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arXiv:1612.02713 · IEEE Transactions on Applied Superconductivity

NbN/AlN/NbN Josephson Junctions on Sapphire for SIS Receiver Applications

Michael Merker, Christian Bohn, Marvin Vollinger, Konstantin Ilin, Michael Siegel

Published Dec 9, 2016• 6 citations
arXivHTMLPDF

Abstract

The most developed integrated receivers for THz radiation nowadays are based on Josephson junction superconductor-insulator-superconductor devices. In this kind of devices, the highest receivable frequency is determined by the energy gap of the superconducting electrodes and limited to approximately 700 GHz in case of Nb/AlOx/Nb multilayers. We have developed a technology for NbN/AlN/NbN Josephson junctions on sapphire substrates which allow operation at frequencies above 1 THz. The trilayers are deposited in situ in a three-chamber dc-magnetron sputtering system at temperatures as high as 775 °C. Each layer is reactively sputtered in an argon and nitrogen atmosphere. By variation of the partial gas pressures and discharge current of the plasma, optimum deposition conditions for the tri-layers were found. So far, gap voltages as high as 5.1 mV at 4.2 K have been achieved which allows the operation frequency of the JJ devices to exceed 1 THz.

DOI
10.1109/tasc.2016.2631841

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•Jul 13, 2005•1 citation
The most developed integrated receivers for THz radiation nowadays are based on Josephson junction superconductor-insulator-superconductor devices. In this kind of devices, the highest receivable frequency is determined by the energy gap of the superconducting electrodes and limited to approximately 700 GHz in case of Nb/AlOx/Nb multilayers. We have developed a technology for NbN/AlN/NbN Josephson junctions on sapphire substrates which allow operation at frequencies above 1 THz. The trilayers are deposited in situ in a three-chamber dc-magnetron sputtering system at temperatures as high as 775 °C. Each layer is reactively sputtered in an argon and nitrogen atmosphere. By variation of the partial gas pressures and discharge current of the plasma, optimum deposition conditions for the tri-layers were found. So far, gap voltages as high as 5.1 mV at 4.2 K have been achieved which allows the operation frequency of the JJ devices to exceed 1 THz.
To improve the performance of Josephson oscillators and SIS mixers over 700 GHz, we have developed a fabrication process to grow epitaxial NbN/MgO/NbN trilayers by reactive dc-sputtering. Trilayers were fabricated on a single-crystal MgO substrate at ambient temperature. NbN and MgO films were deposited by reactive dc-sputtering with an Nb and Mg target, respectively. The MgO inter-layer thickness was changed up to 480 nm, but, T/sub C/ and 20-K resistivity of the NbN upper-layer showed no remarkable dependency and they were 15.7 K and about 60 /spl mu//spl Omega/cm, respectively. To evaluate the RF performance of the epitaxial NbN films, we fabricated Josephson junctions with a microstrip resonator constructed from an epitaxial NbN/MgO/NbN trilayer. The I-V characteristics of the junction exhibited resonance steps up to 2.5 mV, which suggests that the epitaxial NbN films have low loss up to 1.2 THz.
We have fabricated both NbN/Ta x N/NbN SN*S-type, NbN/MgO/NbN SIS-type Josephson junctions and microwave band-pass filters on different substrates (Si, Sapphire, MgO). NbN films have been deposited on both sides of (100) oriented, 250 µm thick, MgO substrates with a high crystalline texture quality. The aim was to investigate the performances and the maximum achievable operating frequency in an NbN based RSFQ modulator front-end of an ADC in the 4 K-10 K temperature range. We observed that Ta x N thin films can be tuned from an insulating phase to a superconducting phase (Tc ∼4K) by varying the nitrogen content during sputter deposition while the barrier height of MgO can also be controlled by deposition conditions and by tri-layer postdeposition annealing. Junction properties (Jc∼10-25 kA/cm 2 ), Mac Cumber parameter and RnIc product measured up to 1 mV are shown to be controlled by the reactive sputtering conditions. We have designed three pole band-pass filters and resonators in a micro-strip configuration and studied the junction coupling with the filters. We will show that a sigma-delta NbN technology is a suitable solution for analogue-to-digital conversion in the future generations of telecommunication satellites to achieve high sampling frequency and large bandwidth at high carrier frequency signal.
A generic NbN Superconducting Tunnel Junctions (STJ) technology has been developed using conventional substrates (Si and SOI-SIMOX) for making THz spectrometers including SIS receivers and RSFQ logic gates. NbN/MgO/NbN junctions with area of 1 /spl mu/m/sup 2/, Jc of 10 kA/cm/sup 2/ and low sub-gap leakage current (Vm>25 mV) are currently obtained from room temperature sputtered multilayers followed by a post-annealing at 250/spl deg/C. Using a thin MgO buffer layer deposited underneath the NbN electrodes, ensures lower NbN surface resistance values (Rs=7 /spl mu//spl Omega/) at 10 GHz and 4 K. Epitaxial NbN [100] films on MgO [100] with high gap frequency (1.4 THz) have also been achieved under the same deposition conditions at room temperature. The NbN SIS has shown good I-V photon induced steps when LO pumped at 300 GHz. We have developed an 8 levels Al/NbN multilayer process for making 1.5 THz SIS mixers (including Al antennas) on Si membranes patterned in SOI-SIMOX. Using the planarization techniques developed at the Si-MOS CEA-LETI Facility, we have also demonstrated on the possibility of extending our NbN technology to high level RSFQ circuit integration with 0.5 /spl mu/m/sup 2/ junction area, made on large area substrates (up to 8 inches).
Heterodyne mixers based on superconducting SIS (superconductor-insulator-superconductor) tunnel junctions have been demonstrated to be the most sensitive coherent detectors at millimeter and submillimeter wavelengths. In fact, conventional superconducting SIS mixers with Nb/AlOx/Nb junction and Nb/SiO2/Nb tuning circuit have shown good performances with the noise temperature reaching as low as three times the quantum limit below 0.7THz, which is the gap frequency of Nb-based SIS junctions. However, due to the large loss in Nb thin-film superconducting microstrip lines, the noise performance of Nb SIS mixers deteriorates significantly above 0.7THz. With a gap frequency double that of Nb-based SIS junctions, NbN-based SIS junctions are of particular interest for the development of heterodyne mixers in the terahertz region. Considering the bandwidth and output power of local-oscillator (LO) signal sources are quite limited around 1THz, we firstly develop a waveguide NbN-based SIS mixer at 0.5THz. Three types of SIS junctions, i.e., long junction, parallel-connected tunnel junction (PCTJ) and distributed junction array (DJ) are investigated. They are all comprised of NbN-AlN-NbN tri-layer fabricated on an MgO substrate and have the same current density (Jc) of 10kA/cm2. In this paper, we describe their design, fabrication and preliminary experimental results.
We have evaluated the electrical characteristics of NbN/Al-AlNx/NbN tunnel junctions fabricated on sapphire-C or fused-silica substrates. NbN/Al-AlNx/NbN multilayers were prepared by reactive dc-magnetron sputtering deposition of lower and upper NbN layers, and rf-magnetron sputtering deposition of the Al layer, followed by radical-nitridation. The junctions showed low sub-gap leakage currents in the current-voltage characteristics at 4.2 K. The quality parameter, Rsg/Rn, where respective Rsgand Rnare the sub-gap resistance at 2 mV and junction resistance at 5 mV, was above 15. The gap voltage (Vg) was around 3.3 mV, which was reduced in comparison with Vgvalues of ~4.3 mV for junctions on MgO substrates. The reduced Vgwas caused by superconducting properties of lower NbN layers deposited on the sapphire or fused-silica substrates. Uniformity in critical current (Ic) was relatively good, and the maximum-to-minimum spread in Icwas ±1.7% for 200 junctions on a sapphire substrate and ±2.0% for the junctions on a fused-silica substrate.
ABSTRACT: Active superconducting circuits based on picoseconds switching, i.e. THz oscillating, Josephson tunnel junctions are expected to find a large domain of applications in spatial sub-millimeter wave and FIR detectors as well as in satellite based wideband signal and data processors. In the first case SIS (superconductor-insulator-superconductor) tunnel junctions are required, while in the second case SNS (superconductor-normal metal-superconductor) self-shunted junctions are preferred. We present the advantages of the nitride junction technology currently developed at CEA-Grenoble, based on high-performance MTS (medium temperature superconductor) NbN films in both SIS and SNS junctions. In the SIS case the device performances rely on a sputter deposited and post-annealed, only 0.5-0.7 nm thick, dielectric MgO barrier. This leads to junctions with a Josephson critical current in the range of 10-25 kA/cm, and a large superconducting energy gap (> 5 meV) associated with a low sub-gap quasi-particle leakage current. These parameters are suitable for low “noise temperature ” heterodyne mixers, local oscillators, and integrated receivers in the 0.8 to 1.4 THz frequency range. In the SNS case, a new