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arXiv:2511.14241

Current Switching of Topological Spin Chirality in the van der Waals Antiferromagnet Co1/3TaS2

Kai-Xuan Zhang, Seungbok Lee, Woonghee Cho, Je-Geun Park

cond-mat.mtrl-sciphysics.app-phquant-phSubmitted Nov 18, 2025• Announced Nov 19, 2025• Revised Mar 3, 2026 (v2)
v1 · Nov 18, 2025v2 · Mar 3, 2026
arXivHTMLPDF

Abstract

Magnetic topology is central to modern quantum magnet, where spin chirality governs exotic spin winding, real-space Berry phase, and topological Hall effect. A key unresolved challenge is how to electrically switch topological spin chirality and its associated gauge flux, an essential requirement for manipulating its topological quantum properties. In this work, we propose and experimentally demonstrate the concept of current-switching spin chirality. We identify the new vdW antiferromagnet Co1/3TaS2 as an ideal platform, hosting a topological 3Q state with a minimum chirality cell, an ultrahigh skyrmion density, a non-centrosymmetric geometry, and a strong Berry curvature. We discover intrinsic self-torque-induced chirality switching within Co1/3TaS2, driven purely by current, without the need of heavy metals or a magnetic field, and with high energy efficiency. Our results establish a promising framework for electrically generating and controlling topological spin chirality, and demonstrate a practical route toward chiral spintronics. They can be naturally generalised to other skyrmion systems, offering new opportunities in symmetry control, topological manipulation, and spin-chirality-based quantum functionalities.

Journal reference
Advanced Materials 38, e22943 (2026)
DOI
10.1002/adma.202522943
Comments
Accepted by Advanced Materials; 37 pages, 4 main figures, 6 supporting figures

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Magnetic topology is central to modern quantum magnet, where spin chirality governs exotic spin winding, real-space Berry phase, and topological Hall effect. A key unresolved challenge is how to electrically switch topological spin chirality and its associated gauge flux, an essential requirement for manipulating its topological quantum properties. In this work, we propose and experimentally demonstrate the concept of current-switching spin chirality. We identify the new vdW antiferromagnet Co1/3TaS2 as an ideal platform, hosting a topological 3Q state with a minimum chirality cell, an ultrahigh skyrmion density, a non-centrosymmetric geometry, and a strong Berry curvature. We discover intrinsic self-torque-induced chirality switching within Co1/3TaS2, driven purely by current, without the need of heavy metals or a magnetic field, and with high energy efficiency. Our results establish a promising framework for electrically generating and controlling topological spin chirality, and demonstrate a practical route toward chiral spintronics. They can be naturally generalised to other skyrmion systems, offering new opportunities in symmetry control, topological manipulation, and spin-chirality-based quantum functionalities.
Chirality, a central concept across many scientific disciplines, continues to inspire the discovery of novel physical phenomena. In condensed matter physics, structural chirality - defined by the absence of mirror plane symmetries - has primarily been explored in bulk materials. However, new chiral phenomena can emerge uniquely at the interface, distinct from their bulk counterparts, when a chiral material forms a heterostructure. Here, we demonstrate that all van-der-Waals (vdW) heterostructure composed of the chiral Co1/3TaS2 and the achiral vdW ferromagnet Fe3GeTe2 exhibits two distinct and unconventional spin-orbit torques originating from the interfacial chirality. These torques enable magnetic-field-free switching of perpendicular magnetization with ultralow current density ~ 10^6 A/cm^2 and minimal power dissipation < 10^15 W/m^3. Moreover, by replacing Fe3GeTe2 with a similar vdW ferromagnet, Fe3GaTe2, but of higher Curie temperature, we achieved the magnetic-field-free switching at room temperature in the Fe3GaTe2/Co1/3TaS2 vdW heterostructure. Our findings establish interfacial chirality as a powerful new handle for spintronic control, opening a new pathway to explore chirality-induced phenomena beyond the bulk symmetry constraints - and paving the way toward highly efficient, low-power spintronic devices based on all-vdW heterostructures.
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Altermagnetism has recently emerged as a third fundamental branch of magnetism, combining the vanishing net magnetization of antiferromagnets with the high-momentum-dependent spin splitting of ferromagnets. This study provides a comprehensive real- and momentum-space analysis of topological phases in two-dimensional d-wave altermagnets. By employing a tight-binding Hamiltonian, we characterize the topological phase transition occurring at a critical intra-sublattice hopping strength (taCt_a^CtaC​). We examine the emergence of Dirac nodal points and the resulting Berry curvature singularities, supported by a visual analysis of pseudospin texture winding. Crucially, we analize spin splitting, effective altermagnetic strength, and investigate the transport implications of these phases, uncovering giant conductivity anisotropy and spin-dependent ``steering'' effects driven by group velocity distribution across the Fermi surface. Beyond bulk properties, we analyze the edge state topology in ribbon geometries through the lens of information-theoretic markers like fidelity-susceptibility and inverse participation ratio, offering a robust alternative to traditional Chern number calculations, without relying on translational symmetry. Our results demonstrate that the hybridization of edge states in ultra-narrow nanoribbons opens a controllable energy gap, a feature we exploit to propose a novel topological altermagnetic field-effect transistor design where ballistic and spatially spin-polarized transport can be electrostatically gated. This work establishes a theoretical and information-theoretic framework for ``edgetronics'' in altermagnetic materials, paving the way for next-generation, high-speed spintronic and ``spin-splitter'' logic devices and architectures.
The scalar spin chirality (SSC), whose nonzero value ⟨Si⋅(Sj×Sk)⟩≠0\langle {\bf S}_i \cdot ({\bf S}_j \times {\bf S}_k) \rangle \neq 0⟨Si​⋅(Sj​×Sk​)⟩=0 implies the breaking of time-reversal and certain point-group symmetries in the ground state, is a key quantity characterizing chiral magnetism in both classical and quantum settings. The classical SSC is manifested, for instance, in skyrmion crystal phase, while the quantum SSC is still highly sought after in various frustrated spin-1/2 models. An interesting possibility that has not been explored so far is the case in which SSC is symmetry-wise allowed, yet remains zero classically due to the collinear or coplanar arrangement of spins, but is generated by virtue of quantum fluctuation. We demonstrate the existence of precisely such a phase in a spin-1/2 triangular-lattice model with XXZ interaction, spin-orbit-induced exchange interactions, and an external magnetic field. Using iDMRG, we thoroughly map out the phase diagram of the model and identify several phases with coexisting magnetic order and SSC. The nonzero SSC arises despite the classical magnetic order being collinear or coplanar. We provide detailed magnon analysis to ascribe its origin to quantum fluctuations around classical magnetic order. The estimate of SSC from magnon analysis agrees with iDMRG results quantitatively. We map out the magnon spectrum and its Berry curvature, culminating in the prediction of finite thermal Hall conductivity in these phases with SSC.
Recent experiments in moiré quantum materials exhibit quantized Hall states without an external magnetic field, motivating continuum mechanisms based on smooth moiré-periodic pseudospin textures. We present a controlled theory of skyrmion Chern bands generated by such textures. An exact local SU(2)SU(2)SU(2) transformation reveals an emergent non-Abelian gauge field; for large branch splitting we perform an operator-level Schrieffer-Wolff expansion, yielding a single-branch Hamiltonian together with systematically dressed physical operators that define the projected interacting theory beyond strict adiabaticity. The leading dynamics is governed by a U(1)U(1)U(1) Berry connection whose flux is set by the skyrmion density, while controlled non-adiabatic corrections are fixed by the texture's real-space quantum geometric tensor. In a Landau-level representation built from the averaged emergent field, moiré-periodic modulations induce Umklapp-resolved deformations of Girvin-MacDonald-Platzman kinematics and microscopic sources of excess optical quantum weight above the topological lower bound. Assuming a gapped Hall phase, we further derive a skyrmion-crystal effective field theory with a universal Berry-phase term and a noncommutative magnetophonon. Our results provide experimentally accessible signatures for twisted transition-metal dichalcogenide homobilayers and rhombohedral graphene aligned with hexagonal boron nitride.
The interplay between topology and correlation can give rise to exotic collective excitations. The integer and fractional quantum anomalous Hall (QAH) magnets recently discovered in two-dimensional (2D) flatband systems are predicted to host spin excitations distinct from those in conventional magnets. Experimentally, nevertheless, these new excitations remain largely unexplored. Here we investigate spin-valley excitations in a twisted MoTe2 moiré superlattice using resonant ultrafast pump-probe spectroscopy. We observe a metastable spin-valley excitation in the QAH magnet below T ~ 3.7 K that survives reverse magnetic field several times larger than the saturation field. The behavior of this excitation is sharply distinct from ordinary domain walls and magnons, indicating a new type of spin-valley textures unique to topological magnets. We propose that these textures are chiral domain walls with an in-plane winding of the pseudospin order parameter along the domain wall. Their metastability arises from the interplay between the topological winding in real space and the quantum geometry of the parent bands in momentum space through a universal mechanism. These chiral domain walls govern the nonequilibrium dynamics of QAH magnets and may play a central role in their stability. Our study highlights intrinsic quantum geometry effects on spin excitations in topological magnets; and provides key insights into the fundamental mechanism limiting stability of topological protection.