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The Journal of Chemical Physics

Quantum heat transport of a two-qubit system: Interplay between system-bath coherence and qubit-qubit coherence

Akihito Kato, Yoshitaka Tanimura

Published Aug 14, 2015• 68 citations
Publisher

Abstract

We consider a system consisting of two interacting qubits that are individually coupled to separate heat baths at different temperatures. The quantum effects in heat transport are investigated in a numerically rigorous manner with a hierarchial equations of motion (HEOM) approach for non-perturbative and non-Markovian system-bath coupling cases under non-equilibrium steady-state conditions. For a weak interqubit interaction, the total system is regarded as two individually thermostatted systems, whereas for a strong interqubit interaction, the two-qubit system is regarded as a single system coupled to two baths. The roles of quantum coherence (or entanglement) between the two qubits (q-q coherence) and between the qubit and bath (q-b coherence) are studied through the heat current calculated for various strengths of the system-bath coupling and interqubit coupling for high and low temperatures. The same current is also studied using the time convolutionless (TCL) Redfield equation and using an expression derived from the Fermi golden rule (FGR). We find that the HEOM results exhibit turnover behavior of the heat current as a function of the system-bath coupling strength for all values of the interqubit coupling strength, while the results obtained with the TCL and FGR approaches do not exhibit such behavior, because they do not possess the capability of treating the q-b and q-q coherences. The maximum current is obtained in the case that the q-q coherence and q-b coherence are balanced in such a manner that coherence of the entire heat transport process is realized. We also find that the heat current does not follow Fourier's law when the temperature difference is very large, due to the non-perturbative system-bath interactions.

DOI
10.1063/1.4928192

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We consider a system consisting of two interacting qubits that are individually coupled to separate heat baths at different temperatures. The quantum effects in heat transport are investigated in a numerically rigorous manner with a hierarchial equations of motion (HEOM) approach for non-perturbative and non-Markovian system-bath coupling cases under non-equilibrium steady-state conditions. For a weak interqubit interaction, the total system is regarded as two individually thermostatted systems, whereas for a strong interqubit interaction, the two-qubit system is regarded as a single system coupled to two baths. The roles of quantum coherence (or entanglement) between the two qubits (q-q coherence) and between the qubit and bath (q-b coherence) are studied through the heat current calculated for various strengths of the system-bath coupling and interqubit coupling for high and low temperatures. The same current is also studied using the time convolutionless (TCL) Redfield equation and using an expression derived from the Fermi golden rule (FGR). We find that the HEOM results exhibit turnover behavior of the heat current as a function of the system-bath coupling strength for all values of the interqubit coupling strength, while the results obtained with the TCL and FGR approaches do not exhibit such behavior, because they do not possess the capability of treating the q-b and q-q coherences. The maximum current is obtained in the case that the q-q coherence and q-b coherence are balanced in such a manner that coherence of the entire heat transport process is realized. We also find that the heat current does not follow Fourier's law when the temperature difference is very large, due to the non-perturbative system-bath interactions.
We study the steady-state entanglement and heat current of two coupled qubits, in which two qubits are connected with two independent heat baths (IHBs) or two common heat baths (CHBs). We construct the master equation in the eigenstate representation of two coupled qubits to describe the dynamics of the total system and derive the solutions in the steady-state with stronger coupling regime between two qubits than qubit–baths. We do not make the rotating wave approximation (RWA) for the qubit–qubit interaction, and so we are able to investigate the behaviors of the system in both the strong coupling regime and the weak coupling regime, respectively. In an equilibrium bath, we find that the entanglement decreases with the bath temperature and energy detuning increasing under the strong coupling regime. In the weak coupling regime, the entanglement increases with coupling strength increasing and decreases with the bath temperature and energy detuning increasing. In a nonequilibrium bath, the entanglement without RWA is useful for entanglement at lower temperatures. We also study the heat currents of the two coupled qubits and their variations with the energy detuning, coupling strength and low temperature. In the strong (weak) coupling regime, the heat current increases (decreases) with coupling strength increasing when the temperature of one bath is lower (higher) than the other, and the energy detuning leads to a positive (negative) effect when the temperature is low (high). In the weak coupling regime, the variation trend of heat current is opposite to that of coupling strength for the IHB case and the CHB case.
We investigate the dynamics of a two-qubit open quantum system, in particular the two-qubit spin-boson model in the strong coupling regime, coupled to two thermal bosonic baths under non-Markovian and non-equilibrium conditions. Two complementary approaches, the Hierarchical Equations of Motion (HEOM) and Reaction Coordinate Mapping (RCM), are employed to examine various coupling regimes between the qubits and their respective baths. The dynamical features of the model and the impact of the tunneling amplitude on quantum coherence of the system are probed using the l1l_1l1​-norm of coherence. The model is further shown to have non-Markovian evolution. The nontrivial task of calculating entropy production in the strong-coupling regime is performed using auxiliary density operators in HEOM. Motivated by the realization of a quantum thermal device in the strong-coupling regime, the non-equilibrium steady-state behavior of the system is investigated. Furthermore, the relationship between the heat and spin currents and the tunneling amplitude is probed.
Abstract Whether genuine quantum effects, particularly quantum coherences, can offer an advantage to quantum devices is a topic of much interest. Here, we study a minimal model, the three-level V system coupled to two heat baths, and investigate the role of quantum coherences in heat transport in both the transient regime and in the nonequilibrium steady-state. In our model, energy is exchanged between the baths through two parallel pathways, which can be made distinct through the nondegeneracy of excited levels (energy splitting Δ) and a control parameter α , which adjusts the strength of one of the arms. Using a nonsecular quantum master equation of Redfield form, we succeed in deriving closed-form expressions for the quantum coherences and the heat current in the steady state limit for closely degenerate excited levels. By including three ingredients in our analysis: nonequilibrium baths, nondegeneracy of levels, and asymmetry of pathways, we show that quantum coherences are generated and sustained in the V model in the steady-state limit if three conditions, conjoining thermal and coherent effects are simultaneously met: (i) the two baths are held at different temperatures. (ii) Bath-induced pathways do not interfere destructively. (iii) Thermal rates do not mingle with the control parameter α to destroy interference through an effective local equilibrium condition. Particularly, we find that coherences are maximized when the heat current is suppressed. Although we mainly focus on analytical results in the steady state limit, numerical simulations reveal that the transient behavior of coherences contrasts the steady-state limit: large long-lived transient coherences vanish at steady state, while weak short-lived transient coherences survive, suggesting that different mechanisms are at play in these two regimes. Enhancing either the lifetime of transient coherences or their magnitude at steady state thus requires the control and optimization of different physical parameters.
Understanding how coherence of quantum systems affects thermodynamic quantities, such as work and heat, is essential for harnessing quantumness effectively in thermal quantum technologies. Here, we study the unique contributions of quantum coherence among different subsystems of a multipartite system, specifically in non-equilibrium steady states, to work and heat currents. Our system comprises two coupled ensembles, each consisting of N particles, interacting with two baths of different temperatures, respectively. The particles in an ensemble interact with their bath either simultaneously or sequentially, leading to non-local dissipation and enabling the decomposition of work and heat currents into local and non-local components. We find that the non-local heat current, as well as both the local and non-local work currents, are linked to the system quantum coherence. We provide explicit expressions of coherence-related quantities that determine the work currents under various intrasystem interactions. Our scheme is versatile, capable of functioning as a refrigerator, an engine, and an accelerator, with its performance being highly sensitive to the configuration settings. These findings establish a connection between thermodynamic quantities and quantum coherence, supplying valuable insights for the design of quantum thermal machines.
Abstract Understanding how coherence of quantum systems affects thermodynamic quantities, such as work and heat, is essential for harnessing quantumness effectively in thermal quantum technologies. Here, we study the unique contributions of quantum coherence among different subsystems of a multipartite system, specifically in non-equilibrium steady states, to work and heat currents. Our system comprises two coupled ensembles, each consisting of N particles, interacting with two baths of different temperatures, respectively. The particles in an ensemble interact with their bath either simultaneously or sequentially, leading to non-local dissipation and enabling the decomposition of work and heat currents into local and non-local components. We find that the non-local heat current, as well as both the local and non-local work currents, are linked to the system quantum coherence. We provide explicit expressions of coherence-related quantities that determine the work currents under various intrasystem interactions. Our scheme is versatile, capable of functioning as a refrigerator, an engine, and an accelerator, with its performance being highly sensitive to the configuration settings. These findings establish a connection between thermodynamic quantities and quantum coherence, supplying valuable insights for the design of quantum thermal machines.
We analytically and numerically investigate the steady-state entanglement and coherence of two coupled qubits, each interacting with a local boson or fermion reservoir, based on the Bloch-Redfield master equation beyond the secular approximation. We find that there is nonvanishing steady-state coherence in the nonequilibrium scenario, which grows monotonically with the nonequilibrium condition quantified by the temperature difference or chemical potential difference of the two baths. The steady-state entanglement, in general, is a nonmonotonic function of the nonequilibrium condition as well as the bath parameters in the equilibrium setting. We also discover that weak interqubit coupling and high base temperature or chemical potential of the baths can strongly suppress the steady-state entanglement and coherence, regardless of the strength of the nonequilibrium condition. On the other hand, the energy detuning of the two qubits, when used in a compensatory way with the nonequilibrium condition, can lead to significant enhancement of the steady-state entanglement in some parameter regimes. In addition, the qubits typically have a stronger steady-state entanglement when coupled to fermion baths exchanging particles with the system than boson baths exchanging energy with the system, under similar conditions. We also identify a close connection between the energy current flowing through the system and the steady-state coherence. Preliminary investigations suggest that these results are insensitive to the form of the reservoir spectral densities in the Markovian regime. Feasible experimental realization of measuring the steady-state entanglement and coherence is discussed for the coupled qubit system in nonequilibrium environments. Our findings offer some general guidelines for optimizing the steady-state entanglement and coherence in the coupled qubit system and may find potential applications in quantum information technology.