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Journal of Experimental and Theoretical Physics

Two-photon interaction of coherent radiation with a thin film of resonant atoms

Ashat M. Basharov, Andrei I. Maimistov, S. O. Elyutin

Published Jan 1, 1999• 6 citations
Publisher

Abstract

The problem of the interaction of an ultrashort optical pulse and a thin film of resonant atoms under the conditions of two-photon absorption, third-harmonic generation, and the inverse effect of the latter on the pump pulse via Raman scattering is studied. The fact that the field acting on an atom differs from the macroscopic field in the film is also taken into consideration. It is shown that the polarization of the film undergoes dynamic relaxation even in the absence of irreversible relaxation, suppressing Rabi oscillations and establishing stationary values of the populations of the resonant energy levels and of the polarization of the film at the pump and the third-harmonic frequencies.

DOI
10.1134/1.558757

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The problem of the interaction of an ultrashort optical pulse and a thin film of resonant atoms under the conditions of two-photon absorption, third-harmonic generation, and the inverse effect of the latter on the pump pulse via Raman scattering is studied. The fact that the field acting on an atom differs from the macroscopic field in the film is also taken into consideration. It is shown that the polarization of the film undergoes dynamic relaxation even in the absence of irreversible relaxation, suppressing Rabi oscillations and establishing stationary values of the populations of the resonant energy levels and of the polarization of the film at the pump and the third-harmonic frequencies.
The refraction of a short pulse by a thin film of atoms at two-photon resonance is numerically considered with the process of third harmonic generation involved in the analysis. It is shown that a light pulse, being refracted by a thin film of resonance atoms, decays into subpulses, whose number is determined by the energy penetrating the film. The process depends on the angle of incidence. The variation on the resonance detuning allows compensation of the Stark effect and creation of preferable conditions for light pulse transmission. The effect of local field is similar in its action to the Stark effect, but its contribution to the frequency shift could be significant only in media with a greater concentration of the resonance atoms.
A refraction of short pulses by a thin film of atoms at two- photon resonance is numerically considered with the process of third harmonic generation involved in analysis. It is shown that a light pulse, being refracted by a tin film of resonance atoms, decays into subpulses, which number is determined by the energy penetrated in the film. The process depends on the angle of incidence. The variation of the resonance detuning allows compensating Stark effect and creating the preferable conditions for light pulse transmission. The effect of local field is similar in its action to the Stark effect, but its contribution to the frequency shift could be significant only in the media with greater concentration of the resonance atoms.
Refraction of a double-frequency optical pulse at the interface between two linear dielectrics containing a thin film of resonant atoms is considered. The dynamics of the system is treated based on the model of three-level atoms with the V -type energy diagram. Refraction of short and long (compared with the Rabi oscillation period) pulses is analyzed with allowance for local-field effects. In both cases, the shape of the pulse corresponding to one carrier wave frequency is shown to depend on the energy of the pulse with the other carrier wave frequency. In particular, both the frequency and the depth of the amplitude modulation arising in the refracted pulse are changed.
A theory of coherent interaction between a sequence of ultrashort laser pulses and planar, thin-film microcavities in the form of Fabry-Perot resonators containing resonating atoms has been developed. The dynamics of transmission of single laser pulses has been analyzed numerically. Analytic solutions of the problem of four-wave mixing of optical fields separated in time have been obtained in the small-area approximation. The dynamic efficiency of conversion of incident waves to the coherent response field (photon echo) generated in a microcavity can be higher than in the case of a bulk resonant structure. Specific features of photon echo generation in a microcavity for arbitrary “areas” of laser pump pulses are discussed.
A numerical investigation is made of third harmonic generation (THG) under conditions of two-photon resonance between the fundamental frequency and a selected transition in the atoms of a medium. It is shown that under conditions of coherent interaction between the pump pulse and the medium, a THG efficiency of ∼20% or higher may be achieved. In this case, THG in the form of high-power ultrashort pulses may be obtained. It is shown that experimental observation of similar effects in specific media should not present particular difficulties.
We investigate the problem of resonant re flection and transmission of an ultrashort light pulse passing through a medium consisting of two-level atoms. We show that for a thin layer it is important to take into account the difference between the external macroscopic field and the field acting on the individual atoms within the medium. The local field correction leads to an inversion dependent resonant frequency. In thin layers this generates a new mechanism of nonlinear transparency induced by the dynamical frequency shift. When the excitation frequency is larger than the original resonant frequency, then the transmission of the layer exhibits bistable behavior.