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Brazilian Journal of Physics

From Macroscopic Quantum Tunneling to Circuit QED: Coherence and Dissipation in 3D Transmon Qubits

Gustavo Moreto, Diego Molina, Saulo Gabriel Pereira Nascimento Alberton, Denys Brito, Ednilson Cunha, Arthur Rebello, Daniel Benvenutti, Agatha Dutra, Beatriz Sacramento, Italo Soares Andrade, L. M. Ruela, Francisco P. M. Rouxinol

Published Oct 23, 2026• 1 citation
Publisher

Abstract

Abstract Superconducting quantum circuits are a leading platform for quantum-information processing, but their development requires expertise spanning device design, microfabrication, cryogenic operation, microwave control, and quantum characterization. In this work, we report the realization of a flux-tunable superconducting transmon platform and present an integrated workflow encompassing design, fabrication, measurement, and numerical modeling. The device consists of an $$Al/AlO_x/Al$$ transmon coupled to a three-dimensional microwave cavity operating in the circuit quantum electrodynamics (cQED) dispersive regime. Two-tone spectroscopy reveals a fundamental transition frequency of $$\omega _{01}=5.0122~\textrm{GHz}$$ and an anharmonicity of $$\alpha /2\pi =-202.4~\textrm{MHz}$$ , corresponding to $$E_J/E_C \approx 82.9$$ . Flux spectroscopy yields a cavity-qubit coupling strength of $$g/2\pi = 260~\textrm{MHz}$$ , while the cavity linewidth gives a loaded quality factor of $$Q_L=6127$$ and a Purcell limit of $$T_1^{\textrm{Purcell}}\approx 82~\mu \textrm{s}$$ . Time-domain measurements yield coherence times of $$T_1 = 17.4~\mu \textrm{s}$$ and $$T_2^* = 5.8~\mu \textrm{s}$$ . To investigate coherence and dissipation in the device, the experimental observations are analyzed within a Lindblad master-equation framework describing cavity photon loss and thermal excitation, qubit energy relaxation, and pure dephasing processes. Using a set of experimentally extracted parameters, the model reproduces the measured spectroscopic and time-domain observables, providing a quantitative description of the open-system dynamics of the transmon-cavity platform. The analysis shows that the measured coherence is primarily limited by pure dephasing and energy-relaxation processes, whereas thermal excitation plays a minor role under the experimental conditions. Inspired by the broader framework of quantum dissipation in macroscopic quantum systems pioneered by Caldeira and collaborators, this approach enables a quantitative analysis of relaxation and dephasing processes in superconducting quantum circuits. Beyond the characterization of a single device, the present work demonstrates the establishment of the expertise, infrastructure, and experimental workflow required for the design, fabrication, measurement, and modeling of superconducting quantum circuits, contributing to the development of quantum technologies in Brazil and related applications.

DOI
10.1007/s13538-026-02171-y

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Abstract Superconducting quantum circuits are a leading platform for quantum-information processing, but their development requires expertise spanning device design, microfabrication, cryogenic operation, microwave control, and quantum characterization. In this work, we report the realization of a flux-tunable superconducting transmon platform and present an integrated workflow encompassing design, fabrication, measurement, and numerical modeling. The device consists of an Al/AlOx/AlAl/AlO_x/AlAl/AlOx​/Al transmon coupled to a three-dimensional microwave cavity operating in the circuit quantum electrodynamics (cQED) dispersive regime. Two-tone spectroscopy reveals a fundamental transition frequency of ω01=5.0122 GHz\omega _{01}=5.0122~\textrm{GHz}ω01​=5.0122 GHz and an anharmonicity of α/2π=−202.4 MHz\alpha /2\pi =-202.4~\textrm{MHz}α/2π=−202.4 MHz , corresponding to EJ/EC≈82.9E_J/E_C \approx 82.9EJ​/EC​≈82.9 . Flux spectroscopy yields a cavity-qubit coupling strength of g/2π=260 MHzg/2\pi = 260~\textrm{MHz}g/2π=260 MHz , while the cavity linewidth gives a loaded quality factor of QL=6127Q_L=6127QL​=6127 and a Purcell limit of T1Purcell≈82 μsT_1^{\textrm{Purcell}}\approx 82~\mu \textrm{s}T1Purcell​≈82 μs . Time-domain measurements yield coherence times of T1=17.4 μsT_1 = 17.4~\mu \textrm{s}T1​=17.4 μs and T2∗=5.8 μsT_2^* = 5.8~\mu \textrm{s}T2∗​=5.8 μs . To investigate coherence and dissipation in the device, the experimental observations are analyzed within a Lindblad master-equation framework describing cavity photon loss and thermal excitation, qubit energy relaxation, and pure dephasing processes. Using a set of experimentally extracted parameters, the model reproduces the measured spectroscopic and time-domain observables, providing a quantitative description of the open-system dynamics of the transmon-cavity platform. The analysis shows that the measured coherence is primarily limited by pure dephasing and energy-relaxation processes, whereas thermal excitation plays a minor role under the experimental conditions. Inspired by the broader framework of quantum dissipation in macroscopic quantum systems pioneered by Caldeira and collaborators, this approach enables a quantitative analysis of relaxation and dephasing processes in superconducting quantum circuits. Beyond the characterization of a single device, the present work demonstrates the establishment of the expertise, infrastructure, and experimental workflow required for the design, fabrication, measurement, and modeling of superconducting quantum circuits, contributing to the development of quantum technologies in Brazil and related applications.
Superconducting qubits are a promising technology for building a scalable quantum computer. An important architecture employed in the field is called Circuit Quantum Electrodynamics (circuit QED), where such qubits are combined with high quality microwave cavities to study the interaction between artificial atoms and single microwave photons. The ultra-strong coupling achieved in these systems allows for control and readout of the quantum state of qubits to perform quantum information processing. The work on circuit QED performed in this thesis consisted of realizing an experimental setup for qubit experiments in a new laboratory, investigating the coherence and decay of higher energy levels of superconducting transmon qubits and finally demonstrating a novel coaxial form of circuit QED. Designing and building a 3D circuit QED setup involved the following main accomplishments: producing high quality 3D cavities; designing and installing the cryogenic microwave setup as well as the room temperature amplification and data acquisition circuitry; successfully developing a recipe for the fabrication of Josephson junctions; controlling and measuring superconducting 3D transmon qubits at 10mK. Several qubits were fully characterised and have shown coherence times of several microseconds and relaxation times up to 25μs. Superconducting qubits in fact possess higher energy levels that can provide significant computational advantages in quantum information applications. In experiments performed at MIT, preparation and control of the five lowest states of a transmon qubit was demonstrated, followed by an investigation of the phase coherence and decay dynamics of these higher energy levels. The decay was found to proceed mainly sequentially with relaxation times in excess of 20μs for all transitions. A direct measurement of the charge dispersion of these levels was performed to explore their characteristics of dephasing. This experiment was also reproduced on a 3D transmon fabricated and measured in Oxford, where due to a higher effective qubit temperature a multi-level decay model including thermal excitations was developed to explain the observed relaxation dynamics. Finally, a coaxial transmon, which we name the coaxmon, is presented and measured with a coaxial LC readout resonator and input/output coupling ports placed inline along the third dimension. This novel coaxial circuit QED architecture holds great promise for developing a scalable planar grid of qubits to build a quantum computer.
Quantum information processing holds the promise of a paradigm shift in computational power for specific problem classes. While contemporary quantum processors operate in the Noisy Intermediate-Scale Quantum (NISQ) regime and remain highly susceptible to errors, ongoing experimental efforts on these near-term devices are crucial for advancing the underlying technology. Among the various hardware implementations, superconducting quantum circuits stand out as one of the most robust architectures for scalable quantum technologies. Nevertheless, the primary bottleneck in these systems is the fragility of quantum information: interactions with the environment inevitably perturb the quantum states, a phenomenon known as decoherence. This rapid loss of stored information imposes a fundamental limit on the time available to reliably execute computations on these devices. Within this context, this thesis focuses on the comprehensive experimental characterization of a planar chip featuring isolated, fixed-frequency superconducting transmon qubits. The measurements were conducted in a cryogenic environment, relying on a dilution refrigerator to maintain the device at millikelvin temperatures. To probe the quantum system under these conditions, custom measurement scripts were developed to operate state-of-the-art microwave control electronics (Keysight Quantum Control System), establishing full control over pulse generation, signal acquisition, and digital demodulation. The experimental workflow systematically mapped the physical properties of the device through a progressive series of characterization steps. Initial spectroscopic techniques probed the coupled resonator-qubit system, identifying its fundamental transition frequencies and relevant energy scales. Building upon these frequency-domain measurements, coherent control was achieved by calibrating resonant microwave pulses to drive single-qubit rotations, enabling the reliable preparation of the qubit in excited or coherent superposition states. Finally, specific time-domain protocols were implemented to evaluate the operational limits of the device. By executing standard pulse sequences, the characteristic decoherence metrics of the system, namely the longitudinal energy relaxation time (T1) and the inhomogeneous dephasing time (T2*), were successfully extracted, providing a quantitative assessment of the qubit's overall performance and establishing a baseline for future implementations of more advanced quantum control protocols.
We report experiments on superconducting flux qubits in a circuit quantum electrodynamics (cQED) setup. Two qubits, independently biased and controlled, are coupled to a coplanar waveguide resonator. Dispersive qubit state readout reaches a maximum contrast of 72%. We measure energy relaxation times at the symmetry point of 5 and $10\ensuremath{\mu}\mathrm{s}$, corresponding to 7 and $20\ensuremath{\mu}\mathrm{s}$ when relaxation through the resonator due to Purcell effect is subtracted out, and levels of flux noise of 2.6 and $2.7\phantom{\rule{0.222222em}{0ex}}\ensuremath{\mu}{\mathrm{\ensuremath{\Phi}}}_{0}/\sqrt{\text{Hz}}$ at 1 Hz for the two qubits. We discuss the origin of decoherence in the measured devices. The strong coupling between the qubits and the cavity leads to a large, cavity-mediated, qubit-qubit coupling. This coupling, which is characterized spectroscopically, reaches 38 MHz. These results demonstrate the potential of cQED as a platform for fundamental investigations of decoherence and quantum dynamics of flux qubits.
Superfluid helium at milli-Kelvin temperatures is a dielectric liquid with an extremely low loss tangent at microwave frequencies. As such, it is a promising candidate for incorporation into hybrid quantum systems containing superconducting qubits. We demonstrate the viability of this hybrid systems approach by controllably immersing a three-dimensional superconducting transmon qubit in superfluid 4^44He. By measuring spectroscopic and coherence properties we find that the cavity, the qubit, and their coupling are all modified by the presence of the dielectric superfluid, which we analyze within the framework of circuit quantum electrodynamics (cQED). At temperatures relevant to quantum computing experiments, the energy relaxation time of the qubit is not significantly changed by the presence of the superfluid, while the pure dephasing time modestly increases, which we attribute to improved thermalization via the superfluid.
Circuit quantum electrodynamics (cQED), exemplified by a coupled system of a superconducting qubit and a microwave cavity, is a powerful framework for the quantum control and measurement of macroscopic quantum states in solid-state circuits. Quantum circuits based on superconducting qubits have emerged as one of the leading platforms in the pursuit of fault-tolerant quantum computing. Despite significant progress in extending qubit lifetimes, refining experimental protocols, and scaling up quantum processors, errors arising from the control and measurement of superconducting qubits continue to hinder the realization of a universal quantum computer. To investigate the error mechanisms for state-of-the-art qubits, we realize long-lived superconducting transmon qubits that exhibit fluctuating lifetimes, with an average of 0.2 ms and a maximum exceeding 0.4 ms. We then investigate their dominant error mechanism. By introducing novel time-resolved error measurements that are synchronized with the operation of the pulse tube cooler in a dilution refrigerator, we find that mechanical vibrations from the pulse tube induce nonequilibrium dynamics in highly coherent qubits, leading to their correlated bit-flip errors. Our findings not only deepen our understanding of qubit error mechanisms but also provide valuable insights into potential error-mitigation strategies for achieving fault tolerance by decoupling superconducting qubits from their mechanical environments. We also present a novel scheme for operating a cQED system in a regime where the cavity is largely displaced. We find that a qubit drive at the bare cavity frequency can effectively displace the cavity field while minimizing the cavity-drive-induced dephasing and the ac Stark shift. Furthermore, we demonstrate that standard cQED protocols, such as qubit control, readout, and cavity single-photon generation, remain compatible with largely displaced cavity fields, even beyond the critical photon number. These findings open new pathways for exploring cQED dynamics in large-photon-number regimes, including the study of nonlinear phenomena in microwave cavities, the saturation of two-level system baths for extending the coherence of microwave quantum states, and the acceleration of the dispersive readout. Finally, mechanical resonators have emerged as integral components in quantum computing for storing and transducing quantum information. Low-frequency mechanical resonators, with extremely low energy dissipation rates, are particularly interesting for extending the lifetimes of stored quantum information. However, integrating low-frequency mechanical resonators with qubits is challenging because their small energy gaps make coherent energy exchange and ground-state preparation difficult. In this thesis, we report the first steps towards the characterization of a hybrid quantum device, consisting of a Transmon qubit and a circuit optomechanical system, both coupled to a 3D microwave cavity.
PhD Thesis: Superconducting circuit quantum electrodynamics (QED) has developed into a powerful platform for studying the interaction between matter and different states of light. In this context, superconducting quantum bits (qubits) act as artificial atoms interacting with quantized modes of the electromagnetic field. The field can be trapped in superconducting microwave resonators or propagating in transmission lines. In this thesis, we particularly study circuit QED systems where microwave fields are coupled with superconducting flux and transmon qubits. We optimize the coherence properties of the resonators, by analyzing loss mechanisms at excitation powers of approximately one photon on average. We find that two-level fluctuators associated with oxide layers at substrate and metal surfaces and metal-metal interfaces represent the predominant loss channel. Furthermore, we show how broadband thermal photon fields influence the relaxation and dephasing properties of a superconducting transmon qubit. To this end, we study several second-order loss channels of the transmon qubit and find that the broadband fields introduce a larger decay rate than expected from the Purcell filter defined by the resonator. Additionally, we show that qubit dephasing at the flux-insensitive point as well as low-frequency parameter fluctuations can be enhanced by thermal fields. Finally, we study how artificial atoms react to changes in inherent properties of the light fields. We perform a detailed analysis of the photon statistics of thermal fields using their relation to the qubits coherence properties. We quantitatively recover the expected n2 + nn^{2}\,{+}\,nn2+n-law for the photon number variance and confirm this result by direct correlation measurements. We then show a novel technique for the in-situ conversion of the interaction parity in light-matter interaction. To this end, we couple spatially controlled microwave fields to a flux qubit with two degrees of freedom.