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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Short optical pulse refraction by a thin film of atoms at two-photon resonance

S. O. Elyutin, Andrei I. Maimistov

Published Jan 14, 2000• 0 citations
Publisher

Abstract

A refraction of short pulses by a thin film of atoms at two- photon resonance is numerically considered with the process of third harmonic generation involved in analysis. It is shown that a light pulse, being refracted by a tin film of resonance atoms, decays into subpulses, which number is determined by the energy penetrated in the film. The process depends on the angle of incidence. The variation of the resonance detuning allows compensating Stark effect and creating the preferable conditions for light pulse transmission. The effect of local field is similar in its action to the Stark effect, but its contribution to the frequency shift could be significant only in the media with greater concentration of the resonance atoms.

DOI
10.1117/12.375327

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A refraction of short pulses by a thin film of atoms at two- photon resonance is numerically considered with the process of third harmonic generation involved in analysis. It is shown that a light pulse, being refracted by a tin film of resonance atoms, decays into subpulses, which number is determined by the energy penetrated in the film. The process depends on the angle of incidence. The variation of the resonance detuning allows compensating Stark effect and creating the preferable conditions for light pulse transmission. The effect of local field is similar in its action to the Stark effect, but its contribution to the frequency shift could be significant only in the media with greater concentration of the resonance atoms.
The refraction of a short pulse by a thin film of atoms at two-photon resonance is numerically considered with the process of third harmonic generation involved in the analysis. It is shown that a light pulse, being refracted by a thin film of resonance atoms, decays into subpulses, whose number is determined by the energy penetrating the film. The process depends on the angle of incidence. The variation on the resonance detuning allows compensation of the Stark effect and creation of preferable conditions for light pulse transmission. The effect of local field is similar in its action to the Stark effect, but its contribution to the frequency shift could be significant only in media with a greater concentration of the resonance atoms.
Refraction of a double-frequency optical pulse at the interface between two linear dielectrics containing a thin film of resonant atoms is considered. The dynamics of the system is treated based on the model of three-level atoms with the V -type energy diagram. Refraction of short and long (compared with the Rabi oscillation period) pulses is analyzed with allowance for local-field effects. In both cases, the shape of the pulse corresponding to one carrier wave frequency is shown to depend on the energy of the pulse with the other carrier wave frequency. In particular, both the frequency and the depth of the amplitude modulation arising in the refracted pulse are changed.
The problem of the interaction of an ultrashort optical pulse and a thin film of resonant atoms under the conditions of two-photon absorption, third-harmonic generation, and the inverse effect of the latter on the pump pulse via Raman scattering is studied. The fact that the field acting on an atom differs from the macroscopic field in the film is also taken into consideration. It is shown that the polarization of the film undergoes dynamic relaxation even in the absence of irreversible relaxation, suppressing Rabi oscillations and establishing stationary values of the populations of the resonant energy levels and of the polarization of the film at the pump and the third-harmonic frequencies.
Numerical and analytic investigations are made of the reflection and propagation of short optical pulses through an inverted thin film consisting of two-level atoms. An analysis is made of cases where pulses having rectangular, hyperbolic-secant, and Gaussian profiles are incident normally on a thin film. It is shown that, as a result of the initial inversion of the atoms, induced superradiance occurs. The dependences of the parameters of the reflected and transmitted pulses on the characteristics of the incident pulse are determined.
The refraction is theoretically considered of ultra-short pulses at interface of two dielectrics that contains a thin film of nonlinear material featured by the negative refractive index in a certain frequency band. For the models of meta-material composed of nanoparticles and magnetic nanocircuits (split-ring resonators), the equations are obtained suitable for describing the coherent responses: photon echo, optical nutations, and harmonic generation. The numerical simulation demonstrates the emergence of photon echo in inhomogeneous system of meta-atoms. It is supposed that the reported methods are applicable for investigation of thin meta-material films.
Abstract We have studied the nonstationary transmission of two ultrashort laser pulses incident on a thin film. The radiation frequency of one of these pulses is in resonance with the two-photon transition from the ground state of the crystal to the biexciton state, while the other pulse coherently mixes the exciton and biexciton states, leading to strong renormalization of the energy spectrum of the crystal. We have obtained a system of nonlinear equations describing the time evolution of the exciton and biexciton amplitudes and the fields of three pulses transmitted through the film. We have analyzed the effect of amplitudes and widths of incident pulsed and of the time delay between them on the peculiarities of film transmission of these pulses. We have predicted the effect of a substantial time delay in the generation of the pulse transmitted through the film relative to the incident pulse, which is in resonance with the exciton–biexciton transition frequency. The possibility of generation of a precursor, viz., a pulse transmitted through the film sooner than the peak of the incident pulse reaches the film, as well as possibility of generation of a reflected pulse in the absence of the incident pulse, has been proven.