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arXiv:1711.07889 · Physical Review Letters

Resonant Thermalization of Periodically Driven Strongly Correlated Electrons

Francesco Peronaci, Marco Schirò, Olivier Parcollet

Published May 8, 2018• 53 citations
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Abstract

We study the dynamics of the Fermi-Hubbard model driven by a time-periodic modulation of the interaction within nonequilibrium dynamical mean-field theory. For moderate interaction, we find clear evidence of thermalization to a genuine infinite-temperature state with no residual oscillations. Quite differently, in the strongly correlated regime, we find a quasistationary extremely long-lived state with oscillations synchronized with the drive (Floquet prethermalization). Remarkably, the nature of this state dramatically changes upon tuning the drive frequency. In particular, we show the existence of a critical frequency at which the system rapidly thermalizes despite the large interaction. We characterize this resonant thermalization and provide an analytical understanding in terms of a breakdown of the periodic Schrieffer-Wolff transformation.

DOI
10.1103/physrevlett.120.197601

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We study the dynamics of the Fermi-Hubbard model driven by a time-periodic modulation of the interaction within nonequilibrium dynamical mean-field theory. For moderate interaction, we find clear evidence of thermalization to a genuine infinite-temperature state with no residual oscillations. Quite differently, in the strongly correlated regime, we find a quasistationary extremely long-lived state with oscillations synchronized with the drive (Floquet prethermalization). Remarkably, the nature of this state dramatically changes upon tuning the drive frequency. In particular, we show the existence of a critical frequency at which the system rapidly thermalizes despite the large interaction. We characterize this resonant thermalization and provide an analytical understanding in terms of a breakdown of the periodic Schrieffer-Wolff transformation.
We demonstrate the existence of long-lived prethermalized states in the Mott insulating Hubbard model driven by periodic electric fields. These states, which also exist in the resonantly driven case with a large density of photo-induced doublons and holons, are characterized by a nonzero current and an effective temperature of the doublons and holons which depends sensitively on the driving condition. Focusing on the specific case of resonantly driven models whose effective time-independent Hamiltonian in the high-frequency driving limit corresponds to noninteracting fermions, we show that the time evolution of the double occupation can be reproduced by the effective Hamiltonian, and that the prethermalization plateaus at finite driving frequency are controlled by the next-to-leading–order correction in the high-frequency expansion of the effective Hamiltonian. We propose a numerical procedure to determine an effective Hubbard interaction that mimics the correlation effects induced by these higher-order terms.
We study the dynamics and stability in a strongly interacting resonantly driven two-band model. Using exact numerical simulations, we find a stable regime at large driving frequencies where the time evolution is governed by a local Floquet Hamiltonian that is approximately conserved out to very long times. For slow driving, on the other hand, the system becomes unstable and heats up to infinite temperature. While thermalization is relatively fast in these two regimes (but to different ``temperatures''), in the crossover between them we find slow nonthermalizing time evolution: temporal fluctuations become strong and temporal correlations long lived. Microscopically, we trace back the origin of this nonthermalizing time evolution to the properties of rare Floquet many-body resonances, whose proliferation at lower driving frequency removes the approximate energy conservation, and thus produces thermalization to infinite temperature.
Prethermalization phenomena in driven systems are generally understood via a local Floquet Hamiltonian obtained from a high-frequency expansion. Remarkably, recently it has been shown that a driven Kitaev spin liquid with fractionalized excitations can realize a quasistationary state that is not captured by this paradigm. Instead distinct types of fractionalized excitations are characterized by vastly different temperatures—a phenomenon dubbed . In our work, we analyze fractionalized prethermalization in a driven one-dimensional Hubbard model at strong coupling which hosts spin-charge fractionalization. At intermediate frequencies quasisteady states emerge which are characterized by a low spin and high charge temperature with lifetimes set by two competing processes: the lifetime of the quasiparticles determined by Fermi's Golden rule and the exponentially long lifetime of a Floquet prethermal plateau. We classify drives into three categories, each giving rise to distinct (fractional) prethermalization dynamics. Resorting to a time-dependent variant of the Schrieffer-Wolff transformation, we systematically analyze how these drive categories are linked to the underlying driven Hubbard model, thereby providing a general understanding of the emergent thermalization dynamics. We discuss routes toward an experimental realization of this phenomenon in quantum simulation platforms.
We use a self-consistent strong-coupling expansion for the self-energy (perturbation theory in the hopping) to describe the nonequilibrium dynamics of strongly correlated lattice fermions. We study the three-dimensional homogeneous Fermi-Hubbard model driven by an external electric field showing that the damping of the ensuing Bloch oscillations depends on the direction of the field and that for a broad range of field strengths a long-lived transient prethermalized state emerges. This long-lived transient regime implies that thermal equilibrium may be out of reach of the time scales accessible in present cold atom experiments but shows that an interesting new quasiuniversal transient state exists in nonequilibrium governed by a thermalized kinetic energy but not a thermalized potential energy. In addition, when the field strength is equal in magnitude to the interaction between atoms, the system undergoes a rapid thermalization, characterized by a different quasiuniversal behavior of the current and spectral function for different values of the hopping.
We investigate a class of periodically driven many-body systems that allows us to extend the phenomenon of prethermalization to the vicinity of isolated intermediate-to-low drive frequencies away from the high-frequency limit. We provide numerical evidence for the formation of a parametrically long-lived prethermal plateau, captured by an effective Floquet Hamiltonian computed using the replica inverse-frequency expansion, and demonstrate its stability with respect to random perturbations in the drive period. Considering exclusively nonintegrable Floquet Hamiltonians, we find that heating rates are nonuniversal: we observe Fermi's golden rule scaling, power-law scaling inconsistent with the golden rule, and non-power-law scaling, depending on the drive. Despite the asymptotic character of the inverse-frequency expansion, we show that it describes the thermostatic properties of the state all along the evolution up to infinite temperature, with higher-order terms improving the accuracy. Our results suggest a dynamical mechanism to gradually increase the temperature in isolated quantum simulators, such as ultracold atoms, and open up an alternative possibility to investigate thermal phase transitions and the interplay between thermal and quantum criticality using Floquet drives.
Time-periodically driven systems are a versatile toolbox for realizing interesting effective Hamiltonians. Heating, caused by excitations to high-energy states, is a challenge for experiments. While most setups so far address the relatively weakly interacting regime, it is of general interest to study heating in strongly correlated systems. Using Floquet dynamical mean-field theory, we study nonequilibrium steady states (NESS) in the Falicov-Kimball model, with time-periodically driven kinetic energy or interaction. We systematically investigate the nonequilibrium properties of the NESS. For a driven kinetic energy, we show that resonant tunneling, where the interaction is an integer multiple of the driving frequency, plays an important role in the heating. In the strongly correlated regime, we show that this can be well understood using Fermi's golden rule and the Schrieffer-Wolff transformation for a time-periodically driven system. We furthermore demonstrate that resonant tunneling can be used to control the population of Floquet states to achieve ``photodoping.'' For driven interactions introduced by an oscillating magnetic field near a widely adopted Feshbach resonance, we find that the double occupancy is strongly modulated. Our calculations apply to shaken ultracold-atom systems and to solid-state systems in a spatially uniform but time-dependent electric field. They are also closely related to lattice modulation spectroscopy. Our calculations are helpful to understand the latest experiments on strongly correlated Floquet systems.