-microwave double resonance technique conventionally employed in atomic frequency standards. All-optical interrogation enables the reduction of the size and power consumption of an atomic clock by two orders of magnitude, and vertical-cavity surface-emitting lasers (VCSELs) are preferred optical sources due to their low power consumption and circular output beam. Several research teams are currently using VCSELs for DARPA's chip-scale atomic clock (CSAC) program with the goal of producing an atomic clock having a volume < 1 cm^3, a power consumption < 30 mW, and an instability (Allan deviation) < 1x10^-11 during a 1-hour averaging interval. This paper describes the VCSEL requirements for CPT-based atomic clocks, which include single mode operation, single polarization operation, modulation bandwidth > 4 GHz, low power consumption (for the CSAC), narrow linewidth, and low relative intensity noise (RIN). A significant manufacturing challenge is to reproducibly obtain the required wavelength at the specified VCSEL operating temperature and drive current. Data are presented that show the advantage of operating at the D1 (rather than D2) resonance of the alkali atoms. Measurements of VCSEL linewidth will be discussed in particular, since atomic clock performance is especially sensitive to this parameter.
We demonstrate a microfabricated atomic clock physics package based on coherent population trapping (CPT) on the D1 line of 87Rb atoms. The package occupies a volume of 12 mm3 and requires 195 mW of power to operate at an ambient temperature of 200 degrees C. Compared to a previous microfabricated clock exciting the D2 transition in Cs [1], this 87Rb clock shows significantly improved short- and long-term stability. The instability at short times is 4 x?10-11 / tau?/2 and the improvement over the Cs device is due mainly to an increase in resonance amplitude. At longer times (tau?> 50 s), the improvement results from the reduction of a slow drift to ?5 x 10-9 / day. The drift is most likely caused by a chemical reaction of nitrogen and barium inside the cell. When probing the atoms on the D1 line, spin-exchange collisions between Rb atoms and optical pumping appear to have increased importance compared to the D2 line.
We have undertaken the development of a chip-scale atomic clock (CSAC) whose design goals include short-term stability, sigma(sub y)(tau=1 hour), of 1x10(exp 11) with a total power consumption of 30 mW and an overall device volume of 1 cu cm. The stringent power requirement dominates the physics package architecture, dictating a small (<5 mm(exp 3) gaseous atomic ensemble interrogated by a low-power semiconductor laser. At PTTI 2002, we reported on initial experimental investigations leading to the decision to employ the coherent population trapping (CPT) interrogation technique. This paper describes our further progress on the CSAC effort, including the development of custom vertical cavity surface emitting laser (VCSEL) sources and techniques for microfabricating miniature cesium vapor cells comprised of anodically bonded silicon and glass. Measurements of the signal contrast and linewidth of both the cesium D1 and D2 resonance transitions are compared, and frequency stability measurements of the CSAC testbed are presented.
Herein, a microfabricated millimeter-level vapor alkali cell with a high hermeticity is fabricated through a wet etching and single-chip anodic bonding process. The vapor cell, containing Rb and N2, was investigated in a coherent population trapping (CPT) setup for the application of a chip-scale atomic clock (CSAC). The contrast of CPT resonance is up to 1.1% within the only 1 mm length of light interacting with atom. The effects of some critical external parameters on the CPT resonance, such as laser intensity, cell temperature, and buffer gas pressure, are thoroughly studied and optimized. The improved microfabricated vapor cell also exhibited great potential for other chip-scale atomic devices.