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arXiv:1709.03021 · Physical review. B./Physical review. B

Nonequilibrium steady states and resonant tunneling in time-periodically driven systems with interactions

Tao Qin, Walter Hofstetter

Published Mar 12, 2018• 23 citations

Abstract

Time-periodically driven systems are a versatile toolbox for realizing interesting effective Hamiltonians. Heating, caused by excitations to high-energy states, is a challenge for experiments. While most setups so far address the relatively weakly interacting regime, it is of general interest to study heating in strongly correlated systems. Using Floquet dynamical mean-field theory, we study nonequilibrium steady states (NESS) in the Falicov-Kimball model, with time-periodically driven kinetic energy or interaction. We systematically investigate the nonequilibrium properties of the NESS. For a driven kinetic energy, we show that resonant tunneling, where the interaction is an integer multiple of the driving frequency, plays an important role in the heating. In the strongly correlated regime, we show that this can be well understood using Fermi's golden rule and the Schrieffer-Wolff transformation for a time-periodically driven system. We furthermore demonstrate that resonant tunneling can be used to control the population of Floquet states to achieve ``photodoping.'' For driven interactions introduced by an oscillating magnetic field near a widely adopted Feshbach resonance, we find that the double occupancy is strongly modulated. Our calculations apply to shaken ultracold-atom systems and to solid-state systems in a spatially uniform but time-dependent electric field. They are also closely related to lattice modulation spectroscopy. Our calculations are helpful to understand the latest experiments on strongly correlated Floquet systems.

DOI: 10.1103/physrevb.97.125115

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We study the dynamics of the Fermi-Hubbard model driven by a time-periodic modulation of the interaction within nonequilibrium dynamical mean-field theory. For moderate interaction, we find clear evidence of thermalization to a genuine infinite-temperature state with no residual oscillations. Quite differently, in the strongly correlated regime, we find a quasistationary extremely long-lived state with oscillations synchronized with the drive (Floquet prethermalization). Remarkably, the nature of this state dramatically changes upon tuning the drive frequency. In particular, we show the existence of a critical frequency at which the system rapidly thermalizes despite the large interaction. We characterize this resonant thermalization and provide an analytical understanding in terms of a breakdown of the periodic Schrieffer-Wolff transformation.

Laser technology has developed and accelerated photo-induced nonequilibrium physics, from both the scientific and engineering viewpoints. Floquet engineering, i.e., controlling material properties and functionalities by time-periodic drives, is at the forefront of quantum physics of light-matter interaction. However, it is limited to ideal dissipationless systems. Extending Floquet engineering to various materials requires understanding of the quantum states emerging in a balance of the periodic drive and energy dissipation. Here, we derive a general description for nonequilibrium steady states (NESSs) in periodically driven dissipative systems by focusing on systems under high-frequency drive and time-independent Lindblad-type dissipation. Our formula correctly describes the time average, fluctuation, and symmetry properties of the NESS, and can be computed efficiently in numerical calculations. This approach will play fundamental roles in Floquet engineering in a broad class of dissipative quantum systems from atoms and molecules to mesoscopic systems, and condensed matter.

We study the dynamics and timescales of a periodically driven Fermi-Hubbard model in a three-dimensional hexagonal lattice. The evolution of the Floquet many-body state is analyzed by comparing it to an equivalent implementation in undriven systems. The dynamics of double occupancies for the near- and off-resonant driving regime indicate that the effective Hamiltonian picture is valid for several orders of magnitude in modulation time. Furthermore, we show that driving a hexagonal lattice compared to a simple cubic lattice allows us to modulate the system up to 1 s, corresponding to hundreds of tunneling times, with only minor atom loss. Here, driving at a frequency close to the interaction energy does not introduce resonant features to the atom loss.

Periodically driven quantum systems provide a powerful route to engineer novel states of matter by controlling their effective Hamiltonians through external fields. However, most treatments are usually simplified by considering the high-frequency limit, and do not account for the processes taking place in the transient regime during the onset of the drive. In this work, we introduce a time and momentum resolved tunneling spectroscopy protocol to probe the instantaneous energy spectrum of Floquet-driven systems beyond the high-frequency regime, capturing both emergent effects and non-adiabatic phenomena without requiring explicit reconstruction of the full time-dependent Green's function. We benchmark the method on driven non-interacting fermionic models, and then generalize the approach to strongly correlated systems with the aid of time-dependent density matrix renormalization group techniques. We also provide a microscopic description to the emergence of in-gap states under resonant driving, and briefly explore its finite temperature analog.

We perform an ab initio comparison between nonequilibrium dynamical mean-field theory and optical lattice experiments by studying the time evolution of double occupations in the periodically driven Fermi-Hubbard model. For off-resonant driving, the range of validity of a description in terms of an effective static Hamiltonian is determined and its breakdown due to energy absorption close to resonance is demonstrated. For near-resonant driving, we investigate the response to a change in driving amplitude and discover an asymmetric excitation spectrum with respect to the detuning. In general, we find good agreement between experiment and theory, which cross validates the experimental and numerical approaches in a strongly correlated nonequilibrium system.

Experiments on periodically driven quantum systems have effectively realized quasi-Hamiltonians, in the sense of Floquet theory, that are otherwise inaccessible in static condensed matter systems. Although the Floquet quasi-Hamiltonians are time-independent, however, these continuously driven systems can still suffer from heating due to a secular growth in the expectation value of the time-dependent physical Hamiltonian. Here we use an exact space-time mapping to construct a class of many-body systems with rapid periodic driving which we nonetheless prove to be completely free of heating, by mapping them exactly onto time-independent systems. The absence of heating despite the periodic driving occurs in these cases of harmonically trapped dilute Bose gas because the driving is a certain periodic but anharmonic modulation of the gas's two-body contact interaction, at a particular frequency. Although we prove that the absence of heating is exact within full quantum many-body theory, we then use mean-field theory to simulate 'Floquet heating spectroscopy' and compute the heating rate when the driving frequency is varied away from the critical value for zero heating. In both weakly and strongly non-linear regimes, the heating rate as a function of driving frequency appears to show a number of Fano resonances, suggesting that the exactly proven absence of heating at the critical frequency may be explained in terms of destructive interferences between excitation modes.