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Bloch Oscillations of Metastable Helium in an optical lattice

Rudolf F.H.J. van der Beek

Published Mar 17, 2021• 0 citations
OpenAlex

Abstract

The main subject of this thesis is to demonstrate that helium is a promising candidate for matter wave interferometry, with the goal of providing an improved value for the fine-structure constant, α. In particular, fast and efficient momentum transfer via Bloch oscillations in an optical lattice is demonstrated, together with the enhanced sensitivity offered by an ion-detector based detection scheme that is unique to metastable helium (He*). The experiments are performed in a setup that was built to produce, slow down and trap ultracold (~0.2 μK) He-4 atoms. The approach to realising an ultracold sample of He* atoms consists of a sequence of trapping and cooling stages. The experiment starts at the plasma discharge source, where helium atoms are excited to the so-called metastable 2-3S1 state, with a lifetime of ~7800 seconds, 20 eV above the atomic ground state. The atomic beam exiting from the source is 2-D collimated by 1083 nm laser light, resonant to the closed 2-3S1 - 2-3P2 cooling transition. Next, the atoms are slowed down from about 1000- to 50 m/s in a two meter long Zeeman slower through continuous absorption of resonant 1083 nm light. The slowed atoms are captured in a Magneto-Optical Trap (MOT), that holds up to 5x10^8 atoms at a temperature of 1 mK. The MOT cloud is compressed, spin-polarised and transferred to a cloverleaf Magnetic Trap (MT), which provides both axial and radial trapping through a set of coils outside the vacuum. In the MT, 1D-Doppler cooling is applied to the atomic sample to reduce the temperature to about 150 μK. Following this step, the temperature is reduced further by forced evaporative radio-frequency cooling, resulting in the onset of a Bose-Einstein Condensate (BEC). The atoms are transferred from the MT to a crossed horizontal optical dipole trap (ODT), in which the sample is further evaporatively cooled to produce a BEC of 5x10^6 atoms. The BEC is then transferred from the ODT to either a horizontal or vertical optical lattice, consisting of two counter-propagating laser beams at 1557 nm. By detuning the frequency of one of the lattice beams, the standing wave can be accelerated. The trapped helium atoms can follow the accelerating lattice through a process called Bloch oscillations (BO's), which describes the behaviour of particles in a periodic potential that are subjected to a force. Specifically, in this scenario, particles' velocities increase in increments of two recoil velocities, instead of continuously. Bloch oscillations of cold atoms in periodic potentials formed by optical lattices were first studied in 1996. Importantly, BO’s provide a way to efficiently accelerate atoms by coherently transferring a well controlled, large number of photon momenta, which has been used to increase the resolution of recoil measurements with caesium and rubidium atoms. In this thesis, Bloch oscillations with a metastable helium BEC are demonstrated. Due to its light mass, helium can be efficiently accelerated to high velocities which makes it a candidate for experiments that benefit from splitting the atomic wave-function over large distances. Additionally, Rabi-oscillations in an optical lattice are shown, which serve to probe the depth of the lattice, and a measurement of gravity through Bloch oscillations in a static vertical optical lattice is demonstrated, with a statistical uncertainty of 4x10^-5. Finally, the first proof of principle demonstration of a pulsed light He* atom interferometer is shown. The measurements illustrate the high signal-to-noise that can be obtained using an MCP detector. Next to that, we have demonstrated a method for determining the polarizability of atoms at specific wavelengths, by observing the induced change of the characteristic Bloch oscillation frequency by introducing that wavelength to the system.

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Bloch oscillations with a metastable helium Bose-Einstein condensate

Rudolf F.H.J. van der Beek, O. Onishchenko, W. Vassen +2 more

We have observed Bloch oscillations of a ${}^{4}{\text{He}}^{*}$ Bose-Einstein condensate in an optical lattice at 1557.3 nm. Due to its low mass, metastable helium was efficiently accelerated orders of magnitude faster than demonstrated with other atoms. In a horizontal lattice, we could transfer a total of $800\ensuremath{\hbar}k$ of momentum by shuttling the atomic cloud back and forth 50 times between the $4\ensuremath{\hbar}k$ and $\ensuremath{-}4\ensuremath{\hbar}k$ momentum states with an efficiency of over 99% per Bloch cycle. In a vertical lattice, gravity-induced Bloch oscillations were demonstrated, from which the local gravitational acceleration was derived with a statistical uncertainty of $4\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}5}$. A clear advantage of ${\text{He}}^{*}$ over other atoms is that it can be detected with a microchannel plate detector with near unity efficiency, and this enabled observation of Bloch oscillations up to 12 s even though the number of atoms decreased by three orders of magnitude. These results establish ${\text{He}}^{*}$ as a promising candidate for future precision measurements with atom interferometry.

Physical Review A•Dec 21, 2020•1 citation

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This thesis describes the work done over the past three and a half years on the new metastable helium experiment at the Institut d'Optique in Palaiseau. In the first chapter it describes a study to improve both the efficiency and the accuracy of the Microchannel Plate (MCP) detection system. We have experimented with adding a gold layer on the top of the input plate, something that we have found increases the efficiency but also decreases the accuracy. The addition of a voltage between the two stacked plates has been shown to both raise the efficiency and improve the accuracy in non-coated MCPs.The second chapter is devoted to the construction of the experimental apparatus. Here the excitation of ground state helium to its metastable state is described, as well as the subsequent collimation and cooling by Zeeman slower of the resulting hot atomic beam. The slowed beam is then captured in a Magneto-Optical Trap, in which we have captured 8x108 atoms.In the third chapter an original study on three-dimensional Doppler cooling in a red-detuned molasses and in the Magneto-Optical trap is presented. The metastable helium system is unique as there is no multiple scattering of photons and there are no sub-Doppler effects. This allows for a never before seen experimental realisation of pure Doppler cooling theory. The fourth chapter describes a study on collisions in a magneto-optical trap of metastable helium. Light-induced Penning collisions are responsible for high trap losses at high intensities and at frequencies close to the transition frequency. We measure the constant rate coefficient to Ksp = 2.8 ± 0.4 x 10-7cm3/s.

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This thesis describes recent experiments conducted on a Bose-Einstein condensate in an optical waveguide. This optical potential confines the atoms against gravity in the vertical dimension, guiding them to freely propagate in the horizontal. Being supported against gravity enables long expansion times of hundreds of milliseconds, facilitating techniques such as delta-kick cooling. In an ideal atom interferometer, the beamsplitters would impart a large momentum splitting between the interfering states in order to increase the signal. However, their effective use requires both an even narrower momentum width source and good vibration isolation. Three such techniques were investigated in this thesis: reflection from a repulsive light potential barrier, Bragg transitions from an optical lattice (which are effectively bouncing atoms off a moving grating), and Bloch-acceleration by loading the atoms into such an optical lattice and then accelerating the combined system. It is found that a combination of both Bragg and Bloch provides the most promising route to truly large momentum transfer in a system which is sensitive only to acceleration. Lastly, large-momentum transfer techniques can be used to effectively increase the way in which the output signal scales with time, creating interferometers which generate the same sensitivity faster (increasing the bandwidth of a sensor), or generate a much better sensitivity in the same time. We form a dual condensate of both rubidium-85 an rubidium-87 via sympathetic cooling. The collisional properties of Rubidium-85 can be modified by applying an external magnetic field, at an easy-to-experimentally-reach value of between 150-170G. It turns out that this combination of atomic isotopes is ideal for an interferometric test of the weak equivalence principle, one of the underpinnings of General Relativity. This thesis also presents the results of the first Bose-condensed version of such a dual-species interferometer. By removing any 87Rb left after condensation, we have created a pure 85Rb BEC. Using this we can now explore how the inter-atomic interactions affect the phase shift of a condensed atom interferometer, as we have complete control over the interaction strength. A condensate with no inter-particle interactions should behave like an ideal particle. With a small attractive interaction between atoms, it is possible to create a self-trapped cloud of atoms which propagates dispersionlessly. This cloud is known as a soliton, and it is predicted to have even more interesting quantum mechanical properties. For example it is predicted that by colliding two such solitons, an entangled state can be generated. Our results indicate that the dispersionless character of the soliton out-performs all other interaction strengths in an atom interferometer, including even the non-interacting cloud.

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The velocities of atoms can be manipulated by near-resonant laser light. After many absorption-spontaneous emission cycles momentum is transferred to the atoms in the direction of the laser beam. In this way atoms can be slowed down and cooled to milliKelvin temperatures and below. In three mutually orthogonal pairs of counter-propagating laser beams in combination with a magnetic field atoms can be cooled and trapped. In this so-called magneto-optical trap (MOT) two atoms can be excited to a molecular state by absorption of a photon. This technique is called photoassociation spectroscopy. In our case we study metastable helium atoms, which have a large internal energy. When two metastable helium atoms approach each other, one of the atoms ionizes and the ions are detected by a microchannelplates detector. When a probe laser beam is directed onto the MOT cloud and scanned in frequency, atom pairs can be excited to several ro-vibrational states. In the excited state the metastable helium atoms are accelerated towards each other and ionize at short internuclear distance. The ro-vibrational states appear as peaks in the ionization signal and from the position of these states information on the excited state interaction potential can be extracted.

•Jan 19, 2004•8 citations
The main subject of this thesis is to demonstrate that helium is a promising candidate for matter wave interferometry, with the goal of providing an improved value for the fine-structure constant, α. In particular, fast and efficient momentum transfer via Bloch oscillations in an optical lattice is demonstrated, together with the enhanced sensitivity offered by an ion-detector based detection scheme that is unique to metastable helium (He*). The experiments are performed in a setup that was built to produce, slow down and trap ultracold (~0.2 μK) He-4 atoms. The approach to realising an ultracold sample of He* atoms consists of a sequence of trapping and cooling stages. The experiment starts at the plasma discharge source, where helium atoms are excited to the so-called metastable 2-3S1 state, with a lifetime of ~7800 seconds, 20 eV above the atomic ground state. The atomic beam exiting from the source is 2-D collimated by 1083 nm laser light, resonant to the closed 2-3S1 - 2-3P2 cooling transition. Next, the atoms are slowed down from about 1000- to 50 m/s in a two meter long Zeeman slower through continuous absorption of resonant 1083 nm light. The slowed atoms are captured in a Magneto-Optical Trap (MOT), that holds up to 5x10^8 atoms at a temperature of 1 mK. The MOT cloud is compressed, spin-polarised and transferred to a cloverleaf Magnetic Trap (MT), which provides both axial and radial trapping through a set of coils outside the vacuum. In the MT, 1D-Doppler cooling is applied to the atomic sample to reduce the temperature to about 150 μK. Following this step, the temperature is reduced further by forced evaporative radio-frequency cooling, resulting in the onset of a Bose-Einstein Condensate (BEC). The atoms are transferred from the MT to a crossed horizontal optical dipole trap (ODT), in which the sample is further evaporatively cooled to produce a BEC of 5x10^6 atoms. The BEC is then transferred from the ODT to either a horizontal or vertical optical lattice, consisting of two counter-propagating laser beams at 1557 nm. By detuning the frequency of one of the lattice beams, the standing wave can be accelerated. The trapped helium atoms can follow the accelerating lattice through a process called Bloch oscillations (BO's), which describes the behaviour of particles in a periodic potential that are subjected to a force. Specifically, in this scenario, particles' velocities increase in increments of two recoil velocities, instead of continuously. Bloch oscillations of cold atoms in periodic potentials formed by optical lattices were first studied in 1996. Importantly, BO’s provide a way to efficiently accelerate atoms by coherently transferring a well controlled, large number of photon momenta, which has been used to increase the resolution of recoil measurements with caesium and rubidium atoms. In this thesis, Bloch oscillations with a metastable helium BEC are demonstrated. Due to its light mass, helium can be efficiently accelerated to high velocities which makes it a candidate for experiments that benefit from splitting the atomic wave-function over large distances. Additionally, Rabi-oscillations in an optical lattice are shown, which serve to probe the depth of the lattice, and a measurement of gravity through Bloch oscillations in a static vertical optical lattice is demonstrated, with a statistical uncertainty of 4x10^-5. Finally, the first proof of principle demonstration of a pulsed light He* atom interferometer is shown. The measurements illustrate the high signal-to-noise that can be obtained using an MCP detector. Next to that, we have demonstrated a method for determining the polarizability of atoms at specific wavelengths, by observing the induced change of the characteristic Bloch oscillation frequency by introducing that wavelength to the system.
We have observed Bloch oscillations of a 4He∗{}^{4}{\text{He}}^{*}4He∗ Bose-Einstein condensate in an optical lattice at 1557.3 nm. Due to its low mass, metastable helium was efficiently accelerated orders of magnitude faster than demonstrated with other atoms. In a horizontal lattice, we could transfer a total of $800\ensuremath{\hbar}k$ of momentum by shuttling the atomic cloud back and forth 50 times between the $4\ensuremath{\hbar}k$ and $\ensuremath{-}4\ensuremath{\hbar}k$ momentum states with an efficiency of over 99% per Bloch cycle. In a vertical lattice, gravity-induced Bloch oscillations were demonstrated, from which the local gravitational acceleration was derived with a statistical uncertainty of $4\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}5}$. A clear advantage of He∗{\text{He}}^{*}He∗ over other atoms is that it can be detected with a microchannel plate detector with near unity efficiency, and this enabled observation of Bloch oscillations up to 12 s even though the number of atoms decreased by three orders of magnitude. These results establish He∗{\text{He}}^{*}He∗ as a promising candidate for future precision measurements with atom interferometry.
This thesis describes the work done over the past three and a half years on the new metastable helium experiment at the Institut d'Optique in Palaiseau. In the first chapter it describes a study to improve both the efficiency and the accuracy of the Microchannel Plate (MCP) detection system. We have experimented with adding a gold layer on the top of the input plate, something that we have found increases the efficiency but also decreases the accuracy. The addition of a voltage between the two stacked plates has been shown to both raise the efficiency and improve the accuracy in non-coated MCPs.The second chapter is devoted to the construction of the experimental apparatus. Here the excitation of ground state helium to its metastable state is described, as well as the subsequent collimation and cooling by Zeeman slower of the resulting hot atomic beam. The slowed beam is then captured in a Magneto-Optical Trap, in which we have captured 8x108 atoms.In the third chapter an original study on three-dimensional Doppler cooling in a red-detuned molasses and in the Magneto-Optical trap is presented. The metastable helium system is unique as there is no multiple scattering of photons and there are no sub-Doppler effects. This allows for a never before seen experimental realisation of pure Doppler cooling theory. The fourth chapter describes a study on collisions in a magneto-optical trap of metastable helium. Light-induced Penning collisions are responsible for high trap losses at high intensities and at frequencies close to the transition frequency. We measure the constant rate coefficient to Ksp = 2.8 ± 0.4 x 10-7cm3/s.
This thesis describes recent experiments conducted on a Bose-Einstein condensate in an optical waveguide. This optical potential confines the atoms against gravity in the vertical dimension, guiding them to freely propagate in the horizontal. Being supported against gravity enables long expansion times of hundreds of milliseconds, facilitating techniques such as delta-kick cooling. In an ideal atom interferometer, the beamsplitters would impart a large momentum splitting between the interfering states in order to increase the signal. However, their effective use requires both an even narrower momentum width source and good vibration isolation. Three such techniques were investigated in this thesis: reflection from a repulsive light potential barrier, Bragg transitions from an optical lattice (which are effectively bouncing atoms off a moving grating), and Bloch-acceleration by loading the atoms into such an optical lattice and then accelerating the combined system. It is found that a combination of both Bragg and Bloch provides the most promising route to truly large momentum transfer in a system which is sensitive only to acceleration. Lastly, large-momentum transfer techniques can be used to effectively increase the way in which the output signal scales with time, creating interferometers which generate the same sensitivity faster (increasing the bandwidth of a sensor), or generate a much better sensitivity in the same time. We form a dual condensate of both rubidium-85 an rubidium-87 via sympathetic cooling. The collisional properties of Rubidium-85 can be modified by applying an external magnetic field, at an easy-to-experimentally-reach value of between 150-170G. It turns out that this combination of atomic isotopes is ideal for an interferometric test of the weak equivalence principle, one of the underpinnings of General Relativity. This thesis also presents the results of the first Bose-condensed version of such a dual-species interferometer. By removing any 87Rb left after condensation, we have created a pure 85Rb BEC. Using this we can now explore how the inter-atomic interactions affect the phase shift of a condensed atom interferometer, as we have complete control over the interaction strength. A condensate with no inter-particle interactions should behave like an ideal particle. With a small attractive interaction between atoms, it is possible to create a self-trapped cloud of atoms which propagates dispersionlessly. This cloud is known as a soliton, and it is predicted to have even more interesting quantum mechanical properties. For example it is predicted that by colliding two such solitons, an entangled state can be generated. Our results indicate that the dispersionless character of the soliton out-performs all other interaction strengths in an atom interferometer, including even the non-interacting cloud.
In this thesis, a transportable setup of an Yb atomic source for a lattice optical clock is built and characterized. All three laser setups for cooling and trapping the Yb atoms, together with the vacuum system, are contained on a transportable optical table. The preparation of the atomic sample before doing spectroscopy on the clock transition starts by slowing the atoms in the Zeeman slower. This is followed by trapping the atoms in the pre-cooling and the post-cooling MOTs, before loading the atoms into the optical lattice. Slowing and pre-cooling the atoms is done using the strong transition at 399 nm. This cools the atoms down to around a mK. To successfully load the atoms in the optical lattice, we have to cool the atoms further to beyond 50 μK. This is done by exciting the weak transition at 556 nm. The atoms that are transferred into the post-cooling stage are cooled down to a few tens of μK. The atoms are then ready to be loaded into the optical lattice at the magic wavelength. The amplified laser light at 760 nm inside the 1-D intra-vacuum cavity results in a lattice trapping potential of approximately 50 μK. A transfer efficiency, from the MOT into the optical lattice, of more than 25% was measured. The spectroscopy on the clock transition was done for 171Yb. A step-by-step mechanism was adopted, starting by exciting the forbidden transition at 578 nm inside the post-cooling stage MOT, by using the ”chopped-MOT” method. The 300 kHz Doppler-broadened line is then narrowed down to 3 kHz by switching on the light at 760 nm, while keeping the MOT on. The so-called ”chopped-lattice” technique helped suppress the Doppler-broadening; however the other effects due to the light and the magnetic fields of the MOT were still present. By switching off the MOT’s light and magnetic fields, the Yb atoms are completely trapped in the optical lattice. As a result, the FWHM of the spectroscopy line was reduced by a factor of 10.
Trapped ultracold gases of metastable helium atoms provide a unique experimental system. The high internal energy enables electronic detection of single atoms. This thesis presents a number of experimental studies using metastable helium. Ionization rates in a mixture of metastable helium and rubidium were measured. Spin polarisation of the system has been shown to result in suppression of Penning ionization of rubidium by metastable helium atoms, suppressed by at least a hundred fold. This demonstration is a promising step towards the first creation of a binary BEC comprising atoms in both ground and excited states. The other experiments presented are mainly concerned with Hanbury Brown-Twiss and Higher order correlations. Single atom detection for metastable helium empowers experimenters to acquire spatial and temporal information, and to obtain full 3D reconstruction for released atomic clouds. Measurements on incoherent boson sources show bunching of particles. This enhancement to probability of joint detection events for two or more particles within short separations is in contrast to the uniform distribution of a coherent state, as measured for a Bose-Einstein condensate or an atom laser. By manipulating correlation length at the detector we were able to demonstrate the first atomic measurement of spatial three-particle correlation, and the results show significant improvement over previously reported values. Furthermore, by using a different trap geometry, it was possible perform measurement of atomic correlation functions to the 6th order, and have observed near ideal correlation functions to the 5th order, demonstrating enhancement for multi-particle detection probability consistent with the prediction of Wick's theorem. Correlations are then exploited to monitor the evolution of coherence property during the formation of a Bose-Einstein condensate. The experimental results are consistent with the existence of a quasi-condensation stage during the system's evolution from an incoherent thermal cloud towards a condensate with long range order. Two cases of mixing processes leading to the production of paired atom beams were Studied. In one case, correlation measurement provided the first higher order test of coherence of amplified matter waves. Coherence properties of matter waves generated via Bose stimulation are critical for active atom optical devices. Previously, coherence properties of amplified matter waves have only been demonstrated to first order by interference fringes. In the second case, a novel mixing process previously unknown was observed. Single atom counting is used to show number difference squeezing between opposite modes. Both processes studied hold potential of providing simple and elegant ways of producing pairs of coherent, sub-Poissonian number difference, and even entangled modes of atomic beams. Finally, physics of lower dimensions was studied. Observation was made of the phenomenon of two-step condensation in a quasi-1D system, where the gas condenses in the tightly confining transverse directions, yet remain thermal in the longitudinal direction. The lack of long-rang coherence of the system is revealed with correlations. Furthermore, an attempt was made to identify the Berezinskii-Kosterlitz-Thouless (BKT) transition.
The velocities of atoms can be manipulated by near-resonant laser light. After many absorption-spontaneous emission cycles momentum is transferred to the atoms in the direction of the laser beam. In this way atoms can be slowed down and cooled to milliKelvin temperatures and below. In three mutually orthogonal pairs of counter-propagating laser beams in combination with a magnetic field atoms can be cooled and trapped. In this so-called magneto-optical trap (MOT) two atoms can be excited to a molecular state by absorption of a photon. This technique is called photoassociation spectroscopy. In our case we study metastable helium atoms, which have a large internal energy. When two metastable helium atoms approach each other, one of the atoms ionizes and the ions are detected by a microchannelplates detector. When a probe laser beam is directed onto the MOT cloud and scanned in frequency, atom pairs can be excited to several ro-vibrational states. In the excited state the metastable helium atoms are accelerated towards each other and ionize at short internuclear distance. The ro-vibrational states appear as peaks in the ionization signal and from the position of these states information on the excited state interaction potential can be extracted.