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arXiv:2608.06569

Observation of metastable chiral domain walls in a topological magnet

Richen Xiong, Chenxin Qin, Zhaoyu Han, Nisarg Chadha, Qiang Gao, William Holtzmann, Weijie Li, Jiaqi Cai, Yi Guo, Weihanzhang Guo, Qi Chen, Samuel L. Brantly, Sam Bonkowsky, Chen Huang, Kenji Watanabe, Takashi Taniguchi, Andrea F. Young, Xiaodong Xu, Eslam Khalaf, Chenhao Jin

cond-mat.mes-hallcond-mat.str-elquant-phSubmitted Aug 6, 2026• Announced Aug 10, 2026
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Abstract

The interplay between topology and correlation can give rise to exotic collective excitations. The integer and fractional quantum anomalous Hall (QAH) magnets recently discovered in two-dimensional (2D) flatband systems are predicted to host spin excitations distinct from those in conventional magnets. Experimentally, nevertheless, these new excitations remain largely unexplored. Here we investigate spin-valley excitations in a twisted MoTe2 moiré superlattice using resonant ultrafast pump-probe spectroscopy. We observe a metastable spin-valley excitation in the QAH magnet below T ~ 3.7 K that survives reverse magnetic field several times larger than the saturation field. The behavior of this excitation is sharply distinct from ordinary domain walls and magnons, indicating a new type of spin-valley textures unique to topological magnets. We propose that these textures are chiral domain walls with an in-plane winding of the pseudospin order parameter along the domain wall. Their metastability arises from the interplay between the topological winding in real space and the quantum geometry of the parent bands in momentum space through a universal mechanism. These chiral domain walls govern the nonequilibrium dynamics of QAH magnets and may play a central role in their stability. Our study highlights intrinsic quantum geometry effects on spin excitations in topological magnets; and provides key insights into the fundamental mechanism limiting stability of topological protection.

Comments
4+10 figures

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•Mar 17, 2021•0 citations
The interplay between topology and correlation can give rise to exotic collective excitations. The integer and fractional quantum anomalous Hall (QAH) magnets recently discovered in two-dimensional (2D) flatband systems are predicted to host spin excitations distinct from those in conventional magnets. Experimentally, nevertheless, these new excitations remain largely unexplored. Here we investigate spin-valley excitations in a twisted MoTe2 moiré superlattice using resonant ultrafast pump-probe spectroscopy. We observe a metastable spin-valley excitation in the QAH magnet below T ~ 3.7 K that survives reverse magnetic field several times larger than the saturation field. The behavior of this excitation is sharply distinct from ordinary domain walls and magnons, indicating a new type of spin-valley textures unique to topological magnets. We propose that these textures are chiral domain walls with an in-plane winding of the pseudospin order parameter along the domain wall. Their metastability arises from the interplay between the topological winding in real space and the quantum geometry of the parent bands in momentum space through a universal mechanism. These chiral domain walls govern the nonequilibrium dynamics of QAH magnets and may play a central role in their stability. Our study highlights intrinsic quantum geometry effects on spin excitations in topological magnets; and provides key insights into the fundamental mechanism limiting stability of topological protection.
We study an interacting spinless quadratic band touching model that realizes a topological Mott insulating state. We quench the interaction from a value corresponding to the nematic insulator to that of the quantum anomalous Hall (QAH) ordered phase. We perform time-dependent Hartree-Fock simulations and show that after the quench the system realizes an excited Dirac semimetal state, which is however unstable and spontaneously evolves to a state with inhomogeneous nematic and QAH order parameters. The modulations form a stripe pattern that grows exponentially with time until the local Chern marker reaches unity. The alternating QAH order defines a domain structure with boundaries that host chiral sublattice currents.
We study an interacting spinless quadratic band touching model that realizes a topological Mott insulating state. We quench the interaction from a value corresponding to the nematic insulator to that of the quantum anomalous Hall (QAH) ordered phase. We perform time-dependent Hartree-Fock simulations and show that after the quench the system realizes an excited Dirac semimetal state, which is, however, unstable and spontaneously evolves to a state with inhomogeneous nematic and QAH order parameters. The modulations form a stripe pattern that grows exponentially with time until the local Chern marker reaches unity. The alternating QAH order defines a domain structure with boundaries that host chiral sublattice currents.
Recent experiments in moiré quantum materials exhibit quantized Hall states without an external magnetic field, motivating continuum mechanisms based on smooth moiré-periodic pseudospin textures. We present a controlled theory of skyrmion Chern bands generated by such textures. An exact local SU(2)SU(2)SU(2) transformation reveals an emergent non-Abelian gauge field; for large branch splitting we perform an operator-level Schrieffer-Wolff expansion, yielding a single-branch Hamiltonian together with systematically dressed physical operators that define the projected interacting theory beyond strict adiabaticity. The leading dynamics is governed by a U(1)U(1)U(1) Berry connection whose flux is set by the skyrmion density, while controlled non-adiabatic corrections are fixed by the texture's real-space quantum geometric tensor. In a Landau-level representation built from the averaged emergent field, moiré-periodic modulations induce Umklapp-resolved deformations of Girvin-MacDonald-Platzman kinematics and microscopic sources of excess optical quantum weight above the topological lower bound. Assuming a gapped Hall phase, we further derive a skyrmion-crystal effective field theory with a universal Berry-phase term and a noncommutative magnetophonon. Our results provide experimentally accessible signatures for twisted transition-metal dichalcogenide homobilayers and rhombohedral graphene aligned with hexagonal boron nitride.
Nanoscale topological spin textures in magnetic systems are emerging as promising candidates for scalable quantum architectures. Despite their potential as qubits, previous studies have been limited to semiclassical approaches, leaving a critical gap: the lack of a fully quantum demonstration. Here, we address this challenge by employing the density matrix renormalization group (DMRG) method to establish domain wall (DW) qubits in coupled quantum spin-1/2 chains. We calculate the ground-state energies and excitation gaps of the system and find that DWs with opposite chiralities form a well-defined low-energy sector, distinctly isolated from higher excited states in the presence of anisotropies. This renders the chirality states suitable for encoding quantum information, serving as robust qubits. Interestingly, when a magnetic field is applied, we observe tunneling between quantum DW states with opposite chiralities. Through quantum simulations, we construct an effective qubit Hamiltonian that exhibits strongly anisotropic ggg factors, offering a way to implement single-qubit gates. Furthermore, we obtain an effective interacting Hamiltonian for two mobile DWs in coupled quantum spin chains from DMRG simulations, enabling the implementation of two-qubit gates. Single-qubit and two-qubit gates are also demonstrated in real-time simulations using the time-dependent variational principle. Our work represents a critical step from semiclassical constructions to a fully quantum demonstration of the potential of DW textures for scalable quantum computing, establishing a solid foundation for future quantum architectures based on topological magnetic textures.
Metastability, i.e., partial relaxation to long-lived, quasi-stationary states before true asymptotic equilibrium sets in, emerges ubiquitously in classical and quantum dynamical systems as a result of timescales separation. In open quantum systems, an intrinsically nonequilibrium analogue, dynamical metastability, can originate from the spectral geometry of a non-Hermitian operator. In noninteracting models, this mechanism produces boundary-sensitive anomalous relaxation, transient amplification, and topologically mandated long-lived edge modes, all of which are enhanced as system size grows. Here we extend dynamical metastability into the nonlinear, interacting regime and identify magnetic heterostructures as a natural platform for its exploration. We introduce an interacting spin Lindbladian whose linearized magnon dynamics map onto a dynamically metastable Hatano-Nelson chain, and show that dynamical metastability in the noninteracting limit seeds genuinely nonlinear phenomena, including size-dependent spin dipping and anomalous attraction to unstable equilibria. Long-lived edge states associated to topologically mandated Dirac bosons persist under nonlinearities and disorder. We further analyze the magnetization dynamics in magnetic multilayers within the classical Landau-Lifshitz-Gilbert-Slonczewski framework, identifying Dzyaloshinskii-Moriya interaction, nonlocal damping, and spin-transfer torque as control parameters governing bulk-boundary stability mismatch and band topology. While all the distinctive dynamical phenomena previously identified reappear in this experimentally relevant setting, the LLGS framework also supports multistability and limit cycles that are absent in the quantum model. Our results constitute the first systematic study of dynamical metastability in nonlinear dynamics, directly relevant to spin-torque oscillator arrays, magnonic devices, and beyond.
An SU(4)SU(4)SU(4) chiral spin liquid and quantized dipole Hall effect in moir\'e bilayers
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