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Optics and Spectroscopy

Resonant interaction of light with a thin film of three-level atoms

S. O. Elyutin, Andrei I. Maimistov

Published May 1, 2001• 2 citations
Publisher

Abstract

Refraction of a double-frequency optical pulse at the interface between two linear dielectrics containing a thin film of resonant atoms is considered. The dynamics of the system is treated based on the model of three-level atoms with the V -type energy diagram. Refraction of short and long (compared with the Rabi oscillation period) pulses is analyzed with allowance for local-field effects. In both cases, the shape of the pulse corresponding to one carrier wave frequency is shown to depend on the energy of the pulse with the other carrier wave frequency. In particular, both the frequency and the depth of the amplitude modulation arising in the refracted pulse are changed.

DOI
10.1134/1.1374667

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Refraction of a double-frequency optical pulse at the interface between two linear dielectrics containing a thin film of resonant atoms is considered. The dynamics of the system is treated based on the model of three-level atoms with the V -type energy diagram. Refraction of short and long (compared with the Rabi oscillation period) pulses is analyzed with allowance for local-field effects. In both cases, the shape of the pulse corresponding to one carrier wave frequency is shown to depend on the energy of the pulse with the other carrier wave frequency. In particular, both the frequency and the depth of the amplitude modulation arising in the refracted pulse are changed.
The refraction of a short pulse by a thin film of atoms at two-photon resonance is numerically considered with the process of third harmonic generation involved in the analysis. It is shown that a light pulse, being refracted by a thin film of resonance atoms, decays into subpulses, whose number is determined by the energy penetrating the film. The process depends on the angle of incidence. The variation on the resonance detuning allows compensation of the Stark effect and creation of preferable conditions for light pulse transmission. The effect of local field is similar in its action to the Stark effect, but its contribution to the frequency shift could be significant only in media with a greater concentration of the resonance atoms.
A refraction of short pulses by a thin film of atoms at two- photon resonance is numerically considered with the process of third harmonic generation involved in analysis. It is shown that a light pulse, being refracted by a tin film of resonance atoms, decays into subpulses, which number is determined by the energy penetrated in the film. The process depends on the angle of incidence. The variation of the resonance detuning allows compensating Stark effect and creating the preferable conditions for light pulse transmission. The effect of local field is similar in its action to the Stark effect, but its contribution to the frequency shift could be significant only in the media with greater concentration of the resonance atoms.
The problem of the interaction of an ultrashort optical pulse and a thin film of resonant atoms under the conditions of two-photon absorption, third-harmonic generation, and the inverse effect of the latter on the pump pulse via Raman scattering is studied. The fact that the field acting on an atom differs from the macroscopic field in the film is also taken into consideration. It is shown that the polarization of the film undergoes dynamic relaxation even in the absence of irreversible relaxation, suppressing Rabi oscillations and establishing stationary values of the populations of the resonant energy levels and of the polarization of the film at the pump and the third-harmonic frequencies.
We consider the propagation of extremely short pulses through a dielectric thin film containing resonant atoms (two-level atoms) with permanent dipole. Assuming that the film width is less than the field wavelength, we can solve the wave equation and reduce the problem to a system of generalized Bloch equations describing the resonant atoms. We compute the stationary solutions for a constant irradiation of the film. Superimposing a small amplitude linear wave we calculate the reflection and transmission coefficients. From these, one can then deduce the different parameters of the model. We believe that this technique could be used in experiments to obtain the medium atomic and relaxation parameters.
We consider the propagation of extremely short pulses through a dielectric thin film containing resonant atoms (two level atoms) with permanent dipole. Assuming that the film width is less than the field wave length, we can solve the wave equation and reduce the problem to a system of generalized Bloch equations describing the resonant atoms. We compute the stationary solutions for a constant irradiation of the film. Superimposing a small amplitude linear wave we compute the reflection and transmission coefficients. From these, one can then deduce the different parameters of the model. We believe this technique could be used in experiments to obtain the medium atomic and relaxation parameters.
The refraction is theoretically considered of ultra-short pulses at interface of two dielectrics that contains a thin film of nonlinear material featured by the negative refractive index in a certain frequency band. For the models of meta-material composed of nanoparticles and magnetic nanocircuits (split-ring resonators), the equations are obtained suitable for describing the coherent responses: photon echo, optical nutations, and harmonic generation. The numerical simulation demonstrates the emergence of photon echo in inhomogeneous system of meta-atoms. It is supposed that the reported methods are applicable for investigation of thin meta-material films.