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arXiv:2006.06329 · Physical Review Letters

Subradiant Emission from Regular Atomic Arrays: Universal Scaling of Decay Rates from the Generalized Bloch Theorem

Yu-Xiang Zhang, Klaus Mølmer

Published Dec 14, 2020• 51 citations
arXivHTMLPDF

Abstract

The Hermitian part of the field-mediated dipole-dipole interaction in infinite periodic arrays of two-level atoms yields an energy band of the singly excited states. In this Letter, we show that a dispersion relation, ω_{k}-ω_{k_{ex}}∝(k-k_{ex})^{s}, near the band edge of the infinite system leads to the existence of subradiant states of finite one-dimensional arrays of N atoms with decay rates scaling as N^{-(s+1)}. This explains the recently discovered N^{-3} scaling and it leads to the prediction of power law scaling with higher power for special values of the lattice period. For the quantum optical implementation of the Su-Schrieffer-Heeger topological model in a dimerized emitter array, the band gap closing inherent to topological transitions changes the value of s in the dispersion relation and alters the decay rates of the subradiant states by many orders of magnitude.

DOI
10.1103/physrevlett.125.253601

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The Hermitian part of the field-mediated dipole-dipole interaction in infinite periodic arrays of two-level atoms yields an energy band of the singly excited states. In this Letter, we show that a dispersion relation, ω_{k}-ω_{k_{ex}}∝(k-k_{ex})^{s}, near the band edge of the infinite system leads to the existence of subradiant states of finite one-dimensional arrays of N atoms with decay rates scaling as N^{-(s+1)}. This explains the recently discovered N^{-3} scaling and it leads to the prediction of power law scaling with higher power for special values of the lattice period. For the quantum optical implementation of the Su-Schrieffer-Heeger topological model in a dimerized emitter array, the band gap closing inherent to topological transitions changes the value of s in the dispersion relation and alters the decay rates of the subradiant states by many orders of magnitude.
Atomic arrays provide an important quantum optical platform with photon-mediated dipole–dipole interactions that can be engineered to realize key applications in quantum information processing. A major obstacle for such applications is the fast decay of the excited states. By controlling two-band Bloch oscillations of single excitation in an atomic array under an external magnetic field, here we show that exotic subradiance can be realized and maintained with orders of magnitude longer than the spontaneous decay time in atomic arrays with the finite size. The key finding is to show a way for preventing the wavepacket of excited states scattering into the dissipative zone inside the free space light cone, which therefore leads to the excitation staying at a subradiant state for an extremely long decay time. We show that such operation can be achieved by introducing a spatially linear potential from the external magnetic field in the atomic arrays and then manipulating interconnected two-band Bloch oscillations along opposite directions. Our results also point out the possibility of controllable switching between superradiant and subradiant states, which leads to potential applications in quantum storage.
Energy and lifetime of collective optical excitations in regular arrays of atoms and molecules are significantly influenced by dipole-dipole interaction. While the dynamics of closely positioned atoms can be approximated well by the Dicke superradiance model, the situation of finite regular configurations is hard to access analytically. Most treatments use an exciton based description limited to the lowest excitation manifold. We present a general approach studying the complete decay cascade of a finite regular array of atoms from the fully inverted to the ground state. We explicitly calculate all energy shifts and decay rates for two generic cases of a three-atom linear chain and an equilateral triangle. In numerical calculations we show that despite fairly weak dipole-dipole interactions, collective vacuum coupling allows for superradiant emission as well as subradiant states in larger arrays through multi-particle interference. This induces extra dephasing and modified decay as important limitations for Ramsey experiments in lattice atomic clock setups as well as for the gain and frequency stability of superradiant lasers.
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Atomic arrays provide an important quantum optical platform with photon-mediated dipoledipole interactions, which can be engineered to realize key applications in quantum information processing. A major obstacle for such application is the fast decay of the excited states. By controlling two-band Bloch oscillations in an atomic array under external magnetic field, here we show that exotic subradiance can be realized and maintained at a time scale upto 12 orders of magnitude larger than the spontaneous decay time in atomic arrays with the finite size. The key finding is to show a way for preventing the wavepacket of excited states scattering into the dissipative zone inside the free space light cone, which therefore leads to the excitation staying at a subradiant state for extremely long decay time. We show that such operation can be achieved by introducing a spatially linear potential from external magnetic field in atomic arrays and then manipulating interconnected two-band Bloch oscillations along opposite directions. Our results also point out the possibility of controllable switching between superradiant and subradiant states, which leads to potential applications in quantum storage.
Recently, the subradiant states of one-dimensional two-level atom chains coupled to light modes were found to have decay rates obeying a universal scaling, and an unexpected fermionic character of the multiply excited subradiant states was discovered. In this Letter, we theoretically obtain the singly excited subradiant states, and by eliminating the superradiant modes, we demonstrate a relation between the multiply excited subradiant states and the Tonks-Girardeau limit of the Lieb-Liniger model which explains the fermionic behavior. In addition, we identify a new family of subradiant states with correlations different from the fermionic ansatz.
We present a framework to investigate the collective properties of atomic lattices in one, two, and three dimensions. We analyze the single-photon band structure and associated atomic decay rates, revealing a fundamental dependence on dimensionality. One- and two-dimensional arrays are shown to be inherently radiative, exhibiting band gaps and decay rates that oscillate between superradiant and subradiant regimes, as a function of lattice spacing. In contrast, three-dimensional lattices are found to be fundamentally non-radiative due to the inhibition of spontaneous emission, with decay only at discrete Bragg resonances. Furthermore, we demonstrate that this structural difference dictates the system dynamics, which crosses over from dissipative decay in lower dimensions to coherent transport in three dimensions. Our results provide insight into cooperative effects in atomic arrays at the single-photon level.