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Journal of Physics B Atomic Molecular and Optical Physics

Spectral narrowing of magnetic resonance in transverse optical pumping by recurrently using free decay

Takahisa Mitsui, Kiyomitsu Yamashita, Katsumi Sakurai

Published May 28, 1997• 4 citations
Publisher

Abstract

We propose a new type of spectroscopic method to reduce spectral width by recurrently using free decay (FD) in magnetic resonance of transverse optical pumping. Simultaneously with the excitation of the atomic system by a pump beam, the induced FD signal was recorded by a digital waveform memory. Then, in order to induce the next FD, we excited the atomic system by a pump beam, the intensity of which was modulated by the recorded FD, and recorded the FD induced by this pump beam. Recurrent use of this procedure reduced the spectral width of the atomic resonance and increased the signal-to-noise ratio. The narrowing procedure was demonstrated by using a randomly modulated stationary pump beam. Theoretical and experimental studies are presented. Our method serves to increase the precision of the measurement of the centre frequency of the atomic resonance.

DOI
10.1088/0953-4075/30/10/013

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We propose a new type of spectroscopic method to reduce spectral width by recurrently using free decay (FD) in magnetic resonance of transverse optical pumping. Simultaneously with the excitation of the atomic system by a pump beam, the induced FD signal was recorded by a digital waveform memory. Then, in order to induce the next FD, we excited the atomic system by a pump beam, the intensity of which was modulated by the recorded FD, and recorded the FD induced by this pump beam. Recurrent use of this procedure reduced the spectral width of the atomic resonance and increased the signal-to-noise ratio. The narrowing procedure was demonstrated by using a randomly modulated stationary pump beam. Theoretical and experimental studies are presented. Our method serves to increase the precision of the measurement of the centre frequency of the atomic resonance.
Summary form only given. To understand the fundamental properties of an atom, precise measurement of the atomic resonance frequency is important. The main factor that restricts the precision is the spectral broadening. Spectral narrowing by recurrent use of free decay signal in magnetic resonance was proposed and demonstrated in the ground state of Rb atoms. In the present report we apply this technique to the measurement of the hyperfine frequency in the excited state. This is a sublevel spectroscopy with recurrent excitation, where the atomic response is iteratively used as the next excitation. The hyperfine spectra of the excited state /sup 2/P/sub 3/2/ of the D/sub 2/ transition in Rb atoms, whose line width is much narrower than the natural line width, was observed and the hyperfine constants of the excited state were determined precisely.
We describe the theoretical analysis and experimental detail of recurrent excitation spectroscopy (RES), which contributes to precise determination of atomic resonance frequency. The basic idea of RES lies in the iterative excitation of the atomic system by radiation. During the preceding excitation, the output field emitted from the atom is recorded in the form of digital data, and the next excitation field is generated in accordance with these data. This recurrent interaction between the atomic system and the radiation field significantly reduces the spectral width of the atomic resonance, while the signal-to-noise ratio remains sufficiently high. To reflect the actual experimental situation, we present a theoretical model in the presence of background white noise, and using this model, analytical and numerical calculations are performed. We find that RES gives a better signal-to-noise ratio compared to the conventional averaging technique until spectral narrowing is terminated. The combination of RES and the digital-data processing technique has been successfully applied to the magnetic resonance of Rb atoms in the sub-MHz region, where our theoretical findings are experimentally confirmed.
Summary form only given. Spectral narrowing by recurrent use of free-decay signal in magnetic resonance has been proposed and demonstrated in the ground state of Rb atoms. In the present report we apply this technique to the measurement of the hyperfine frequency in the excited state. This is a sublevel spectroscopy with recurrent excitation where the atomic response is iteratively used as the next excitation. The hyperfine spectra of the excited state /sup 2/P/sub 3/2/ of the D/sub 2/ transition in /sup 85/Rb atoms, the line widths of which are much narrower than the natural width, were observed and the hyperfine constants of the excited state were determined precisely.
New sub-Doppler resonances at central frequencies of atomic (molecular) transitions that appear in the spectrum of absorption of the probe optical radiation under the influence of optical pumping propagating in the orthogonal direction through a relatively narrow area of a cylindrical cell containing dilute gas medium are discovered and analyzed. These resonances are induced by specific optical pumping of atoms as they fly freely from the inner cell surface through the pumped region toward the probe optical beam. The obtained mathematical relations are used to investigate the dependence of the discussed resonances on the intensity and spatial distribution of the localized optical pumping. The proposed method could allow reducing the Doppler broadening of the detected spectral lines by the factor equal to the ratio of the effective width of the narrow pumped region to the cell radius. The obtained results may find application in high-resolution spectroscopy of atoms (molecules), as well as for laser-frequency stabilization by using the discovered sub- Doppler resonances.
A theoretical and experimental study has been made of the effect of transverse optical pumping in the optical-rf double resonance of cesium atoms. The solution of Bloch type equations shows that the Hanle effect and new type resonances become notable in the weak magnetic field or for strong rf field, as the effect of the transverse pumping. The new type resonances appear in the unmodulated component and the components modulated at the first and the second harmonics of the applied rf frequency in the pumping light beam transmitted through the sample cell. It is predicted that the new type resonances are not only shifted but also broadened as the intensity of rf field increases. The shift, broadening and the intensity for observed new type resonances are in good agreement with the theoretical prediction.
The spin transverse relaxation time ( T 2 ) of atoms is an important indicator for magnetic field precision measurement. Especially in optically-pumped atomic magnetometer, the linewidth of the magnetic resonance signal is one of the most important parameters of sensitivity, which is inversely correlated with T 2 of atoms. In this paper, we propose four methods, namely spin noise spectroscopy signal fitting, radio-frequency free induction decay (RF-FID) signal fitting, ω m (modulation frequency)-broadening fitting, and magnetic resonance broadening fitting, for in-situ measurement T 2 of atomic vapor cells based on light-atom interactions. Meanwhile, T 2 of three Rubidium (Rb) atomic vapor cells with different parameters are measured and discussed by using these four methods. A comparative analysis visualizes the characteristics of the different methods and the effects of buffer gas on T 2 of Rb atoms. Through theoretical and experimental analysis, we assess the applicability of each method and concluded that the RF-FID signal fitting method provides the most accurate measurements due to the timing sequence control system, which results in a cleaner measurement environment. Furthermore, we demonstrate and qualitatively analyze the relationship between temperature and T 2 of Rb atoms. This work may offer valuable insights into the selection of atomic vapor cells and it is also applicable for the spin-exchange relaxation-free region.