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Journal of Experimental and Theoretical Physics Letters

Effect of nonlinear wave mixing on ultrafast modulation of interband light in semiconductor quantum wells

Arup Neogi

Published Sep 1, 1997• 1 citation
Publisher

Abstract

We investigate the effect of an induced sum-frequency signal on the transient modulation of interband-resonant probe light by a train of intersubband-resonant coupling light pulses in undoped quantum wells. The origin of the generated sum-frequency signal lies in the asymmetry of the three-level quantum well structure. The modulation characteristics are found to be significantly affected in the presence of a strong sum-frequency signal that builds up proportionately to the input probe field.

DOI
10.1134/1.567529

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We investigate the effect of an induced sum-frequency signal on the transient modulation of interband-resonant probe light by a train of intersubband-resonant coupling light pulses in undoped quantum wells. The origin of the generated sum-frequency signal lies in the asymmetry of the three-level quantum well structure. The modulation characteristics are found to be significantly affected in the presence of a strong sum-frequency signal that builds up proportionately to the input probe field.
The interband sum frequency generation process due to three-wave interaction of interband and intersubband coupling lights has been investigated in a semiconductor quantum well using the perturbational density matrix approach. The origin of the nonlinear process lies in the second-order susceptibility /spl chi//sub c2-h1//sup (2)/ arising due to the optical transition between the second conduction subband and the first heavy hole state. Both the sign and the magnitude of the second-order susceptibility of the well may be controlled by the carrier density level and the frequency of the intersubband field.
We explore the transient characteristics of an interband resonant light modulation process by ultrashort intersubband resonant light pulses in semiconductor quantum wells (QW's). The modulation characteristics in a three-level semiconductor QW system, including the effects due to in-plane momentum, have been investigated by a numerical analysis of the coupled Bloch equations using a density-matrix approach. We have studied the effect of the carrier density and the nature of the intersubband coupling light on the transient absorption features of the interband light. The modulation process has been compared in doped and undoped QW's. The switching behavior of the strong interband light field in presence of a train of intersubband light pulses has also been discussed.
We analyze the optical modulation of an interband resonant light pulse by intersubband resonant light pulses in a three-level quantum well system. The origin of the third order self-saturation optical nonlinearity resulting in the modification of the interband light absorption is assumed to lie in the carrier density modulation induced by the interband and intersubband transitions. The optical nonlinearity can be optimized to achieve the maximum modulation by applying control light pulses shorter than the intersubband energy relaxation time but longer than the intersubband phase relaxation time. We have also experimentally investigated the material system suitable for optical communication regime and have observed that the In0.53Ga0.47As/AlAs0.56Sb0.44 quantum well lattice matched to InP yielding an intersubband transition as short as 1.4 μm is the most suitable system for the proposed modulation scheme.
We investigate the interband difference-frequency-generation process arising from the three-wave interaction of resonant interband and intersubband coupling lights by theoretical estimation of the linear and the nonlinear susceptibilities of an asymmetric AlGaAs–GaAs quantum well. The three-level quantum-well system is analyzed by the perturbational density-matrix approach. The effect of the variation of carrier density in the quantum well on the interband mixing process is also considered. The nonlinear polarization induced by the intersubband coupling field is significantly enhanced in the case of doped structures. The peak second-order susceptibility estimated at the difference frequency is more than 2 orders of magnitude larger, whereas the coupling-field-induced third-order susceptibility is more than 4 orders of magnitude larger than that of bulk GaAs.
An efficient modulation scheme at relatively lower control light intensities is proposed using ultrashort interband and intersubband-resonant coupling light pulses in a novel asymmetric In x Ga1-x As/AlAs semiconductor quantum well structure. The shape of the intersubband-control light pulses can manipulate the interband-signal light pulse absorption. The carrier relaxation rate of the quantum well system can be estimated from the interband nonlinear optical parameters induced by the intersubband control light field. The modulation efficiency in the proposed structure is twice than in a conventional symmetric quantum well structure. This reduces the threshold optical energy below 1 pJ in a 100-µm2 waveguide structure on using 500 fs control light pulses owing to the enhanced optical nonlinearities in the proposed structure.