The velocities of atoms can be manipulated by near-resonant laser light. After many absorption-spontaneous emission cycles momentum is transferred to the atoms in the direction of the laser beam. In this way atoms can be slowed down and cooled to milliKelvin temperatures and below. In three mutually orthogonal pairs of counter-propagating laser beams in combination with a magnetic field atoms can be cooled and trapped. In this so-called magneto-optical trap (MOT) two atoms can be excited to a
molecular state by absorption of a photon. This technique is called photoassociation spectroscopy. In our case we study metastable helium atoms, which have a large internal energy. When two metastable helium
atoms approach each other, one of the atoms ionizes and the ions are detected by a microchannelplates detector. When a probe laser beam is directed onto the MOT cloud and scanned in frequency, atom pairs can
be excited to several ro-vibrational states. In the excited state the metastable helium atoms are accelerated towards each other and ionize at short internuclear distance. The ro-vibrational states appear as peaks in
the ionization signal and from the position of these states information on the excited state interaction potential can be extracted.
The velocities of atoms can be manipulated by near-resonant laser light. After many absorption-spontaneous emission cycles momentum is transferred to the atoms in the direction of the laser beam. In this way atoms can be slowed down and cooled to milliKelvin temperatures and below. In three mutually orthogonal pairs of counter-propagating laser beams in combination with a magnetic field atoms can be cooled and trapped. In this so-called magneto-optical trap (MOT) two atoms can be excited to a
molecular state by absorption of a photon. This technique is called photoassociation spectroscopy. In our case we study metastable helium atoms, which have a large internal energy. When two metastable helium
atoms approach each other, one of the atoms ionizes and the ions are detected by a microchannelplates detector. When a probe laser beam is directed onto the MOT cloud and scanned in frequency, atom pairs can
be excited to several ro-vibrational states. In the excited state the metastable helium atoms are accelerated towards each other and ionize at short internuclear distance. The ro-vibrational states appear as peaks in
the ionization signal and from the position of these states information on the excited state interaction potential can be extracted.
The high velocity of free atoms associated with the thermal motion, together with the velocity distribution of atoms has imposed the ultimate limitation on the precision of ultrahigh resolution spectroscopy. A sample consisting of low velocity atoms would provide a substantial improvement in spectroscopy resolution. To overcome the problem of thermal motion, atomic physicists have pursued two goals; first, the reduction of the thermal motion (cooling); and second, the confinement of the atoms by means of electromagnetic fields (trapping). Cooling carried sufficiently far, eliminates the motional problems, whereas trapping allows for long observation times. In this work the laser cooling and trapping of an argon atomic beam will be discussed. The experiments involve a time-of-flight spectroscopy on metastable argon atoms. Laser deceleration or cooling of atoms is achieved by counter propagating a photon against an atomic beam of metastable atoms. The solution to the Doppler shift problem is achieved using spatially varying magnetic field along the beam path to Zeeman shift the atomic resonance frequency so as to keep the atoms in resonance with a fixed frequency cooling laser. For trapping experiments a Magnetooptical trap (MOT) will be used. The MOT is formed by three pairs of counter-propagating laser beams with mutual opposite circular polarization and a frequency tuned slightly below the center of the atomic resonance and superimposed on a magnetic quadrupole field.
The main subject of this thesis is to demonstrate that helium is a promising candidate for matter wave interferometry, with the goal of providing an improved value for the fine-structure constant, α. In particular, fast and efficient momentum transfer via Bloch oscillations in an optical lattice is demonstrated, together with the enhanced sensitivity offered by an ion-detector based detection scheme that is unique to metastable helium (He*). The experiments are performed in a setup that was built to produce, slow down and trap ultracold (~0.2 μK) He-4 atoms. The approach to realising an ultracold sample of He* atoms consists of a sequence of trapping and cooling stages. The experiment starts at the plasma discharge source, where helium atoms are excited to the so-called metastable 2-3S1 state, with a lifetime of ~7800 seconds, 20 eV above the atomic ground state. The atomic beam exiting from the source is 2-D collimated by 1083 nm laser light, resonant to the closed 2-3S1 - 2-3P2 cooling transition. Next, the atoms are slowed down from about 1000- to 50 m/s in a two meter long Zeeman slower through continuous absorption of resonant 1083 nm light. The slowed atoms are captured in a Magneto-Optical Trap (MOT), that holds up to 5x10^8 atoms at a temperature of 1 mK. The MOT cloud is compressed, spin-polarised and transferred to a cloverleaf Magnetic Trap (MT), which provides both axial and radial trapping through a set of coils outside the vacuum. In the MT, 1D-Doppler cooling is applied to the atomic sample to reduce the temperature to about 150 μK. Following this step, the temperature is reduced further by forced evaporative radio-frequency cooling, resulting in the onset of a Bose-Einstein Condensate (BEC). The atoms are transferred from the MT to a crossed horizontal optical dipole trap (ODT), in which the sample is further evaporatively cooled to produce a BEC of 5x10^6 atoms. The BEC is then transferred from the ODT to either a horizontal or vertical optical lattice, consisting of two counter-propagating laser beams at 1557 nm. By detuning the frequency of one of the lattice beams, the standing wave can be accelerated. The trapped helium atoms can follow the accelerating lattice through a process called Bloch oscillations (BO's), which describes the behaviour of particles in a periodic potential that are subjected to a force. Specifically, in this scenario, particles' velocities increase in increments of two recoil velocities, instead of continuously. Bloch oscillations of cold atoms in periodic potentials formed by optical lattices were first studied in 1996. Importantly, BO’s provide a way to efficiently accelerate atoms by coherently transferring a well controlled, large number of photon momenta, which has been used to increase the resolution of recoil measurements with caesium and rubidium atoms. In this thesis, Bloch oscillations with a metastable helium BEC are demonstrated. Due to its light mass, helium can be efficiently accelerated to high velocities which makes it a candidate for experiments that benefit from splitting the atomic wave-function over large distances. Additionally, Rabi-oscillations in an optical lattice are shown, which serve to probe the depth of the lattice, and a measurement of gravity through Bloch oscillations in a static vertical optical lattice is demonstrated, with a statistical uncertainty of 4x10^-5. Finally, the first proof of principle demonstration of a pulsed light He* atom interferometer is shown. The measurements illustrate the high signal-to-noise that can be obtained using an MCP detector. Next to that, we have demonstrated a method for determining the polarizability of atoms at specific wavelengths, by observing the induced change of the characteristic Bloch oscillation frequency by introducing that wavelength to the system.
The advent of the laser opened the way to the development of powerful new methods for manipulating and cooling atoms which were exploited in the realization of Bose–Einstein condensation in alkali atom vapours. To set the stage we describe a typical experiment, which is shown schematically in Fig. 4.1. A beam of sodium atoms emerges from an oven at a temperature of about 600 K, corresponding to a speed of about 800 m s –1 , and is then passed through a so-called Zeeman slower, in which the velocity of the atoms is reduced to about 30 m s –1 , corresponding to a temperature of about 1 K. In the Zeeman slower, a laser beam propagates in the direction opposite that of the atomic beam, and the radiation force produced by absorption of photons retards the atoms. Due to the Doppler effect, the frequency of the atomic transition in the laboratory frame is not generally constant, since the atomic velocity varies. However, by applying an inhomogeneous magnetic field designed so that the Doppler and Zeeman effects cancel, the frequency of the transition in the rest frame of the atom may be held fixed. On emerging from the Zeeman slower the atoms are slow enough to be captured by a magneto-optical trap (MOT), where they are further cooled by interactions with laser light to temperatures of order 100 μK. Another way of compensating for the changing Doppler shift is to increase the laser frequency in time, which is referred to as ‘chirping’. In other experiments the MOT is filled by transferring atoms from a second MOT where atoms are captured directly from the vapour.
The helium dimer in its metastable triplet state is a promising candidate to be the first laser-cooled homonuclear molecule. An ultracold gas of He2∗ would enable a new generation of precision measurements to test quantum electrodynamics for three- and four-electron molecules through Rydberg spectroscopy. Nearly diagonal Franck-Condon factors are obtained because the electron employed for optical cycling occupies a Rydberg orbital that does not take part in the chemical bond. Three possible laser cooling transitions are identified and the spin-rovibronic energy-level structure of the relevant states as well as electronic transition moments, linestrengths, and lifetimes are determined. The production of He2∗ molecules in a supersonic beam is discussed, and a laser slowing scheme to load a magneto-optical trap under such conditions is simulated using a rate equation approach. Various repumping schemes involving one or two upper electronic states are compared to maximize the radiative force. Loss mechanisms such as spin-forbidden transitions, predissociation, and ionization processes are studied and found to not introduce significant challenges for laser cooling and trapping He2∗. The sensitivity of the vibrational levels of He2+ with respect to the static polarizability of atomic helium is determined and its implications for a new quantum pressure standard are discussed.
We have constructed a magneto-optical trap (MOT) for metastable triplet helium atoms utilizing the $2{}^{3}{S}_{1}\ensuremath{\rightarrow}3{}^{3}{P}_{2}$ line at 389 nm as the trapping and cooling transition. The far-red-detuned MOT (detuning $\ensuremath{\Delta}=\ensuremath{-}41\mathrm{MHz})$ typically contains few times 107 atoms at a relatively high $(\ensuremath{\sim}{10}^{9}{\mathrm{cm}}^{\ensuremath{-}3})$ density, which is a consequence of the large momentum transfer per photon at 389 nm and a small two-body loss rate coefficient $(2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}10}{\mathrm{cm}}^{3}/\mathrm{s}<\ensuremath{\beta}<1.0\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}{\mathrm{cm}}^{3}/\mathrm{s}).$ The two-body loss rate is more than five times smaller than in a MOT on the commonly used $2{}^{3}{S}_{1}\ensuremath{\rightarrow}2{}^{3}{P}_{2}$ line at 1083 nm. Furthermore, laser cooling at 389 nm results in temperatures somewhat lower than those achieved using 1083 nm. The 389-nm MOT exhibits small losses due to two-photon ionization, which have been investigated as well.
During the last decades the study of cold atoms has grown in a great measure. Research in this field has been made possible due to the development of laser cooling and trapping techniques. We use laser cooling to cool helium atoms down to a temperature of 1 mK and we are able to trap 106 atoms in our magneto-optical trap. The helium atoms are in a metastable state, the He 23S1 state, which has a lifetime of more than 2 hours. With cold atoms phenomena can be studied that are not accessible using thermal atoms, such as high resolution spectroscopy. Furthermore cold atoms are the first step towards Bose-Einstein condensation. Cold alkali-metal atoms have been extensively studied, using photoassociation spectroscopy. In this thesis the first photoassociation results for rare gas atoms, namely metastable helium atoms will be discussed. Various experiments are described and an analysis of the results is given.