Atomic arrays can exhibit collective light emission when the transition wavelength exceeds their lattice spacing. Subradiant states take advantage of this phenomenon to drastically reduce their overall decay rate, allowing for long-lived states in dissipative open systems. We build on previous work to investigate whether or not disorder can further decrease the decay rate of a singly excited atomic array. More specifically, we consider spatial disorder of varying strengths in a one-dimensional (1D) half waveguide and in 1D, two-dimensional (2D), and three-dimensional (3D) atomic arrays in free space and analyze the effect on the most subradiant modes. While we confirm that the dilute half waveguide exhibits an analog of Anderson localization, the dense half waveguide and free-space systems can be understood through the creation of close-packed, few-body subradiant states similar to those found in the Dicke limit. In general, we find that disorder provides little advantage in generating darker subradiant states in free space on average and will often accelerate decay. However, one could potentially change interatomic spacing within the array to engineer specific subradiant states.
Atomic arrays can exhibit collective light emission when the transition wavelength exceeds their lattice spacing. Subradiant states take advantage of this phenomenon to drastically reduce their overall decay rate, allowing for long-lived states in dissipative open systems. We build on previous work to investigate whether or not disorder can further decrease the decay rate of a singly excited atomic array. More specifically, we consider spatial disorder of varying strengths in a one-dimensional (1D) half waveguide and in 1D, two-dimensional (2D), and three-dimensional (3D) atomic arrays in free space and analyze the effect on the most subradiant modes. While we confirm that the dilute half waveguide exhibits an analog of Anderson localization, the dense half waveguide and free-space systems can be understood through the creation of close-packed, few-body subradiant states similar to those found in the Dicke limit. In general, we find that disorder provides little advantage in generating darker subradiant states in free space on average and will often accelerate decay. However, one could potentially change interatomic spacing within the array to engineer specific subradiant states.
Ordered ensembles of atoms, such as atomic arrays, exhibit distinctive features from their disordered counterpart. In particular, while collective modes in disordered ensembles show a linear optical response, collective subradiant excitations of subwavelength arrays are endowed with an intrinsic nonlinearity. Such nonlinearity has both a coherent and a dissipative component: two excitations propagating in the array scatter off each other leading to formation of correlations and to emission into free-space modes. We show how to take advantage of such nonlinearity to coherently prepare a single excitation in a subradiant (dark) collective state of a one-dimensional array as well as to perform an entangling operation on dark states of parallel arrays. We discuss the main source of errors represented by disorder introduced by atomic center-of-mass fluctuations, and we propose a practical way to mitigate its effects.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
We present a framework to investigate the collective properties of atomic lattices in one, two, and three dimensions. We analyze the single-photon band structure and associated atomic decay rates, revealing a fundamental dependence on dimensionality. One- and two-dimensional arrays are shown to be inherently radiative, exhibiting band gaps and decay rates that oscillate between superradiant and subradiant regimes, as a function of lattice spacing. In contrast, three-dimensional lattices are found to be fundamentally non-radiative due to the inhibition of spontaneous emission, with decay only at discrete Bragg resonances. Furthermore, we demonstrate that this structural difference dictates the system dynamics, which crosses over from dissipative decay in lower dimensions to coherent transport in three dimensions. Our results provide insight into cooperative effects in atomic arrays at the single-photon level.
Subradiance is a phenomenon where coupled emitters radiate light at a slower rate than independent ones. While its observation was first reported in disordered cold atom clouds, ordered subwavelength arrays of emitters have emerged as promising platforms to design highly cooperative optical properties based on dipolar interactions. In this work we characterize the eigenmodes of 2D and 3D regular arrays, using a method which can be used for both infinite and very large systems. In particular, we show how finite-size effects impact the lifetimes of these large arrays. Our results may have interesting applications for quantum memories and topological effects in ordered atomic arrays.
When quantum emitters couple indistinguishably to light, they can synchronize into a collective light matter system with radiative properties profoundly different from those of independent particles. To date, the resulting collective effects have largely been confined to point like or homogeneous ensembles. Here, we open access to a qualitatively new collective regime by realizing geometrically ordered, spatially extended atom arrays with subwavelength spacing. This establishes a fundamentally new platform in which collective emission is no longer confined to a single Dicke mode but instead emerges from an ordered network of photon mediated interactions. We find that 2D atom arrays undergo strong super and subradiant emission. Despite subwavelength spacing, we achieve site resolved imaging and directly observe the buildup of spatial correlations, demonstrating the transformation of cooperative decay into a strongly correlated many-body process. We observe extensive scaling of superradiance, uncover superradiant revivals, and reveal the ferromagnetic nature of superradiance and the antiferromagnetic nature of subradiance. Our results realize a novel programmable platform for exploring and utilizing dissipative many-body quantum physics, opening new possibilities for photon capture, storage, and atom photon entanglement.
We study the collective emission of a disordered array of N excited two-level atoms into a one-dimensional photonic waveguide. In the perfectly ordered case, where atoms are spaced by exact integer multiples of the wavelength, the system exhibits the characteristic superradiant burst with a peak emission rate scaling as N 2 . Using large-scale semiclassical simulations, we find that this key signature of superradiance remains asymptotically robust under strong spatial and spectral disorder, but also exhibits subtle finite-size scaling toward this limit. To explain our observations, we provide an analytical variational estimate for the maximal decay rate, which tightly bounds the numerical results and reveals how disorder shapes the collective decay. Specifically, we find that even in the presence of strong disorder, the spins tend to self-organize spontaneously according to their locations, which overall optimizes constructive interference effects and explains the emergence of mirror-asymmetric correlations in superradiant decay. These findings resolve important open questions regarding the existence and nature of superradiance in strongly disordered arrays and offer valuable insights for understanding collective quantum optical phenomena in realistic systems.