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arXiv:2310.06791 · Nanophotonics

Strongly subradiant states in planar atomic arrays

Ilya A. Volkov, Nikita Ustimenko, Danil Kornovan, A. S. Sheremet, Roman S. Savelev, Mihail I. Petrov

Published Jan 30, 2024• 6 citations
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Abstract

Abstract The optically trapped ensembles of atoms provide a versatile platform for storing and coherent manipulation of quantum information. However, efficient realization of quantum information processing requires long‐lived quantum states protected from the decoherence e.g. via spontaneous emission. Here, we theoretically study collective dipolar oscillations in finite planar arrays of quantum emitters in free space and analyze mechanisms that govern the emergence of strongly subradiant collective states. We demonstrate that the external coupling between the collective states associated with the symmetry of the array and with the quasi‐flat dispersion of the corresponding infinite lattice plays a crucial role in the boost of their radiative lifetime. We show that among different regular arrangements of the atoms the square atomic arrays support eigenstates with minimal radiative losses scaled with the total number of atoms N tot .

DOI
10.1515/nanoph-2023-0624

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Abstract The optically trapped ensembles of atoms provide a versatile platform for storing and coherent manipulation of quantum information. However, efficient realization of quantum information processing requires long‐lived quantum states protected from the decoherence e.g. via spontaneous emission. Here, we theoretically study collective dipolar oscillations in finite planar arrays of quantum emitters in free space and analyze mechanisms that govern the emergence of strongly subradiant collective states. We demonstrate that the external coupling between the collective states associated with the symmetry of the array and with the quasi‐flat dispersion of the corresponding infinite lattice plays a crucial role in the boost of their radiative lifetime. We show that among different regular arrangements of the atoms the square atomic arrays support eigenstates with minimal radiative losses scaled with the total number of atoms N tot .
We study collective "free-space" radiation properties of two distant single-layer arrays of quantum emitters as two-level atoms. We show that this system can support a long-lived Bell superposition state of atomic excitations exhibiting strong subradiance, which corresponds to a nonlocal excitation of the two arrays. We describe the preparation of these states and their application in quantum information as a resource of nonlocal entanglement, including deterministic quantum state transfer with high fidelity between the arrays representing quantum memories. We discuss experimental realizations using cold atoms in optical trap arrays with subwavelength spacing, and analyze the role of imperfections.
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
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Collective excitations in ordered subwavelength atomic arrays can exhibit strongly suppressed radiative decay due to interference between light scattered by neighboring emitters. These so-called subradiant states make these systems a promising platform for storing and manipulating photonic excitations. The external geometry of the array, combined with dynamical control of the atomic dipole orientation, enables localized trapping and coherent transport of these subradiant excitations. Here, we theoretically demonstrate these capabilities in ring-shaped atomic arrays. Specifically, we show adiabatic transport of a localized excitation around a single ring, coherent transfer of a single excitation between two neighboring rings with geometry-controlled selectivity, and interaction-induced conditional phase shifts between two simultaneously trapped excitations in neighboring rings. The latter can be interpreted as effective controlled-phase operations between stored excitations. Together, these results demonstrate the potential of ordered atomic arrays as a platform for coherent photonic quantum information processing with dissipation-protected collective excitations.
Atomic arrays provide an important quantum optical platform with photon-mediated dipole–dipole interactions that can be engineered to realize key applications in quantum information processing. A major obstacle for such applications is the fast decay of the excited states. By controlling two-band Bloch oscillations of single excitation in an atomic array under an external magnetic field, here we show that exotic subradiance can be realized and maintained with orders of magnitude longer than the spontaneous decay time in atomic arrays with the finite size. The key finding is to show a way for preventing the wavepacket of excited states scattering into the dissipative zone inside the free space light cone, which therefore leads to the excitation staying at a subradiant state for an extremely long decay time. We show that such operation can be achieved by introducing a spatially linear potential from the external magnetic field in the atomic arrays and then manipulating interconnected two-band Bloch oscillations along opposite directions. Our results also point out the possibility of controllable switching between superradiant and subradiant states, which leads to potential applications in quantum storage.