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arXiv:2603.14192

Emergent giant topological Hall effect in twisted Fe3GeTe2 metallic system

Hyuncheol Kim, Kai-Xuan Zhang, Yu-Hang Li, Giung Park, Ran Cheng, Je-Geun Park

cond-mat.mtrl-scicond-mat.mes-hallphysics.app-phquant-phSubmitted Mar 15, 2026• Announced Mar 17, 2026
arXivHTMLPDF

Abstract

The topological Hall effect, driven by the exchange interaction between conduction electrons and topological magnetic textures such as skyrmions, is a powerful probe for investigating the topological properties of magnetic materials. Typically, this phenomenon arises in systems with broken global inversion symmetry, where Dzyaloshinskii-Moriya interactions stabilize such textures. Here, we report the discovery of an emergent giant topological Hall effect in the twisted Fe3GeTe2 metallic system, which notably preserves the general global inversion symmetry. This effect manifests exclusively within a narrow window of "magic" twist angles ranging from 0.45° to 0.75°, while it is absent identically outside of that range, highlighting its unique and emergent nature. Micromagnetic simulations reveal that this topological Hall effect originates from a skyrmion lattice induced by alternating in-plane and layer-contrasting Dzyaloshinskii-Moriya interactions that result from local inversion symmetry breaking. Our findings underscore twisted Fe3GeTe2 as a versatile platform for engineering and controlling topological magnetic textures in metallic twisted van der Waals magnets, thereby opening up new avenues for next-generation spintronic devices.

Journal reference
Nature Communications 17, 2931 (2026)
DOI
10.1038/s41467-026-69454-5
Comments
Accepted by Nature Coummunications; 47 pages, 4 main figures, 14 supporting figures

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The topological Hall effect, driven by the exchange interaction between conduction electrons and topological magnetic textures such as skyrmions, is a powerful probe for investigating the topological properties of magnetic materials. Typically, this phenomenon arises in systems with broken global inversion symmetry, where Dzyaloshinskii-Moriya interactions stabilize such textures. Here, we report the discovery of an emergent giant topological Hall effect in the twisted Fe3GeTe2 metallic system, which notably preserves the general global inversion symmetry. This effect manifests exclusively within a narrow window of "magic" twist angles ranging from 0.45° to 0.75°, while it is absent identically outside of that range, highlighting its unique and emergent nature. Micromagnetic simulations reveal that this topological Hall effect originates from a skyrmion lattice induced by alternating in-plane and layer-contrasting Dzyaloshinskii-Moriya interactions that result from local inversion symmetry breaking. Our findings underscore twisted Fe3GeTe2 as a versatile platform for engineering and controlling topological magnetic textures in metallic twisted van der Waals magnets, thereby opening up new avenues for next-generation spintronic devices.
Many-body spin systems represent a paradigmatic platform for the realization of emergent states of matter in a strongly interacting regime. Spin models are commonly studied in one-dimensional periodic chains, whose lattice constant is on the order of the interatomic distance. However, in cold atomic setups or functionalized twisted van der Waals heterostructures, long-range modulations of the spin physics can be engineered. Here we show that such superlattice modulations in a many-body spin Hamiltonian can give rise to observable topological boundary modes in the excitation spectrum of the spin chain. In the case of an XY spin-1/2 chain, these boundary modes stem from a mathematical correspondence with the chiral edge modes of a two-dimensional quantum Hall state. Our results show that the addition of many-body interactions does not close some of the topological gaps in the excitation spectrum, and the topological boundary modes visibly persist in the isotropic Heisenberg limit. These observations carry through when the spin moment is increased and a large-spin limit of the phenomenon is established. Our results show that such spin superlattices provide a promising route to observe many-body topological boundary effects in cold atomic setups and functionalized twisted van der Waals materials.
Magnetic topology is central to modern quantum magnet, where spin chirality governs exotic spin winding, real-space Berry phase, and topological Hall effect. A key unresolved challenge is how to electrically switch topological spin chirality and its associated gauge flux, an essential requirement for manipulating its topological quantum properties. In this work, we propose and experimentally demonstrate the concept of current-switching spin chirality. We identify the new vdW antiferromagnet Co1/3TaS2 as an ideal platform, hosting a topological 3Q state with a minimum chirality cell, an ultrahigh skyrmion density, a non-centrosymmetric geometry, and a strong Berry curvature. We discover intrinsic self-torque-induced chirality switching within Co1/3TaS2, driven purely by current, without the need of heavy metals or a magnetic field, and with high energy efficiency. Our results establish a promising framework for electrically generating and controlling topological spin chirality, and demonstrate a practical route toward chiral spintronics. They can be naturally generalised to other skyrmion systems, offering new opportunities in symmetry control, topological manipulation, and spin-chirality-based quantum functionalities.
Altermagnetism has recently emerged as a third fundamental branch of magnetism, combining the vanishing net magnetization of antiferromagnets with the high-momentum-dependent spin splitting of ferromagnets. This study provides a comprehensive real- and momentum-space analysis of topological phases in two-dimensional d-wave altermagnets. By employing a tight-binding Hamiltonian, we characterize the topological phase transition occurring at a critical intra-sublattice hopping strength (taCt_a^CtaC​). We examine the emergence of Dirac nodal points and the resulting Berry curvature singularities, supported by a visual analysis of pseudospin texture winding. Crucially, we analize spin splitting, effective altermagnetic strength, and investigate the transport implications of these phases, uncovering giant conductivity anisotropy and spin-dependent ``steering'' effects driven by group velocity distribution across the Fermi surface. Beyond bulk properties, we analyze the edge state topology in ribbon geometries through the lens of information-theoretic markers like fidelity-susceptibility and inverse participation ratio, offering a robust alternative to traditional Chern number calculations, without relying on translational symmetry. Our results demonstrate that the hybridization of edge states in ultra-narrow nanoribbons opens a controllable energy gap, a feature we exploit to propose a novel topological altermagnetic field-effect transistor design where ballistic and spatially spin-polarized transport can be electrostatically gated. This work establishes a theoretical and information-theoretic framework for ``edgetronics'' in altermagnetic materials, paving the way for next-generation, high-speed spintronic and ``spin-splitter'' logic devices and architectures.
Topological kagome magnets offer a rich landscape for exploring the intricate interplay of quantum interactions among geometry, topology, spin, and correlation. GdTi3Bi4 crystallizes in layered Ti based kagome nets intertwined with zigzag Gd chains along the a axis and orders antiferromagnetically below 15 K. Here, we present the temperature and field dependent electrical transport of GdTi3Bi4 in different directions. The material exhibits anomalous Hall conductivity (AHC) of 410 S cm-1 at 2 K for B parallel c and it is completely absent for B parallel a, despite the similar magnetization observed in both orientations. This behavior is quite contradictory, as anomalous Hall effect (AHE) typically scales with the magnetization. Through first principles calculations, it is demonstrated that in the presence of time reversal symmetry broken by the Gd 4f sublattice and spin orbit coupling, the magnetization direction controls the orbital mixing in the Ti t2g bands, relocating Berry curvature hot spots and producing the observed orientation selective AHC. The results establish GdTi3Bi4 as platform for investigating new avenues of AHE, such as directional AHE, and thus shed new light on the intricate coupling between magnetic and electronic structures, paving the way for exploring novel quantum phenomena.
Chirality, a central concept across many scientific disciplines, continues to inspire the discovery of novel physical phenomena. In condensed matter physics, structural chirality - defined by the absence of mirror plane symmetries - has primarily been explored in bulk materials. However, new chiral phenomena can emerge uniquely at the interface, distinct from their bulk counterparts, when a chiral material forms a heterostructure. Here, we demonstrate that all van-der-Waals (vdW) heterostructure composed of the chiral Co1/3TaS2 and the achiral vdW ferromagnet Fe3GeTe2 exhibits two distinct and unconventional spin-orbit torques originating from the interfacial chirality. These torques enable magnetic-field-free switching of perpendicular magnetization with ultralow current density ~ 10^6 A/cm^2 and minimal power dissipation < 10^15 W/m^3. Moreover, by replacing Fe3GeTe2 with a similar vdW ferromagnet, Fe3GaTe2, but of higher Curie temperature, we achieved the magnetic-field-free switching at room temperature in the Fe3GaTe2/Co1/3TaS2 vdW heterostructure. Our findings establish interfacial chirality as a powerful new handle for spintronic control, opening a new pathway to explore chirality-induced phenomena beyond the bulk symmetry constraints - and paving the way toward highly efficient, low-power spintronic devices based on all-vdW heterostructures.
Magnetic skyrmions are topologically protected spin textures that are promising candidates for low-power spintronic memory and logic devices. Realizing skyrmion-based devices requires an understanding of how structural disorder affects their stability and transport properties. This study uses Ne+^{+}+ ion irradiation at fluences from 101110^{11}1011 to 101410^{14}1014 ions-cm−2^{-2}−2 to systematically vary defect densities in 80 nm epitaxial FeGe films and quantify the resulting modifications to magnetic phase boundaries and electronic scattering. Temperature- and field-dependent Hall measurements reveal that increasing disorder progressively extends the topological Hall signal from a narrow window near 200K in pristine films down to 4K at the highest fluence, with peak amplitude more than doubling. Simultaneously, the anomalous Hall effect transitions from quadratic Berry curvature scaling to linear skew scattering behavior, with the skew coefficient increasing threefold. These results establish quantitative correlations between defect concentration, skyrmion phase space, and transport mechanisms in a chiral magnet. It demonstrates that ion-beam modification provides systematic control over both topological texture stability and electrical detectability.