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Quantum Electronics and Laser Science Conference

High-resolution coherent spectroscopy: linewidth reduction by recurrent excitation

K. Nakayama, Shingo Furue, Masatoshi Misono, T. Mitsui, T. Kohmoto, Yukio Fukuda, Masakazu Kunitomo

Published Jun 25, 2003• 0 citations
Publisher

Abstract

Summary form only given. Spectral narrowing by recurrent use of free-decay signal in magnetic resonance has been proposed and demonstrated in the ground state of Rb atoms. In the present report we apply this technique to the measurement of the hyperfine frequency in the excited state. This is a sublevel spectroscopy with recurrent excitation where the atomic response is iteratively used as the next excitation. The hyperfine spectra of the excited state /sup 2/P/sub 3/2/ of the D/sub 2/ transition in /sup 85/Rb atoms, the line widths of which are much narrower than the natural width, were observed and the hyperfine constants of the excited state were determined precisely.

DOI
10.1109/qels.2002.1031317

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Summary form only given. Spectral narrowing by recurrent use of free-decay signal in magnetic resonance has been proposed and demonstrated in the ground state of Rb atoms. In the present report we apply this technique to the measurement of the hyperfine frequency in the excited state. This is a sublevel spectroscopy with recurrent excitation where the atomic response is iteratively used as the next excitation. The hyperfine spectra of the excited state /sup 2/P/sub 3/2/ of the D/sub 2/ transition in /sup 85/Rb atoms, the line widths of which are much narrower than the natural width, were observed and the hyperfine constants of the excited state were determined precisely.
Summary form only given. To understand the fundamental properties of an atom, precise measurement of the atomic resonance frequency is important. The main factor that restricts the precision is the spectral broadening. Spectral narrowing by recurrent use of free decay signal in magnetic resonance was proposed and demonstrated in the ground state of Rb atoms. In the present report we apply this technique to the measurement of the hyperfine frequency in the excited state. This is a sublevel spectroscopy with recurrent excitation, where the atomic response is iteratively used as the next excitation. The hyperfine spectra of the excited state /sup 2/P/sub 3/2/ of the D/sub 2/ transition in Rb atoms, whose line width is much narrower than the natural line width, was observed and the hyperfine constants of the excited state were determined precisely.
We describe the theoretical analysis and experimental detail of recurrent excitation spectroscopy (RES), which contributes to precise determination of atomic resonance frequency. The basic idea of RES lies in the iterative excitation of the atomic system by radiation. During the preceding excitation, the output field emitted from the atom is recorded in the form of digital data, and the next excitation field is generated in accordance with these data. This recurrent interaction between the atomic system and the radiation field significantly reduces the spectral width of the atomic resonance, while the signal-to-noise ratio remains sufficiently high. To reflect the actual experimental situation, we present a theoretical model in the presence of background white noise, and using this model, analytical and numerical calculations are performed. We find that RES gives a better signal-to-noise ratio compared to the conventional averaging technique until spectral narrowing is terminated. The combination of RES and the digital-data processing technique has been successfully applied to the magnetic resonance of Rb atoms in the sub-MHz region, where our theoretical findings are experimentally confirmed.
Subnatural-width resonances due to coherent effects in optical pumping at hyperfine (hf) transitions of Rb are investigated using a linearly or circularly polarized single-frequency diode laser beam. The sign and amplitude of the resonances in the fluorescence are measured by scanning the laser frequency over the hf transitions of the Rb D 1 and D 2 lines. The fluorescence perpendicular to the laser beam is detected as a function of magnetic field parallel to the beam propagation and scanned around zero value. In the case of linear polarization of the field, dark resonances are observed for hf transitions with F g → F e = F g -1 and F g → F e = F g , and bright resonances are observed for transitions with F g → F e = F g + 1. This is in agreement with the recently developed theories. For all (except F g = 2→ F e = 3, 85 Rb, D 1 line) hf transitions the sign of the resonances reverses when the polarization of the field changes to circular. The amplitudes of the resonances correspond to the probability of the hf transitions and to the calculated loss rate of the population to the ground hf level not excited by the laser field. The observed narrow resonances (FWHM: few tens of kHz) and their sensitivity to weak magnetic fields are interesting for high-resolution spectroscopy and for development of simple and precise magnetometers.
We propose a new type of spectroscopic method to reduce spectral width by recurrently using free decay (FD) in magnetic resonance of transverse optical pumping. Simultaneously with the excitation of the atomic system by a pump beam, the induced FD signal was recorded by a digital waveform memory. Then, in order to induce the next FD, we excited the atomic system by a pump beam, the intensity of which was modulated by the recorded FD, and recorded the FD induced by this pump beam. Recurrent use of this procedure reduced the spectral width of the atomic resonance and increased the signal-to-noise ratio. The narrowing procedure was demonstrated by using a randomly modulated stationary pump beam. Theoretical and experimental studies are presented. Our method serves to increase the precision of the measurement of the centre frequency of the atomic resonance.