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arXiv:2512.21213 · APS Open Science

3D cavity-based graphene superconducting quantum circuits in two-qubit architectures

Kuei-Lin Chiu, Avishma J. Lasrado, Cheng-Han Lo, Yen-Chih Chen, Shih-Po Shih, Yen-Hsiang Lin, Chung-Ting Ke

quant-phcond-mat.mes-hallSubmitted Dec 24, 2025• Announced Dec 25, 2025• 0 citations
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Abstract

We construct a series of graphene-based superconducting quantum circuits and integrate them into 3D cavities. For a single-qubit device, we demonstrate flux-tunable qubit transition, with a measured $T_1$ $\approx$ 48 ns and a lower bound estimate of $T_2^\ast$ $\approx$ 17.63 ns. By coupling the device to cavities with different resonant frequencies, we access multiple qubit-cavity coupling regimes, enabling the observation of vacuum Rabi splitting and flux-dependent spectral linewidths. In a two-qubit device consisting of a SQUID and a single junction, power-dependent measurements reveal a two-stage dispersive shift. By flux-tuning the cavity frequency at different readout powers, we attribute the first shift to the fixed-qubit and the second to the SQUID-qubit, indicating successful coupling between the two circuits and a single cavity mode. Our study demonstrates the flexible coupling achievable between 2D-material-based superconducting circuits and 3D cavities, and paves the way toward constructing multi-qubit 3D transmon devices from 2D materials.

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Abstract In this perspective article, we review the current state of research on integrating quantum materials (QMs) into superconducting quantum devices. We begin with the role of QMs as weak links in Josephson junctions, enabling gate- and flux-tunable transmons. We then explore their application in more complex superconducting circuits, such as gate-tunable fluxonium qubits, or gatemonium, which provide additional control over qubit parameters. We also discuss QM-based vertical junctions and their potential for creating merged-element transmons. Further, we highlight QMs’ role in topological superconducting circuits, where they facilitate the study of Majorana zero modes through signatures such as 4π-periodic supercurrents. Additionally, we review the integration of QMs into 3D cavity architectures and discuss how they differ from their 2D counterparts. Beyond weak links, we examine the use of 2D superconducting and insulating materials, such as NbSe2 and hBN, in parallel-plate capacitors, offering a compact alternative to conventional large-footprint transmon capacitors. Finally, we outline the current challenges and future directions for exploration.

Materials for Quantum Technology•May 13, 2025•1 citation
We construct a series of graphene-based superconducting quantum circuits and integrate them into 3D cavities. For a single-qubit device, we demonstrate flux-tunable qubit transition, with a measured T1T_1T1​ ≈\approx≈ 48 ns and a lower bound estimate of T2∗T_2^\astT2∗​ ≈\approx≈ 17.63 ns. By coupling the device to cavities with different resonant frequencies, we access multiple qubit-cavity coupling regimes, enabling the observation of vacuum Rabi splitting and flux-dependent spectral linewidths. In a two-qubit device consisting of a SQUID and a single junction, power-dependent measurements reveal a two-stage dispersive shift. By flux-tuning the cavity frequency at different readout powers, we attribute the first shift to the fixed-qubit and the second to the SQUID-qubit, indicating successful coupling between the two circuits and a single cavity mode. Our study demonstrates the flexible coupling achievable between 2D-material-based superconducting circuits and 3D cavities, and paves the way toward constructing multi-qubit 3D transmon devices from 2D materials.
Integrating two-dimensional (2D) materials into circuit quantum electrodynamics (cQED) devices is an emerging field in recent years. This integration not only facilitates the exploration of potential applications in quantum information processing but also enables the study of material's fundamental properties using microwave techniques. While most studies employ 2D coplanar architectures with scalability potential, three-dimensional (3D) cavity-based cQED devices, due to their simpler design, offer the advantage of a quicker turnaround to probe the composite Josephson junctions (JJs). Here, we construct the first flux-tunable, 3D cavity-compatible superconducting quantum circuit based on 2D materials, featuring a graphene superconducting quantum interference device (SQUID) shunted by a capacitor that is accessible by both dc and microwave probes. We have shown how flux-modulated cavity frequency can be linked to the SQUID critical current under the influence of Fraunhofer's pattern. In addition, we extracted the symmetry information of the SQUIDs based on dc analysis, and correlated this with the flux-modulated cavity frequency observed in microwave measurements. Our platform can extend to topological materials, holding the prospect of establishing valid topological JJs with a dc probe while allowing a fast microwave probe to avoid quasiparticle poisoning.
Transmon-type superconducting qubits have become a popular platform for quantum computing due to their robust qubit coherence properties. In recent years, different types of materials have been searched to replace the Al2O3 tunnel barrier in conventional Al-based Josephson junctions, in order to explore new functions of qubits utilizing the distinct nature of the chosen materials. In this report, we introduce our works involving using Weyl semimetals and graphene as a component in Josephson junctions for qubit designs and coupling to coplanar waveguide (CPW) resonators. We fabricate a MoTe2 transmon and investigate whether it exhibits topological properties by tuning the resonator frequency with magnetic flux. Next, we introduce a graphene gatemon, in which the gate-tunability of resonator frequency has been demonstrated and the two-tone spectroscopy has shown a qubit state transition.
Abstract Superconducting quantum circuits are a leading platform for quantum-information processing, but their development requires expertise spanning device design, microfabrication, cryogenic operation, microwave control, and quantum characterization. In this work, we report the realization of a flux-tunable superconducting transmon platform and present an integrated workflow encompassing design, fabrication, measurement, and numerical modeling. The device consists of an Al/AlOx/AlAl/AlO_x/AlAl/AlOx​/Al transmon coupled to a three-dimensional microwave cavity operating in the circuit quantum electrodynamics (cQED) dispersive regime. Two-tone spectroscopy reveals a fundamental transition frequency of ω01=5.0122 GHz\omega _{01}=5.0122~\textrm{GHz}ω01​=5.0122 GHz and an anharmonicity of α/2π=−202.4 MHz\alpha /2\pi =-202.4~\textrm{MHz}α/2π=−202.4 MHz , corresponding to EJ/EC≈82.9E_J/E_C \approx 82.9EJ​/EC​≈82.9 . Flux spectroscopy yields a cavity-qubit coupling strength of g/2π=260 MHzg/2\pi = 260~\textrm{MHz}g/2π=260 MHz , while the cavity linewidth gives a loaded quality factor of QL=6127Q_L=6127QL​=6127 and a Purcell limit of T1Purcell≈82 μsT_1^{\textrm{Purcell}}\approx 82~\mu \textrm{s}T1Purcell​≈82 μs . Time-domain measurements yield coherence times of T1=17.4 μsT_1 = 17.4~\mu \textrm{s}T1​=17.4 μs and T2∗=5.8 μsT_2^* = 5.8~\mu \textrm{s}T2∗​=5.8 μs . To investigate coherence and dissipation in the device, the experimental observations are analyzed within a Lindblad master-equation framework describing cavity photon loss and thermal excitation, qubit energy relaxation, and pure dephasing processes. Using a set of experimentally extracted parameters, the model reproduces the measured spectroscopic and time-domain observables, providing a quantitative description of the open-system dynamics of the transmon-cavity platform. The analysis shows that the measured coherence is primarily limited by pure dephasing and energy-relaxation processes, whereas thermal excitation plays a minor role under the experimental conditions. Inspired by the broader framework of quantum dissipation in macroscopic quantum systems pioneered by Caldeira and collaborators, this approach enables a quantitative analysis of relaxation and dephasing processes in superconducting quantum circuits. Beyond the characterization of a single device, the present work demonstrates the establishment of the expertise, infrastructure, and experimental workflow required for the design, fabrication, measurement, and modeling of superconducting quantum circuits, contributing to the development of quantum technologies in Brazil and related applications.
We have fabricated and characterized systems consisting of superconducting quantum bits (qubits) of the transmon type, coupled to a tunable transmission line resonator. The resonator consists of a superconducting quarter wavelength coplanar waveguide (CPW) resonator that is made tunable by terminating the transmission line to ground through a superconducting quantum interference device (SQUID). Here we present measurements on two devices where we observe Rabi oscillations as we drive the qubit, and vacuum Rabi splitting both as we tune the qubits into resonance with the resonator and as we tune the resonator into resonance with the qubits. We also observe coherent interaction between two resonant qubits. In addition, we demonstrate that we can calculate the response very accurately using a multilevel Hamiltonian.
A superconducting fluxonium circuit is an RF-superconducting quantum interference device-type flux qubit that uses a large inductance built from an array of Josephson junctions or a high kinetic inductance material. This inductance suppresses charge sensitivity exponentially and flux sensitivity quadratically. In contrast to the transmon qubit, the anharmonicity of fluxonium can be large and positive, allowing for better separation between the low energy qubit manifold of the circuit and higher-lying excited states. Here, we propose a tunable coupling scheme for implementing two-qubit gates on fixed-frequency fluxonium qubits, biased at half flux quantum. In this system, both qubits and couplers are coupled capacitively and implemented as fluxonium circuits with an additional harmonic mode. We investigate the performance of the scheme by simulating a universal two-qubit fSim gate. In the proposed approach, we rely on a planar on-chip architecture for the whole device. Our design is compatible with existing hardware for transmon-based devices with the additional advantage of lower qubit frequency facilitating high-precision gating.
Abstract In this perspective article, we review the current state of research on integrating quantum materials (QMs) into superconducting quantum devices. We begin with the role of QMs as weak links in Josephson junctions, enabling gate- and flux-tunable transmons. We then explore their application in more complex superconducting circuits, such as gate-tunable fluxonium qubits, or gatemonium, which provide additional control over qubit parameters. We also discuss QM-based vertical junctions and their potential for creating merged-element transmons. Further, we highlight QMs’ role in topological superconducting circuits, where they facilitate the study of Majorana zero modes through signatures such as 4π-periodic supercurrents. Additionally, we review the integration of QMs into 3D cavity architectures and discuss how they differ from their 2D counterparts. Beyond weak links, we examine the use of 2D superconducting and insulating materials, such as NbSe2 and hBN, in parallel-plate capacitors, offering a compact alternative to conventional large-footprint transmon capacitors. Finally, we outline the current challenges and future directions for exploration.