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arXiv:2511.05008

Disorder-broadened topological Hall phase and anomalous Hall scaling in FeGe

Chaman Gupta, Chris Matsumura, Hongbin Yang, Sarah Edwards, Rebeca M. Gurrola, Jiun-Haw Chu, Hanjong Paik, Yongqiang Wang, David A. Muller, Robert Streubel, Tzu-Ming Lu, Serena Eley

cond-mat.mtrl-scicond-mat.mes-hallquant-phSubmitted Nov 7, 2025• Announced Nov 10, 2025
arXivHTMLPDF

Abstract

Magnetic skyrmions are topologically protected spin textures that are promising candidates for low-power spintronic memory and logic devices. Realizing skyrmion-based devices requires an understanding of how structural disorder affects their stability and transport properties. This study uses Ne$^{+}$ ion irradiation at fluences from $10^{11}$ to $10^{14}$ ions-cm$^{-2}$ to systematically vary defect densities in 80 nm epitaxial FeGe films and quantify the resulting modifications to magnetic phase boundaries and electronic scattering. Temperature- and field-dependent Hall measurements reveal that increasing disorder progressively extends the topological Hall signal from a narrow window near 200K in pristine films down to 4K at the highest fluence, with peak amplitude more than doubling. Simultaneously, the anomalous Hall effect transitions from quadratic Berry curvature scaling to linear skew scattering behavior, with the skew coefficient increasing threefold. These results establish quantitative correlations between defect concentration, skyrmion phase space, and transport mechanisms in a chiral magnet. It demonstrates that ion-beam modification provides systematic control over both topological texture stability and electrical detectability.

DOI
10.1002/adfm.77825
Comments
20 pages, 5 figures

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Magnetic skyrmions are topologically protected spin textures that are promising candidates for low-power spintronic memory and logic devices. Realizing skyrmion-based devices requires an understanding of how structural disorder affects their stability and transport properties. This study uses Ne+^{+}+ ion irradiation at fluences from 101110^{11}1011 to 101410^{14}1014 ions-cm−2^{-2}−2 to systematically vary defect densities in 80 nm epitaxial FeGe films and quantify the resulting modifications to magnetic phase boundaries and electronic scattering. Temperature- and field-dependent Hall measurements reveal that increasing disorder progressively extends the topological Hall signal from a narrow window near 200K in pristine films down to 4K at the highest fluence, with peak amplitude more than doubling. Simultaneously, the anomalous Hall effect transitions from quadratic Berry curvature scaling to linear skew scattering behavior, with the skew coefficient increasing threefold. These results establish quantitative correlations between defect concentration, skyrmion phase space, and transport mechanisms in a chiral magnet. It demonstrates that ion-beam modification provides systematic control over both topological texture stability and electrical detectability.
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Topological kagome magnets offer a rich landscape for exploring the intricate interplay of quantum interactions among geometry, topology, spin, and correlation. GdTi3Bi4 crystallizes in layered Ti based kagome nets intertwined with zigzag Gd chains along the a axis and orders antiferromagnetically below 15 K. Here, we present the temperature and field dependent electrical transport of GdTi3Bi4 in different directions. The material exhibits anomalous Hall conductivity (AHC) of 410 S cm-1 at 2 K for B parallel c and it is completely absent for B parallel a, despite the similar magnetization observed in both orientations. This behavior is quite contradictory, as anomalous Hall effect (AHE) typically scales with the magnetization. Through first principles calculations, it is demonstrated that in the presence of time reversal symmetry broken by the Gd 4f sublattice and spin orbit coupling, the magnetization direction controls the orbital mixing in the Ti t2g bands, relocating Berry curvature hot spots and producing the observed orientation selective AHC. The results establish GdTi3Bi4 as platform for investigating new avenues of AHE, such as directional AHE, and thus shed new light on the intricate coupling between magnetic and electronic structures, paving the way for exploring novel quantum phenomena.
The interplay between topology and correlation can give rise to exotic collective excitations. The integer and fractional quantum anomalous Hall (QAH) magnets recently discovered in two-dimensional (2D) flatband systems are predicted to host spin excitations distinct from those in conventional magnets. Experimentally, nevertheless, these new excitations remain largely unexplored. Here we investigate spin-valley excitations in a twisted MoTe2 moiré superlattice using resonant ultrafast pump-probe spectroscopy. We observe a metastable spin-valley excitation in the QAH magnet below T ~ 3.7 K that survives reverse magnetic field several times larger than the saturation field. The behavior of this excitation is sharply distinct from ordinary domain walls and magnons, indicating a new type of spin-valley textures unique to topological magnets. We propose that these textures are chiral domain walls with an in-plane winding of the pseudospin order parameter along the domain wall. Their metastability arises from the interplay between the topological winding in real space and the quantum geometry of the parent bands in momentum space through a universal mechanism. These chiral domain walls govern the nonequilibrium dynamics of QAH magnets and may play a central role in their stability. Our study highlights intrinsic quantum geometry effects on spin excitations in topological magnets; and provides key insights into the fundamental mechanism limiting stability of topological protection.