We have developed an interesting and widely applicable technique for measuring lifetimes of low-lying levels of neutral atoms and their first few ionization states. The cascade-photon-coincidence method has been extended by using a light source consisting of excited atoms sputtered from a solid by 10-keV argon ions. We have measured the lifetimes of the
4p2P3/2o state of Ca II, the
6p2P3/2o state of Ba II, and the
4p2P3/2o state of Al III. These measurements are in good agreement with earlier work.
We present lifetime measurements of the
5D3∕2 and
5D5∕2 states of rubidium using the time-correlated single-photon-counting method. We perform the experiment in a magneto-optical trap of
87Rb atoms using a two-step excitation with the trap laser at
780nm as the first step. We record the
761.9nm fluorescence from the decay of the
5D3∕2 state to the
5P1∕2 state, and measure the lifetime of the
5D3∕2 state $\ensuremath{\tau}=246.3(1.6)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$. We record the
420.2nm fluorescence from the cascade decay of the
5D5∕2 state to the
5S1∕2 state through the
6P3∕2 state, and extract the lifetime of the
5D5∕2 state $\ensuremath{\tau}=238.5(2.3)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$.