After reviewing the interpretation of laser operation as a nonequilibrium Bose-Einstein condensation phase transition, we illustrate the novel features arising from the nonequilibrium nature of photon and polariton Bose-Einstein condensates recently observed in experiments. We then propose a quantitative criterion to experimentally assess the equilibrium versus nonequilibrium nature of a specific condensation process, based on fluctuation-dissipation relations. The power of this criterion is illustrated on two models which show very different behaviors. Historical and Conceptual Introduction The first introduction of concepts of nonequilibrium statistical mechanics into the realm of optics dates back to the early 1970s with pioneering works by Graham and Haken [1] and by DeGiorgio and Scully [2], who proposed a very insightful interpretation of the laser threshold in terms of a spontaneous breaking of the U( 1 ) symmetry associated with the phase of the emitted light. Similar to what happens to the order parameter at a second-order phase transition, such an optical phase is randomly chosen every time the device is switched on and remains constant for macroscopic times. Moreover, a long-range spatial order is established, as light emitted by a laser device above threshold is phase-coherent on macroscopic distances. While textbooks typically discuss this interpretation of laser operation in terms of a phase transition for the simplest case of a single-mode laser cavity, rigorously speaking this is valid only in spatially infinite systems. In fact, only in this case one can observe nonanalytic behaviors of the physical quantities at the transition point. In particular, the long-range order is typically assessed by looking at the long-distance behavior of the correlation function of the order parameter, which, for a laser, corresponds to the first-order spatial coherence of the emitted electric field, the spontaneous symmetry breaking is signaled by this quantity becoming nonzero (see Chapter 5). The average is taken on the stationary density matrix of the system. In order to be able to probe this long-distance behavior, experimental studies need devices with a spatially extended active region.
After reviewing the interpretation of laser operation as a nonequilibrium Bose-Einstein condensation phase transition, we illustrate the novel features arising from the nonequilibrium nature of photon and polariton Bose-Einstein condensates recently observed in experiments. We then propose a quantitative criterion to experimentally assess the equilibrium versus nonequilibrium nature of a specific condensation process, based on fluctuation-dissipation relations. The power of this criterion is illustrated on two models which show very different behaviors. Historical and Conceptual Introduction The first introduction of concepts of nonequilibrium statistical mechanics into the realm of optics dates back to the early 1970s with pioneering works by Graham and Haken [1] and by DeGiorgio and Scully [2], who proposed a very insightful interpretation of the laser threshold in terms of a spontaneous breaking of the U( 1 ) symmetry associated with the phase of the emitted light. Similar to what happens to the order parameter at a second-order phase transition, such an optical phase is randomly chosen every time the device is switched on and remains constant for macroscopic times. Moreover, a long-range spatial order is established, as light emitted by a laser device above threshold is phase-coherent on macroscopic distances. While textbooks typically discuss this interpretation of laser operation in terms of a phase transition for the simplest case of a single-mode laser cavity, rigorously speaking this is valid only in spatially infinite systems. In fact, only in this case one can observe nonanalytic behaviors of the physical quantities at the transition point. In particular, the long-range order is typically assessed by looking at the long-distance behavior of the correlation function of the order parameter, which, for a laser, corresponds to the first-order spatial coherence of the emitted electric field, the spontaneous symmetry breaking is signaled by this quantity becoming nonzero (see Chapter 5). The average is taken on the stationary density matrix of the system. In order to be able to probe this long-distance behavior, experimental studies need devices with a spatially extended active region.
The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity.In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms.The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity.We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory.At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition.We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry.In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
The problem of understanding how a coherent, macroscopic Bose- Einstein condensate (BEC) emerges from the cooling of a thermal Bose gas has attracted significant theoretical and experimental interest over several decades. The pioneering achievement of BEC in weakly interacting dilute atomic gases in 1995 was followed by a number of experimental studies examining the growth of the BEC number, as well as the development of its coherence. More recently, there has been interest in connecting such experiments to universal aspects of nonequilibrium phase transitions, in terms of both static and dynamical critical exponents. Here, the spontaneous formation of topological structures such as vortices and solitons in quenched cold-atom experiments has enabled the verification of the Kibble-Zurek mechanism predicting the density of topological defects in continuous phase transitions, first proposed in the context of the evolution of the early universe. This chapter reviews progress in the understanding of BEC formation and discusses open questions and future research directions in the dynamics of phase transitions in quantum gases. Introduction The equilibrium phase diagram of the dilute Bose gas exhibits a continuous phase transition between condensed and noncondensed phases. The order parameter characteristic of the condensed phase vanishes above some critical temperature T c and grows continuously with decreasing temperature below this critical point. However, the dynamical process of condensate formation has proved to be a challenging phenomenon to address both theoretically and experimentally. This formation process is a crucial aspect of Bose systems and of direct relevance to all condensates discussed in this book, despite their evident system-specific properties. Important questions leading to intense discussions in the early literature include the time scale for condensate formation and the role of inhomogeneities and finite-size effects in “closed” systems. These issues are related to the concept of spontaneous symmetry breaking, its causes, and implications for physical systems (see, for example, Chapter 5 by Snoke and Daley). In this chapter, we give an overview of the dynamics of condensate formation and describe the present understanding provided by increasingly well-controlled cold-atom experiments and corresponding theoretical advances over the past twenty years. We focus on the growth of BECs in cooled Bose gases, which, from a theoretical standpoint, requires a suitable nonequilibrium formalism.
Bose-Einstein condensation is a state of matter for which massive bosons develop a macroscopic occupation of the ground state. After the theoretical discovery by Bose and Einstein, it took approximately 70 years to be experimentally realized using Rubidium-87 atoms. Ever since, many different species have been shown to Bose condense. The key in these experiments is cooling down atoms temperatures below 200 nK, while maintaining a large density. Despite all these species, it was thought that photons could not Bose condense. This changed in 2010 when the first Bose-Einstein condensate of photons (phBEC) was achieved. In a table top experiment photons are confined to a dye-filled microcavity where under the right conditions a thermalized photon gas is achieved. Using our setup, we quantitatively show from both the spectral and spatial distribution of photons in the microcavity that a macroscopic occupation of the ground state is achieved, i.e. a condensate of photons. The achievement of phBEC in a dye-filled microcavity has led to a renewed interest in the density distribution of the ideal Bose gas in a two-dimensional harmonic oscillator. We present measurements of the radial profile of photons inside the microcavity below and above the critical point for phBEC with a large signal-to-noise ratio. We obtain good agreement with theoretical profiles obtained using exact summation of eigenstates. An interesting open question is, whether the photons in the condensate are interacting or non-interacting and as a consequence, whether the condensate is also a superfluid or only forms a macroscopically occupied ground state, as predicted by Einstein. When increasing the photon density, we observe an increase in the radius of the condensate which we attribute to effective repulsive interactions. For several dye concentrations we accurately determine the radius of the condensate as a function of the number of condensate photons, and derive from the measurements an effective interaction strength. In many systems ranging from condensed matter physics and particle physics to cosmology, phase transitions and spontaneous symmetry breaking play a crucial role. The information of a polarized condensate from an unpolarized thermal cloud constitutes a directly observable prototype of spontaneous symmetry breaking. For every single-shot of the pump laser, we determine the Stokes parameters of the photons inside the microcavity which fully characterizes the polarization state of the sample. By varying experimental parameters, we investigate if the polarization is randomly chosen from shot-to-shot of the experiment. The dye-filled microcavity is a beautiful tool to achieve phBEC. However, it cannot provide the periodic potential required to achieve quantum phase transitions, such as the Mott insulator that have been so successfully exploited in the field of ultra-cold atoms. We use a local density approach to simulate large-area photonic crystal cavities. Clever interplay with both the electronic and photonic bandgap of these cavities has the potential of achieving phBEC in a periodic potential. We show that when the hole radius varies quadratically as a function of position, the eigenmodes of the photonic crystal can be described by the corresponding eigenmodes of the quantum harmonic oscillator.
The realisation of Bose-Einstein condensation under grand-canonical conditions has provided the experimental evidence for the simultaneous occurrence of macroscopic fluctuations and phase coherence of the condensate. The observation of these two features, against a consolidated tradition which wants the fluctuations to be pathological (grand-canonical catastrophe) and incompatible with spontaneous symmetry braking, calls for a comprehensive rethinking of the approach to the problem. In this paper we consider the uniform ideal gas in a box and we present an alternative conceptual framework. We show that the usually-employed Bogoliubov quasi-average construction fails to reproduce the broken-symmetry state. The observed features are accounted for by a different pattern of spontaneous symmetry breaking, characterised by condensation of fluctuations and long-range correlations of the order parameter.
The question of whether Bose-Einstein condensation involves spontaneous symmetry breaking is surprisingly controversial. We review the theory of spontaneous symmetry breaking in ferromagnets, compare it with the theory of symmetry breaking in condensates, and discuss the different viewpoints on the correspondence to experiments. These viewpoints include alternative perspectives in which we can treat condensates with fixed particle numbers, and where coherence arises from measurements. This question relates to whether condensates of quasiparticles such as polaritons can be viewed as “real” condensates. Introduction Spontaneous symmetry breaking is a deep subject in physics with long historical roots. At the most basic level, it arises in the field of cosmology. Physicists have long had an aesthetic principle that leads us to expect symmetry in the all of the basic equations of physical law. Yet the universe is manifestly full of asymmetries. How does a symmetric system acquire asymmetry merely by evolving in time? Starting in the 1950s, cosmologists began to borrow the ideas of spontaneous symmetry breaking from condensed matter physics, which were originally developed to explain spontaneous magnetization in ferromagnetic systems. Spontaneous coherence in all its forms (e.g., Bose-Einstein condensation [BEC], superconductivity, and lasing) can be viewed as another type of symmetry breaking. The Hamiltonian of the system is symmetric, yet under some conditions, the energy of the system can be reduced by putting the system into a state with asymmetry, namely, a state with a common phase for a macroscopic number of particles. The symmetry of the system implies that it does not matter what the exact choice of that phase is, as long as it is the same for all the particles. It is not obvious, however, whether the symmetry breaking which occurs in spontaneous coherence of the type seen in lasers or in Bose-Einstein condensation is the same as that seen in ferromagnetic systems. There are similarities in the systems which encourage the same view of all types of symmetry breaking, but there are also differences. In fact, there is a substantial school of thought that symmetry breaking in Bose-Einstein condensates with ultracold atoms is a “convenient fiction” (a term applied to optical coherence by Mølmer [1]).
The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity. In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms. The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity. We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory. At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition. We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry. In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.