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arXiv:2412.11585 · Physical review. B./Physical review. B

Density matrix renormalization group study of domain wall qubits

Guanxiong Qu, Ji Zou, Daniel Loss, Tomoki Hirosawa

Published Jul 30, 2025• 5 citations
arXivHTMLPDF

Abstract

Nanoscale topological spin textures in magnetic systems are emerging as promising candidates for scalable quantum architectures. Despite their potential as qubits, previous studies have been limited to semiclassical approaches, leaving a critical gap: the lack of a fully quantum demonstration. Here, we address this challenge by employing the density matrix renormalization group (DMRG) method to establish domain wall (DW) qubits in coupled quantum spin-1/2 chains. We calculate the ground-state energies and excitation gaps of the system and find that DWs with opposite chiralities form a well-defined low-energy sector, distinctly isolated from higher excited states in the presence of anisotropies. This renders the chirality states suitable for encoding quantum information, serving as robust qubits. Interestingly, when a magnetic field is applied, we observe tunneling between quantum DW states with opposite chiralities. Through quantum simulations, we construct an effective qubit Hamiltonian that exhibits strongly anisotropic $g$ factors, offering a way to implement single-qubit gates. Furthermore, we obtain an effective interacting Hamiltonian for two mobile DWs in coupled quantum spin chains from DMRG simulations, enabling the implementation of two-qubit gates. Single-qubit and two-qubit gates are also demonstrated in real-time simulations using the time-dependent variational principle. Our work represents a critical step from semiclassical constructions to a fully quantum demonstration of the potential of DW textures for scalable quantum computing, establishing a solid foundation for future quantum architectures based on topological magnetic textures.

DOI
10.1103/mpgp-pqk2

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Nanoscale topological spin textures in magnetic systems are emerging as promising candidates for scalable quantum architectures. Despite their potential as qubits, previous studies have been limited to semiclassical approaches, leaving a critical gap: the lack of a fully quantum demonstration. Here, we address this challenge by employing the density matrix renormalization group (DMRG) method to establish domain wall (DW) qubits in coupled quantum spin-1/2 chains. We calculate the ground-state energies and excitation gaps of the system and find that DWs with opposite chiralities form a well-defined low-energy sector, distinctly isolated from higher excited states in the presence of anisotropies. This renders the chirality states suitable for encoding quantum information, serving as robust qubits. Interestingly, when a magnetic field is applied, we observe tunneling between quantum DW states with opposite chiralities. Through quantum simulations, we construct an effective qubit Hamiltonian that exhibits strongly anisotropic ggg factors, offering a way to implement single-qubit gates. Furthermore, we obtain an effective interacting Hamiltonian for two mobile DWs in coupled quantum spin chains from DMRG simulations, enabling the implementation of two-qubit gates. Single-qubit and two-qubit gates are also demonstrated in real-time simulations using the time-dependent variational principle. Our work represents a critical step from semiclassical constructions to a fully quantum demonstration of the potential of DW textures for scalable quantum computing, establishing a solid foundation for future quantum architectures based on topological magnetic textures.
Quantum computers allow to solve efficiently certain problems that are intractable for classical computers. For the realization of a quantum computer, a qubit design as the basic building block is a nontrivial starting point. Within a nanoscale ferromagnetic domain wall stabilized by achiral energy, two degenerate chirality forms exist which can be regarded as the two qubit states. Our numerical demonstration shows that the manipulation of spin configurations of the ferromagnetic domain walls is governed by magnetic and electric fields for single-qubit quantum gates, while the Ising exchange coupling facilitates the two-qubit gates. The incorporation of these quantum gates permits universal quantum computation. Furthermore, we discuss the estimation of the coherence time, as well as the initialization and readout of the qubits. Our findings show a practical implementation of quantum computing architectures based on the domain-wall qubits in ferromagnetic materials.
Domain walls (DWs) on magnetic racetracks are at the core of the field of spintronics, providing a basic element for classical information processing. Here, we show that mobile DWs also provide a blueprint for large-scale quantum computers. Remarkably, these DW qubits showcase exceptional versatility, serving not only as stationary qubits, but also performing the role of solid-state flying qubits that can be shuttled in an ultrafast way. We estimate that the DW qubits are long-lived because they can be operated at sweet spots to reduce potential noise sources. Single-qubit gates are implemented by moving the DW, and two-qubit entangling gates exploit naturally emerging interactions between different DWs. These gates, sufficient for universal quantum computing, are fully compatible with current state-of-the-art experiments on racetrack memories. Further, we discuss possible strategies for qubit readout and initialization, paving the way toward future quantum computers based on mobile topological textures on magnetic racetracks.
The interplay between topology and correlation can give rise to exotic collective excitations. The integer and fractional quantum anomalous Hall (QAH) magnets recently discovered in two-dimensional (2D) flatband systems are predicted to host spin excitations distinct from those in conventional magnets. Experimentally, nevertheless, these new excitations remain largely unexplored. Here we investigate spin-valley excitations in a twisted MoTe2 moiré superlattice using resonant ultrafast pump-probe spectroscopy. We observe a metastable spin-valley excitation in the QAH magnet below T ~ 3.7 K that survives reverse magnetic field several times larger than the saturation field. The behavior of this excitation is sharply distinct from ordinary domain walls and magnons, indicating a new type of spin-valley textures unique to topological magnets. We propose that these textures are chiral domain walls with an in-plane winding of the pseudospin order parameter along the domain wall. Their metastability arises from the interplay between the topological winding in real space and the quantum geometry of the parent bands in momentum space through a universal mechanism. These chiral domain walls govern the nonequilibrium dynamics of QAH magnets and may play a central role in their stability. Our study highlights intrinsic quantum geometry effects on spin excitations in topological magnets; and provides key insights into the fundamental mechanism limiting stability of topological protection.
The application of real space renormalization group methods to quantum lattice models has become a topic of great interest following the development of the density matrix renormalization group by White.This method has been used to find the ground and low-lying excited state energies and wave functions of quantum spin models in which the form of the ground state is not clear, for instance because the interactions are frustrated.It has also been applied to fermion problems where the tendency for localization due to the strong Coulomb repulsion is opposed by the lowering of the kinetic energy which occurs as a result of electron transfer.The approach is particularly suitable for one-, or quasi-one-dimensional problems.The method involves truncating the Hilbert space in a systematic and optimised manner.Results for the ground state energy are thus variational bounds.The results for low-lying energies and correlation functions for one-dimensional systems have unprecedented accuracy and the method has become the method of choice for solving one-dimensional quantum spin problems.We review the method and results obtained for the spin-1 chain with biquadratic exchange as well as the spin-1/2 model with competing nearest and next nearest neighbour exchange will be described.More recently, the density matrix renormalization group has been applied to reformulate the coupling constant renormalization group approach which is appropriate for the study of critical properties.This approach has been applied to the anisotropic spin-1/2 Heisenberg chain.Finally, we discuss recent work which has borne promising applications in two dimensions -the Ising model and the two-dimensional Hubbard model.
Magnetic domain walls have long been pursued as carriers of classical information for storage and processing. With the ability to create, control, and probe domain walls at the nanoscale, they are recently recognized as an ideal platform for studying macroscopic quantum effects and provide a natural blueprint for building scalable quantum computing architectures. In particular, the experimentally demonstrated high mobility of domain walls makes them not only suitable as stationary qubits but also as flying qubits, which may offer advantages over currently explored quantum computing platforms. In this Perspective, we outline our current understanding of the essential ingredients and key requirements for realizing universal quantum computation based on magnetic domain walls. We highlight promising concrete material platforms and identify the experiments that are still needed to advance this concept. We also discuss the potential challenges and point to new opportunities in this emerging research direction at the interface between magnetism and quantum information science.
By using the method of density-matrix renormalization-group theory, the ground-state entanglement in the spin-1/2 isotropic antiferromagnetic Heisenberg chain is studied when there are domain walls generated by a boundary magnetic field. It is found that the pairwise entanglement of odd-bond two qubits decreases and even-bond two qubits increases to stable values alternately when the magnetic field increases. The pairwise entanglement of odd bond can be equal to that of even bond for a suitable value of the magnetic field. When the magnetic field increases further, the entanglement of even bond can be larger than that of odd bond. The entanglement entropy increases and then almost saturates as the number of spin sites increases. Due to the domain walls, the entanglement entropy of even bond decreases to a minimum value and then increases as the magnetic field increases.