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Atomic lifetime measurements by the method of correlation photons in a cascade

A. M. Dumont

Published Nov 1, 1976• 0 citations
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We have developed an interesting and widely applicable technique for measuring lifetimes of low-lying levels of neutral atoms and their first few ionization states. The cascade-photon-coincidence method has been extended by using a light source consisting of excited atoms sputtered from a solid by 10-keV argon ions. We have measured the lifetimes of the ${4\mathrm{p}}^{2}$${\mathrm{P}}_{3\mathrm{/}2}^{\mathrm{o}}$ state of Ca II, the ${6\mathrm{p}}^{2}$${\mathrm{P}}_{3\mathrm{/}2}^{\mathrm{o}}$ state of Ba II, and the ${4\mathrm{p}}^{2}$${\mathrm{P}}_{3\mathrm{/}2}^{\mathrm{o}}$ state of Al III. These measurements are in good agreement with earlier work.

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Lifetime measurements of the 5d states of rubidium

D. Sheng, A. Pérez Galván, Luis A. Orozco

We present lifetime measurements of the $5{D}_{3∕2}$ and $5{D}_{5∕2}$ states of rubidium using the time-correlated single-photon-counting method. We perform the experiment in a magneto-optical trap of $^{87}\mathrm{Rb}$ atoms using a two-step excitation with the trap laser at $780\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ as the first step. We record the $761.9\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ fluorescence from the decay of the $5{D}_{3∕2}$ state to the $5{P}_{1∕2}$ state, and measure the lifetime of the $5{D}_{3∕2}$ state $\ensuremath{\tau}=246.3(1.6)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$. We record the $420.2\phantom{\rule{0.3em}{0ex}}\mathrm{nm}$ fluorescence from the cascade decay of the $5{D}_{5∕2}$ state to the $5{S}_{1∕2}$ state through the $6{P}_{3∕2}$ state, and extract the lifetime of the $5{D}_{5∕2}$ state $\ensuremath{\tau}=238.5(2.3)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$.

arXiv:0811.4010•Physical Review A•Dec 15, 2008•74 citations
We have developed an interesting and widely applicable technique for measuring lifetimes of low-lying levels of neutral atoms and their first few ionization states. The cascade-photon-coincidence method has been extended by using a light source consisting of excited atoms sputtered from a solid by 10-keV argon ions. We have measured the lifetimes of the 4p2{4\mathrm{p}}^{2}4p2P3/2o{\mathrm{P}}_{3\mathrm{/}2}^{\mathrm{o}}P3/2o​ state of Ca II, the 6p2{6\mathrm{p}}^{2}6p2P3/2o{\mathrm{P}}_{3\mathrm{/}2}^{\mathrm{o}}P3/2o​ state of Ba II, and the 4p2{4\mathrm{p}}^{2}4p2P3/2o{\mathrm{P}}_{3\mathrm{/}2}^{\mathrm{o}}P3/2o​ state of Al III. These measurements are in good agreement with earlier work.
We present lifetime measurements of the 5D3∕25{D}_{3∕2}5D3∕2​ and 5D5∕25{D}_{5∕2}5D5∕2​ states of rubidium using the time-correlated single-photon-counting method. We perform the experiment in a magneto-optical trap of 87Rb^{87}\mathrm{Rb}87Rb atoms using a two-step excitation with the trap laser at 780nm780\phantom{\rule{0.3em}{0ex}}\mathrm{nm}780nm as the first step. We record the 761.9nm761.9\phantom{\rule{0.3em}{0ex}}\mathrm{nm}761.9nm fluorescence from the decay of the 5D3∕25{D}_{3∕2}5D3∕2​ state to the 5P1∕25{P}_{1∕2}5P1∕2​ state, and measure the lifetime of the 5D3∕25{D}_{3∕2}5D3∕2​ state $\ensuremath{\tau}=246.3(1.6)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$. We record the 420.2nm420.2\phantom{\rule{0.3em}{0ex}}\mathrm{nm}420.2nm fluorescence from the cascade decay of the 5D5∕25{D}_{5∕2}5D5∕2​ state to the 5S1∕25{S}_{1∕2}5S1∕2​ state through the 6P3∕26{P}_{3∕2}6P3∕2​ state, and extract the lifetime of the 5D5∕25{D}_{5∕2}5D5∕2​ state $\ensuremath{\tau}=238.5(2.3)\phantom{\rule{0.3em}{0ex}}\mathrm{ns}$.