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Physics Letters A

Absolute measures of mean lifetimes of excited states using the method of correlated photons in cascade

C. Camhy-Val, A. M. Dumont, M. Dreux, R. Vitry

Published Jul 1, 1970• 22 citations
Publisher
DOI
10.1016/0375-9601(70)90295-1

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We present lifetime measurements of the 5D3∕25{D}_{3∕2}5D3∕2​ and 5D5∕25{D}_{5∕2}5D5∕2​ states of rubidium using the time-correlated single-photon-counting method. We perform the experiment in a magneto-optical trap of 87Rb^{87}\mathrm{Rb}87Rb atoms using a two-step excitation with the trap laser at 780nm780\phantom{\rule{0.3em}{0ex}}\mathrm{nm}780nm as the first step. We record the 761.9nm761.9\phantom{\rule{0.3em}{0ex}}\mathrm{nm}761.9nm fluorescence from the decay of the 5D3∕25{D}_{3∕2}5D3∕2​ state to the 5P1∕25{P}_{1∕2}5P1∕2​ state, and measure the lifetime of the 5D3∕25{D}_{3∕2}5D3∕2​ state $\ensuremath{\tau}=246.3(1.6)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$. We record the 420.2nm420.2\phantom{\rule{0.3em}{0ex}}\mathrm{nm}420.2nm fluorescence from the cascade decay of the 5D5∕25{D}_{5∕2}5D5∕2​ state to the 5S1∕25{S}_{1∕2}5S1∕2​ state through the 6P3∕26{P}_{3∕2}6P3∕2​ state, and extract the lifetime of the 5D5∕25{D}_{5∕2}5D5∕2​ state $\ensuremath{\tau}=238.5(2.3)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$.