Subradiance is a phenomenon where coupled emitters radiate light at a slower rate than independent ones. While its observation was first reported in disordered cold atom clouds, ordered subwavelength arrays of emitters have emerged as promising platforms to design highly cooperative optical properties based on dipolar interactions. In this work we characterize the eigenmodes of 2D and 3D regular arrays, using a method which can be used for both infinite and very large systems. In particular, we show how finite-size effects impact the lifetimes of these large arrays. Our results may have interesting applications for quantum memories and topological effects in ordered atomic arrays.
Subradiance is a phenomenon where coupled emitters radiate light at a slower rate than independent ones. While its observation was first reported in disordered cold atom clouds, ordered subwavelength arrays of emitters have emerged as promising platforms to design highly cooperative optical properties based on dipolar interactions. In this work we characterize the eigenmodes of 2D and 3D regular arrays, using a method which can be used for both infinite and very large systems. In particular, we show how finite-size effects impact the lifetimes of these large arrays. Our results may have interesting applications for quantum memories and topological effects in ordered atomic arrays.
Abstract The optically trapped ensembles of atoms provide a versatile platform for storing and coherent manipulation of quantum information. However, efficient realization of quantum information processing requires long‐lived quantum states protected from the decoherence e.g. via spontaneous emission. Here, we theoretically study collective dipolar oscillations in finite planar arrays of quantum emitters in free space and analyze mechanisms that govern the emergence of strongly subradiant collective states. We demonstrate that the external coupling between the collective states associated with the symmetry of the array and with the quasi‐flat dispersion of the corresponding infinite lattice plays a crucial role in the boost of their radiative lifetime. We show that among different regular arrangements of the atoms the square atomic arrays support eigenstates with minimal radiative losses scaled with the total number of atoms N tot .
When quantum emitters couple indistinguishably to light, they can synchronize into a collective light matter system with radiative properties profoundly different from those of independent particles. To date, the resulting collective effects have largely been confined to point like or homogeneous ensembles. Here, we open access to a qualitatively new collective regime by realizing geometrically ordered, spatially extended atom arrays with subwavelength spacing. This establishes a fundamentally new platform in which collective emission is no longer confined to a single Dicke mode but instead emerges from an ordered network of photon mediated interactions. We find that 2D atom arrays undergo strong super and subradiant emission. Despite subwavelength spacing, we achieve site resolved imaging and directly observe the buildup of spatial correlations, demonstrating the transformation of cooperative decay into a strongly correlated many-body process. We observe extensive scaling of superradiance, uncover superradiant revivals, and reveal the ferromagnetic nature of superradiance and the antiferromagnetic nature of subradiance. Our results realize a novel programmable platform for exploring and utilizing dissipative many-body quantum physics, opening new possibilities for photon capture, storage, and atom photon entanglement.
Atomic arrays can exhibit collective light emission when the transition wavelength exceeds their lattice spacing. Subradiant states take advantage of this phenomenon to drastically reduce their overall decay rate, allowing for long-lived states in dissipative open systems. We build on previous work to investigate whether or not disorder can further decrease the decay rate of a singly excited atomic array. More specifically, we consider spatial disorder of varying strengths in a one-dimensional (1D) half waveguide and in 1D, two-dimensional (2D), and three-dimensional (3D) atomic arrays in free space and analyze the effect on the most subradiant modes. While we confirm that the dilute half waveguide exhibits an analog of Anderson localization, the dense half waveguide and free-space systems can be understood through the creation of close-packed, few-body subradiant states similar to those found in the Dicke limit. In general, we find that disorder provides little advantage in generating darker subradiant states in free space on average and will often accelerate decay. However, one could potentially change interatomic spacing within the array to engineer specific subradiant states.
Collective coupling between dipoles can dramatically modify the optical response of a medium. Such effects depend strongly on the geometry of the medium and the polarization of the light. Using a classical coupled dipole model, here we investigate the simplest case of one-dimensional arrays of interacting atomic dipoles driven by a weak laser field. Changing the polarization and direction of the driving field allows us to separately address superradiant, subradiant, redshifted, and blueshifted eigenmodes, as well as observe strong Fano-like interferences between different modes. The cooperative eigenvectors can be characterized by the phase difference between nearest-neighbor dipoles, ranging from all oscillating in phase to all oscillating out of phase with their nearest neighbors. Investigating the eigenvalue behavior as a function of atom number and lattice spacing, we find that certain eigenmodes of an infinite atomic chain have the same decay rate as a single atom between two mirrors. The effects we observe provide a framework for collective control of the optical response of a medium, giving insight into the behavior of more complicated geometries, as well as providing further evidence for the dipolar analog of cavity QED.
The Hermitian part of the field-mediated dipole-dipole interaction in infinite periodic arrays of two-level atoms yields an energy band of the singly excited states. In this Letter, we show that a dispersion relation, ω_{k}-ω_{k_{ex}}∝(k-k_{ex})^{s}, near the band edge of the infinite system leads to the existence of subradiant states of finite one-dimensional arrays of N atoms with decay rates scaling as N^{-(s+1)}. This explains the recently discovered N^{-3} scaling and it leads to the prediction of power law scaling with higher power for special values of the lattice period. For the quantum optical implementation of the Su-Schrieffer-Heeger topological model in a dimerized emitter array, the band gap closing inherent to topological transitions changes the value of s in the dispersion relation and alters the decay rates of the subradiant states by many orders of magnitude.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.