Laser cooling and trapping of argon metastable atomic beam

Juan Carlos Catala

Published Nov 21, 1998• 0 citations

Abstract

The high velocity of free atoms associated with the thermal motion, together with the velocity distribution of atoms has imposed the ultimate limitation on the precision of ultrahigh resolution spectroscopy. A sample consisting of low velocity atoms would provide a substantial improvement in spectroscopy resolution. To overcome the problem of thermal motion, atomic physicists have pursued two goals; first, the reduction of the thermal motion (cooling); and second, the confinement of the atoms by means of electromagnetic fields (trapping). Cooling carried sufficiently far, eliminates the motional problems, whereas trapping allows for long observation times. In this work the laser cooling and trapping of an argon atomic beam will be discussed. The experiments involve a time-of-flight spectroscopy on metastable argon atoms. Laser deceleration or cooling of atoms is achieved by counter propagating a photon against an atomic beam of metastable atoms. The solution to the Doppler shift problem is achieved using spatially varying magnetic field along the beam path to Zeeman shift the atomic resonance frequency so as to keep the atoms in resonance with a fixed frequency cooling laser. For trapping experiments a Magnetooptical trap (MOT) will be used. The MOT is formed by three pairs of counter-propagating laser beams with mutual opposite circular polarization and a frequency tuned slightly below the center of the atomic resonance and superimposed on a magnetic quadrupole field.

DOI: 10.25148/etd.fi14060115

Related papers

Laser cooling of a metastable argon atomic beam

C. Ávila

A production of low velocity and monoenergetic atomic beams would increase the resolution in spectroscopic studies and many other experiments in atomic physics. Laser Cooling uses the radiation pressure to decelerate and cool atoms. The effusing from a glow discharge metastable argon atomic beam is affected by a counterpropagating laser light tuned to the cycling transition in argon. The Zeeman shift caused by a spatially varying magnetic field compensates for the changing Doppler shift that takes the atoms out of resonance as they decelerated. Deceleration and velocity bunching of atoms to a final velocity that depends on the detuning of the laser relative to a frequency of the transition have been observed. Time-of-Flight (TOF) spectroscopy is used to examine the velocity distribution of the cooled atomic beam. These TOF studies of the laser cooled atomic beam demonstrate the utility of laser deceleration for atomic-beam "velocity selection".

Jul 26, 19960 citations

Trapping and cooling of atoms

C. J. Pethick, H. Smith

The advent of the laser opened the way to the development of powerful new methods for manipulating and cooling atoms which were exploited in the realization of Bose–Einstein condensation in alkali atom vapours. To set the stage we describe a typical experiment, which is shown schematically in Fig. 4.1. A beam of sodium atoms emerges from an oven at a temperature of about 600 K, corresponding to a speed of about 800 m s –1 , and is then passed through a so-called Zeeman slower, in which the velocity of the atoms is reduced to about 30 m s –1 , corresponding to a temperature of about 1 K. In the Zeeman slower, a laser beam propagates in the direction opposite that of the atomic beam, and the radiation force produced by absorption of photons retards the atoms. Due to the Doppler effect, the frequency of the atomic transition in the laboratory frame is not generally constant, since the atomic velocity varies. However, by applying an inhomogeneous magnetic field designed so that the Doppler and Zeeman effects cancel, the frequency of the transition in the rest frame of the atom may be held fixed. On emerging from the Zeeman slower the atoms are slow enough to be captured by a magneto-optical trap (MOT), where they are further cooled by interactions with laser light to temperatures of order 100 μK. Another way of compensating for the changing Doppler shift is to increase the laser frequency in time, which is referred to as ‘chirping’. In other experiments the MOT is filled by transferring atoms from a second MOT where atoms are captured directly from the vapour.

Cambridge University Press eBooksNov 29, 20010 citations

Trapping and cooling of atoms

C. J. Pethick, H. Smith

The advent of the laser opened the way to the development of powerful methods for producing and manipulating cold atomic gases. To set the stage we describe a typical experiment, which is shown schematically in Fig. 4.1. A beam of sodium atoms emerges from an oven at a temperature of about 600 K, corresponding to a speed of about 800 m s −1 , and is then passed through a so-called Zeeman slower, in which the velocity of the atoms is reduced to about 30 m s −1 , corresponding to a temperature of about 1 K. In the Zeeman slower, a laser beam propagates in the direction opposite that of the atomic beam, and the radiation force produced by absorption of photons retards the atoms. Due to the Doppler effect, the frequency of the atomic transition in the laboratory frame is not generally constant, since the atomic velocity varies. However, by applying an inhomogeneous magnetic field designed so that the Doppler and Zeeman effects cancel, the frequency of the transition in the rest frame of the atom may be held fixed. On emerging from the Zeeman slower the atoms are slow enough to be captured by a magneto-optical trap (MOT), where they are further cooled by interactions with laser light to temperatures of order 100 μK. Another way of compensating for the changing Doppler shift is to increase the laser frequency in time, which is referred to as ‘chirping’.

Cambridge University Press eBooksSep 11, 20080 citations

Dynamical Spectroscopy of Transient He2 Molecules

Milou van Rijnbach

The velocities of atoms can be manipulated by near-resonant laser light. After many absorption-spontaneous emission cycles momentum is transferred to the atoms in the direction of the laser beam. In this way atoms can be slowed down and cooled to milliKelvin temperatures and below. In three mutually orthogonal pairs of counter-propagating laser beams in combination with a magnetic field atoms can be cooled and trapped. In this so-called magneto-optical trap (MOT) two atoms can be excited to a molecular state by absorption of a photon. This technique is called photoassociation spectroscopy. In our case we study metastable helium atoms, which have a large internal energy. When two metastable helium atoms approach each other, one of the atoms ionizes and the ions are detected by a microchannelplates detector. When a probe laser beam is directed onto the MOT cloud and scanned in frequency, atom pairs can be excited to several ro-vibrational states. In the excited state the metastable helium atoms are accelerated towards each other and ionize at short internuclear distance. The ro-vibrational states appear as peaks in the ionization signal and from the position of these states information on the excited state interaction potential can be extracted.

Jan 19, 20048 citations

Laser Cooling and Trapping of Metastable Neon and Applications to Photoionization

J. P. Ashmore

This thesis presents an in-depth study into the characterization and enhancement of a metastable neon laser cooled and trapped atomic beam. The apparatus consists of a standard Zeeman slowed atomic beam loaded into a magneto-optical trap and was designed for applications to electron scattering experiments and photoionization. The efficiency of the metastable neon atomic source was investigated to determine the ideal cathode type for maximum metastable production and optimal atomic beam velocity haracteristics. A series of characterization measurements were performed on the MOT, and the trap volume and population were investigated for a range of trapping and slowing laser intensities and detunings, together with the MOT and Zeeman slower magnetic fields. The volume measurements were compared to standard Doppler theory and it was found that the Doppler model inadequately explained the trap behaviour. It was found that the MOT population characteristics were governed by two processes: two-body losses that limit the trap population at high densities, and the efficiency of the atom capture process which limits the operational range of the MOT over the various parameters. The trap temperature was determined to be 1.3mK via a time-of-flight technique. This was nearly twice that predicted by Doppler theory and the lack of agreement once again suggests the inadequacies in the Doppler theory to correctly model the experiment. The application of the MOT to the photoionization cross-section measurement of the (2p53p)3D3 state of neon was investigated. The MOT decay technique was utilized to measure cross-section values of o351 = 2.9+0.2 -0.3 x 10 -18cm2 and o363 = 3.1 +0.3 -0.4 x 10-18cm2 at the wavelengths of 351nm and 363nm respectively. This is an increase in accuracy of around a factor of five from previous measurements and it was found that the results agreed well with the values predicted by current theories.

Jan 1, 20052 citations

Laser cooling, stopping, and magnetic trapping of neutral atoms

William D. Phillips

A thermal atomic Na beam is opposed by a resonantly tuned laser beam. The radiation pressure decelerates and compresses the thermal velocity distribution, bringing the average velocity to zero and reducing the width from ~1000 m/s to a few tens of m/s or less.1 The density of stopped atoms is > 106/cm3 within a bandwidth of a few m/ s. These densities and velocities are suitable for trapping by a number of proposed optical and magnetic traps. Using these stopped atoms, we have demonstrated the first electromagnetic trapping of neutral atoms. The trap, a magnetic quadrupole formed by two separated, coaxial, opposed current loops, confines the atoms by virtue of the force exerted on the Na magnetic dipole moment by the inhomogeneous magnetic field. The time constant for exponential decay of the atomic population in the trap is 0.83(7) s and is limited mainly by collisions with fast background gas atoms. The maximum velocity of atoms contained in the trap is 3.5 m/s, corresponding to a maximum energy of 17 mK.

Annual Meeting Optical Society of AmericaJan 1, 19850 citations