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arXiv:2608.09461

Probing Non-equilibrium baths: Frequency-Resolved Thermometry and Quantum Heat Current Turnover

Akhil Bhartiya, Tobias Kramer, David Gelbwaser-Klimovsky

quant-phSubmitted Aug 10, 2026• Announced Aug 11, 2026• 0 citations
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Abstract

Quantum heat transport for non-equilibrium steady state (NESS) exhibits a characteristic turnover effect, where the heat current reaches a maximum and subsequently declines as system-bath coupling increases. Although numerically exact methods can simulate this non-monotonic behavior, they offer limited information on the thermal state of the heat baths. Here, we introduce a frequency-selective thermometric protocol to probe the baths sustaining an NESS. By extracting a frequency-resolved effective temperature spectrum using a tunable two-level probe, we demonstrate that spectral dispersion serves as a direct witness for the non-equilibrium state of the heat baths. To demonstrate the protocol, we applied the hierarchical equations of motion to spin-boson and two-qubit models, though any exact method can be used. For both models, the turnover effect can be explained by how the thermal state of the heat baths evolves as the system-bath coupling strength increases.

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Quantum heat transport for non-equilibrium steady state (NESS) exhibits a characteristic turnover effect, where the heat current reaches a maximum and subsequently declines as system-bath coupling increases. Although numerically exact methods can simulate this non-monotonic behavior, they offer limited information on the thermal state of the heat baths. Here, we introduce a frequency-selective thermometric protocol to probe the baths sustaining an NESS. By extracting a frequency-resolved effective temperature spectrum using a tunable two-level probe, we demonstrate that spectral dispersion serves as a direct witness for the non-equilibrium state of the heat baths. To demonstrate the protocol, we applied the hierarchical equations of motion to spin-boson and two-qubit models, though any exact method can be used. For both models, the turnover effect can be explained by how the thermal state of the heat baths evolves as the system-bath coupling strength increases.
We consider a system consisting of two interacting qubits that are individually coupled to separate heat baths at different temperatures. The quantum effects in heat transport are investigated in a numerically rigorous manner with a hierarchial equations of motion (HEOM) approach for non-perturbative and non-Markovian system-bath coupling cases under non-equilibrium steady-state conditions. For a weak interqubit interaction, the total system is regarded as two individually thermostatted systems, whereas for a strong interqubit interaction, the two-qubit system is regarded as a single system coupled to two baths. The roles of quantum coherence (or entanglement) between the two qubits (q-q coherence) and between the qubit and bath (q-b coherence) are studied through the heat current calculated for various strengths of the system-bath coupling and interqubit coupling for high and low temperatures. The same current is also studied using the time convolutionless (TCL) Redfield equation and using an expression derived from the Fermi golden rule (FGR). We find that the HEOM results exhibit turnover behavior of the heat current as a function of the system-bath coupling strength for all values of the interqubit coupling strength, while the results obtained with the TCL and FGR approaches do not exhibit such behavior, because they do not possess the capability of treating the q-b and q-q coherences. The maximum current is obtained in the case that the q-q coherence and q-b coherence are balanced in such a manner that coherence of the entire heat transport process is realized. We also find that the heat current does not follow Fourier's law when the temperature difference is very large, due to the non-perturbative system-bath interactions.
Under non-equilibrium conditions, energy/particle currents flow through a quantum system coupled to multiple baths. Although the fluxes increase in the weak coupling regime as the coupling strengthens, the reason why they decrease to zero for large coupling remains unknown. This counterintuitive behavior of energy exchange or transport phenomena is called the turnover effect. It has been predicted in several quantum systems such as photosynthetic complexes, mesoscopic junctions, quantum heat machines, and chemical networks without a single counterexample, and it results in constrained performance due to limited currents. Here, we use scattering theory to study the turnover effect produced by low-zdensity reservoirs of free particles scattered by a quantum system through localized potentials. We find that the turnover effect is a consequence of total reflection that impedes the reservoir particle from reaching the interaction region and exchanging energy with the quantum system. Moreover, we design a protocol based on quantum tunneling to avoid the turnover and to increase the maximum current. This strategy could be used to unleash the full potential of devices based on temperature/chemical potential gradients.
We study low-temperature non-equilibrium quantum thermometry with a bosonic probe: a quantum harmonic oscillator strongly coupled to a bosonic bath at temperature TTT through a Drude--Ohmic spectral density. We treat the probe--bath dynamics both exactly, using the quadratic solution of Boyanovsky and Jasnow, and within a renormalized Gorini--Kossakowski--Lindblad--Sudarshan (GKLS) master equation. From the time-dependent covariance matrix we extract the quantum Fisher information (QFI) for general single-mode Gaussian probe states, including squeezed ones. In the strong-coupling, non-Markovian regime the QFI is non-monotonic in time, displaying bath-memory revivals that make a finite interrogation time t∗>0t^*>0t∗>0 strictly optimal. By contrast, we prove that the Markovian QFI rises monotonically to its stationary value and develops no interior optimum, so that its optimum is always pinned to the boundary t∗→∞t^*\to\inftyt∗→∞; this complements existing Markovian precision-rate bounds, which concern (F(t)/t)(\mathcal F(t)/t)(F(t)/t) rather than the single-shot QFI (F(t))(\mathcal F(t))(F(t)). Squeezed initial states yield a large transient advantage that thermalisation eventually erases, establishing squeezing and interrogation time as complementary thermometric resources. At equilibrium, strong coupling replaces the exponential Boltzmann suppression of the low-temperature relative error by a far milder polynomial divergence. As the model maps directly onto circuit quantum electrodynamics, these protocols appear within current experimental reach.
We investigate the dynamics of a two-qubit open quantum system, in particular the two-qubit spin-boson model in the strong coupling regime, coupled to two thermal bosonic baths under non-Markovian and non-equilibrium conditions. Two complementary approaches, the Hierarchical Equations of Motion (HEOM) and Reaction Coordinate Mapping (RCM), are employed to examine various coupling regimes between the qubits and their respective baths. The dynamical features of the model and the impact of the tunneling amplitude on quantum coherence of the system are probed using the l1l_1l1​-norm of coherence. The model is further shown to have non-Markovian evolution. The nontrivial task of calculating entropy production in the strong-coupling regime is performed using auxiliary density operators in HEOM. Motivated by the realization of a quantum thermal device in the strong-coupling regime, the non-equilibrium steady-state behavior of the system is investigated. Furthermore, the relationship between the heat and spin currents and the tunneling amplitude is probed.
Accurate temperature estimation in the quantum and cryogenic regimes remains a fundamental challenge. Here, we investigate nonequilibrium quantum thermometry using a single-qubit probe coupled to a bosonic bath through noncommuting interaction operators, which unify pure dephasing and dissipative dynamics within a spin-boson model. We show that the interference between these two coupling channels induces strong non-Markovian feedback between populations and coherences, leading to coherence trapping and enhanced thermal sensitivity. Remarkably, by tuning the coupling structure, the probe's temperature sensitivity exhibits a quadratic low-temperature scaling, even under weak coupling. Moreover, while coherence-based measurements are formally suboptimal, they become the most informative in the early nonequilibrium regime, where memory effects dominate. Our findings identify noncommutative system-bath couplings as a practical and tunable resource for achieving high-precision quantum thermometry in realistic open-system architectures.
When a quantum system is subject to a thermal gradient it may sustain a steady non-equilibrium heat current, by entering into a so-called non equilibrium steady state (NESS). Here we show that NESS constitute a thermodynamic resource that can be exploited to fuel a quantum heat engine. This adds to the list of recently reported sources available at the nano-scale, such as coherence, entanglement and quantum measurements. We elucidate this concept by showing analytic and numerical studies of a two-qubits quantum battery that is alternatively charged by a thermal gradient and discharged by application of a properly chosen unitary gate. The presence of a NESS for the charging step guarantees steady operation with positive power output. Decreasing the duration of the charging step results in a time periodic steady state accompanied by increased efficiency and output power. The device is amenable to implementation with different nanotechnology platforms.