We study collective "free-space" radiation properties of two distant single-layer arrays of quantum emitters as two-level atoms. We show that this system can support a long-lived Bell superposition state of atomic excitations exhibiting strong subradiance, which corresponds to a nonlocal excitation of the two arrays. We describe the preparation of these states and their application in quantum information as a resource of nonlocal entanglement, including deterministic quantum state transfer with high fidelity between the arrays representing quantum memories. We discuss experimental realizations using cold atoms in optical trap arrays with subwavelength spacing, and analyze the role of imperfections.
We study collective "free-space" radiation properties of two distant single-layer arrays of quantum emitters as two-level atoms. We show that this system can support a long-lived Bell superposition state of atomic excitations exhibiting strong subradiance, which corresponds to a nonlocal excitation of the two arrays. We describe the preparation of these states and their application in quantum information as a resource of nonlocal entanglement, including deterministic quantum state transfer with high fidelity between the arrays representing quantum memories. We discuss experimental realizations using cold atoms in optical trap arrays with subwavelength spacing, and analyze the role of imperfections.
Recent experimental advances in preparing regular defect-free 2D arrays of atoms with optical traps have offered new opportunities to engineer strong collective couplings between light and atoms as quantum optical dipoles. Applications of such collective light-matter interactions include the realization of atom-thick mirrors, retrieval of quantum memories with high efficiency, or the implementation of topological quantum optics. I will present novel applications in the context of quantum networking. First, I will discuss the design of a chiral photonic quantum link, where distant single atoms interact by exchanging photons propagating in a unique direction in free space. This is achieved by coupling both single atoms, representing qubits implemented using a pair of Rydberg states, to bi-layer atomic arrays which act as quantum phased-array antennas. Exploiting the combination of a “Rydberg-dressing” laser and a control laser driving the atomic arrays, an effective Rydberg dipole-dipole interaction can be engineered between atoms and atomic arrays as quantum emitters, allowing to match the spatial modes of spontaneously emitted and absorbed photons to a Gaussian mode of interest. In this way, we realize a chiral quantum interface, i.e., where atoms couple to photonic modes with a unique direction of propagation. This setup provides a basic building block of a novel platform for quantum networks in free space, i.e., without requiring coupling atoms to modes of cavities or nanostructures, which I will illustrate with the deterministic coherent transfer of quantum states between single atoms with high fidelity. Second, I will discuss the collective radiation properties of two distant single-layer atomic arrays acting as quantum memories. This system can support a long-lived non-local superposition state of atomic excitations exhibiting strong subradiance. This “dark” mode consists of an atomic excitation which is delocalized between the two distant atomic arrays, in such a way that the overall radiation is strongly suppressed by quantum interference. I will describe the preparation of these states and their application as resource of non-local entanglement. In particular, by weakly driving the arrays, the state of the quantum memories, localized in each array, can be transferred to this “non-local” subradiant state, allowing again for a deterministic coherent quantum state transfer with high fidelity between the memories. Finally, I will discuss experimental realizations using cold atoms in optical trap arrays, and the effect of experimental imperfections in the arrays, such as finite defect probability, temperature, and depth of the optical traps.
Abstract The optically trapped ensembles of atoms provide a versatile platform for storing and coherent manipulation of quantum information. However, efficient realization of quantum information processing requires long‐lived quantum states protected from the decoherence e.g. via spontaneous emission. Here, we theoretically study collective dipolar oscillations in finite planar arrays of quantum emitters in free space and analyze mechanisms that govern the emergence of strongly subradiant collective states. We demonstrate that the external coupling between the collective states associated with the symmetry of the array and with the quasi‐flat dispersion of the corresponding infinite lattice plays a crucial role in the boost of their radiative lifetime. We show that among different regular arrangements of the atoms the square atomic arrays support eigenstates with minimal radiative losses scaled with the total number of atoms N tot .
The interaction between light and matter has captivated physicists for centuries, from early studies of vision and refraction in ancient Greece to the development of quantum mechanics and quantum electrodynamics in the past century. While the response of a single quantum emitter to light is well understood, the radiative properties of an ensemble of closely spaced emitters are far more intricate. Coupling to a shared electromagnetic environment induces coherent and dissipative interactions between emitters, giving rise to a collective response that cannot be captured by treating them independently. In the regime of few excitations, the system hosts delocalized subradiant states, that is, coherent superpositions that are largely decoupled from the electromagnetic field and thus decay at suppressed rates. While this weak coupling makes subradiant states attractive for quantum technologies, it also renders them difficult to manipulate. At higher excitation densities, the intrinsic nonlinearity of emitters and the exponential growth of the Hilbert space make theoretical and numerical descriptions of the system and its dynamics increasingly challenging. This thesis explores two fundamental questions: How can subradiant and dark states be selectively accessed and harnessed for practical applications in quantum technologies? And how can interacting ensembles of quantum emitters be efficiently simulated to uncover their many-body physics? The first part of the thesis develops protocols for controlling and addressing dark states in free-space and waveguide-coupled atomic arrays, demonstrating their utility in quantum storage and the deterministic generation of entangled photonic states. Incorporating atomic motion, we further show that collective subradiant states can enhance cooling in dense atomic arrays, offering new avenues for controlling motional dynamics. In the second part, we introduce cumulant expansions of the equations of motion as a powerful tool to analytically and numerically investigate collective decay in the many-body regime. We first examine the collective decay of fully excited atomic arrays in free space, characterizing the onset and scaling of the superradiant burst across different geometries. In collaboration with experiments on ultracold erbium atoms in optical lattices, we provide the first direct observations of many-body collective effects in free-space ordered arrays, including early-time superradiant bursts, late-time subradiant tails, and the emergence of atomic correlations throughout the dynamics. Finally, we theoretically and numerically explore the transient formation of multi-excitation subradiant states, and demonstrate how the existence of multiple dissipation channels suppresses steady-state superradiance in extended arrays.
The collective interaction of electronic excitations with the electromagnetic field in atomic arrays can lead to reduced decay rates, forming subradiant states with applications in quantum information and memories. By including quantized vibrational excitations, we examine the effects of finite trap strength and light-mediated forces on highly subradiant singly excited states for two, three, and many atoms in a one-dimensional waveguide or free space. For waveguide-coupled and tightly trapped atoms, the recoil energy from photon emission can reach a vibrational quantum, even in the Lamb-Dicke regime. For weakly trapped atoms, the vibrational wave packets are shifted or distorted due to induced forces and uneven decay. These effects lead to a time-dependent decay rate, extra vibrational energy transfer, and mixing of different electronic and vibrational states. The resulting entanglement entropy and infidelity can be mitigated by decreasing the induced forces or increasing trap strength. For quantum information storage, these findings suggest optimal array configurations in geometry and polarization. Our results provide insights for quantum memories and atom array experiments.
Collective excitations in ordered subwavelength atomic arrays can exhibit strongly suppressed radiative decay due to interference between light scattered by neighboring emitters. These so-called subradiant states make these systems a promising platform for storing and manipulating photonic excitations. The external geometry of the array, combined with dynamical control of the atomic dipole orientation, enables localized trapping and coherent transport of these subradiant excitations. Here, we theoretically demonstrate these capabilities in ring-shaped atomic arrays. Specifically, we show adiabatic transport of a localized excitation around a single ring, coherent transfer of a single excitation between two neighboring rings with geometry-controlled selectivity, and interaction-induced conditional phase shifts between two simultaneously trapped excitations in neighboring rings. The latter can be interpreted as effective controlled-phase operations between stored excitations. Together, these results demonstrate the potential of ordered atomic arrays as a platform for coherent photonic quantum information processing with dissipation-protected collective excitations.
Ordered ensembles of atoms, such as atomic arrays, exhibit distinctive features from their disordered counterpart. In particular, while collective modes in disordered ensembles show a linear optical response, collective subradiant excitations of subwavelength arrays are endowed with an intrinsic nonlinearity. Such nonlinearity has both a coherent and a dissipative component: two excitations propagating in the array scatter off each other leading to formation of correlations and to emission into free-space modes. We show how to take advantage of such nonlinearity to coherently prepare a single excitation in a subradiant (dark) collective state of a one-dimensional array as well as to perform an entangling operation on dark states of parallel arrays. We discuss the main source of errors represented by disorder introduced by atomic center-of-mass fluctuations, and we propose a practical way to mitigate its effects.