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Physics

Liquid-crystalline phases of ultracold atoms

Jonathan Keeling, Joe Bhaseen, Benjamin D. Simons

Published Oct 18, 2010• 4 citations
Publisher

Abstract

The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity.In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms.The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity.We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory.At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition.We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry.In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.

DOI
10.1103/physics.3.88

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The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity.In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms.The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity.We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory.At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition.We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry.In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity. In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms. The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity. We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory. At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition. We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry. In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
"Spatially modulated ordered states, such as crystals, liquid crystals, and antiferromagnets, are ubiquitous in nature but relatively difficult to realize in ultracold atomic systems. In the present work, we present a scheme for generating controllable cavity-mediated interactions between atoms, and show that these interactions give rise to a crystallization transition in the case of a transversely pumped optical cavity. We focus on the case of multimode cavities, in which the interactions are relatively local and the range of possible ordered configurations (and consequently of low-energy fluctuations) is large; as we show, the crystallization transition for a Bose-Einstein condensate in a multimode cavity is driven first-order by fluctuations, through the Brazovskii effect. The ordered state to which this crystallization transition gives rise is a ""supersolid,"" possessing both superfluid and solid order. We address the crystallization transition and the properties of the ordered state, discuss the experimental feasibility of observing these, and finally show how ordering in layered systems of atoms is geometrically frustrated. We then introduce a more straightforward realization of frustrated cavity-mediated interactions, viz. systems of randomly-positioned spins in multimode cavities. We show by means of a mapping to a variant of the Hopfield associative-memory model that such systems exhibit a spin-glass phase. Finally, we consider a different ultracold-atomic setting---that of spin-orbit-coupled Bose gases---in which the Brazovskii effect has a profound influence on the low-temperature phases, leading to a universal preference for stripe-like ordering at zero temperature and bosonic pair condensation at nonzero temperatures."
Coherent scattering of light from ultracold atoms involves an exchange of energy and momentum introducing a wealth of nonlinear dynamical phenomena.As a prominent example, particles can spontaneously form stationary periodic configurations that simultaneously maximize the light scattering and minimize the atomic potential energy in the emerging optical lattice.Such self-ordering effects resulting in periodic lattices via bimodal symmetry breaking have been experimentally observed with cold gases and Bose-Einstein condensates (BECs) inside an optical resonator.Here, we study a new regime of periodic pattern formation for an atomic BEC in free space, driven by far off-resonant counterpropagating and noninterfering lasers of orthogonal polarization.In contrast to previous works, no spatial light modes are preselected by any boundary conditions and the transition from homogeneous to periodic order amounts to a crystallization of both light and ultracold atoms breaking a continuous translational symmetry.In the crystallized state the BEC acquires a phase similar to a supersolid with an emergent intrinsic length scale whereas the light field forms an optical lattice allowing phononic excitations via collective backscattering, which are gapped due to the infinte-range interactions.The system we study constitutes a novel configuration allowing the simulation of synthetic solid-state systems with ultracold atoms including long-range phonon dynamics.
Atoms in transversely pumped optical cavities ``self-organize'' by forming a density wave and emitting superradiantly into the cavity mode(s). For a single-mode cavity, the properties of this self-organization transition are well characterized both theoretically and experimentally. Here, we explore the self-organization of a Bose-Einstein condensate in the presence of two cavity modes---a system that recently was realized experimentally [L\'eonard et al., Nature (London) 543, 87 (2017)]. We argue that this system can exhibit a ``vestigially ordered'' phase in which neither cavity mode exhibits superradiance but the cavity modes are mutually phase locked by the atoms. We argue that this vestigially ordered phase should generically be present in multimode cavity geometries.
Pattern formation of atoms in high-finesse optical resonators results from the mechanical forces of light associated with superradiant scattering into the cavity mode. It occurs when the laser intensity exceeds a threshold value such that the pumping processes counteract the losses. We consider atoms driven by a laser and coupling with a mode of a standing-wave cavity and describe their dynamics with a Fokker-Planck equation, in which the atomic motion is semiclassical but the cavity field is a full quantum variable. The asymptotic state of the atoms is a thermal state, whose temperature is solely controlled by the detuning between the laser and the cavity frequency and by the cavity loss rate. From this result we derive the free energy and show that in the thermodynamic limit self-organization is a second-order phase transition. The order parameter is the field inside the resonator to which one can associate a magnetization in analogy to ferromagnetism, the control field is the laser intensity, but the steady state is intrinsically out of equilibrium. In the symmetry-broken phase, quantum noise induces jumps of the spatial density between two ordered patterns: We characterize the statistical properties of this temporal behavior at steady state and show that the thermodynamic properties of the system can be extracted by detecting the light at the cavity output. The results of our analysis are in full agreement with previous studies; we extend them by deriving a self-consistent theory which is valid also when the cavity field is in the shot-noise limit and elucidate the nature of the self-organization transition.
Ultracold bosonic atoms in optical lattices self-organize into a variety of structural and quantum phases when placed into a single-mode cavity and pumped by a laser. Cavity optomechanical effects induce an atom density modulation at the cavity-mode wavelength that competes with the optical lattice arrangement. Simultaneously short-range interactions via particle hopping promote superfluid order such that a variety of structural and quantum coherent phases can occur. We analyze the emerging phase diagram in two dimensions by means of an extended Bose-Hubbard model using a local mean-field approach combined with a superfluid cluster analysis. For commensurate ratios of the cavity and external lattice wavelengths, the Mott insulator-superfluid transition is modified by the appearance of charge density wave and supersolid phases, at which the atomic density supports the buildup of a cavity field. For incommensurate ratios, the optomechanical forces induce the formation of Bose-glass and superglass phases, namely, nonsuperfluid and superfluid phases, respectively, displaying quasiperiodic density modulations, which in addition can exhibit structural and superfluid stripe formation. The onset of such structures is constrained by the on-site interaction and is favorable at fractional densities. Experimental observables are identified and discussed.