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arXiv:1601.04900 · Physical Review X

Spontaneous Crystallization of Light and Ultracold Atoms

Stefan Ostermann, F. Piazza, Helmut Ritsch

Published May 24, 2016• 64 citations
arXivHTMLPDF

Abstract

Coherent scattering of light from ultracold atoms involves an exchange of energy and momentum introducing a wealth of nonlinear dynamical phenomena.As a prominent example, particles can spontaneously form stationary periodic configurations that simultaneously maximize the light scattering and minimize the atomic potential energy in the emerging optical lattice.Such self-ordering effects resulting in periodic lattices via bimodal symmetry breaking have been experimentally observed with cold gases and Bose-Einstein condensates (BECs) inside an optical resonator.Here, we study a new regime of periodic pattern formation for an atomic BEC in free space, driven by far off-resonant counterpropagating and noninterfering lasers of orthogonal polarization.In contrast to previous works, no spatial light modes are preselected by any boundary conditions and the transition from homogeneous to periodic order amounts to a crystallization of both light and ultracold atoms breaking a continuous translational symmetry.In the crystallized state the BEC acquires a phase similar to a supersolid with an emergent intrinsic length scale whereas the light field forms an optical lattice allowing phononic excitations via collective backscattering, which are gapped due to the infinte-range interactions.The system we study constitutes a novel configuration allowing the simulation of synthetic solid-state systems with ultracold atoms including long-range phonon dynamics.

DOI
10.1103/physrevx.6.021026

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Coherent scattering of light from ultracold atoms involves an exchange of energy and momentum introducing a wealth of nonlinear dynamical phenomena.As a prominent example, particles can spontaneously form stationary periodic configurations that simultaneously maximize the light scattering and minimize the atomic potential energy in the emerging optical lattice.Such self-ordering effects resulting in periodic lattices via bimodal symmetry breaking have been experimentally observed with cold gases and Bose-Einstein condensates (BECs) inside an optical resonator.Here, we study a new regime of periodic pattern formation for an atomic BEC in free space, driven by far off-resonant counterpropagating and noninterfering lasers of orthogonal polarization.In contrast to previous works, no spatial light modes are preselected by any boundary conditions and the transition from homogeneous to periodic order amounts to a crystallization of both light and ultracold atoms breaking a continuous translational symmetry.In the crystallized state the BEC acquires a phase similar to a supersolid with an emergent intrinsic length scale whereas the light field forms an optical lattice allowing phononic excitations via collective backscattering, which are gapped due to the infinte-range interactions.The system we study constitutes a novel configuration allowing the simulation of synthetic solid-state systems with ultracold atoms including long-range phonon dynamics.
The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity. In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms. The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity. We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory. At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition. We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry. In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity.In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms.The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity.We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory.At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition.We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry.In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
Superfluids under specific conditions can exhibit spontaneous breaking of continuous translation symmetries and form exotic spatially ordered states of matter known as supersolids. Despite its early theoretical prediction, it took over half-a-centrury to experimentally demonstrate the supersolid phase in ultracold atomic Bose-Einstein condensates, forming due to long-range interatomic interactions. Here we propose as a promising new platform for supersolidity exciton-polariton superfluids, confined in annular optically induced traps. The supersolid phase emerges due to effective attractive interactions, mediated by the normal excitonic component of the system. Experimental demonstration of spontaneously formed spatially ordered phase is in agreement with detailed mean-field theoretical analysis and numerical simulation. The spontaneous character of the observed supersolid transition is further evidenced by the formation of specific zero-energy Nambu-Goldstone modes in the collective excitation spectrum.
Although crystallization is a ubiquitous phenomenon in nature, crystal formation and melting still remain fascinating processes with several open questions yet to be addressed. In this work we study the emergent crystallization of a laser-driven dipolar Bose-Einstein condensate due to the interplay between long-range magnetic and effectively infinite-range light-induced interactions. The competition between these two interactions results in a collective excitation spectrum with two-roton minima that introduce two different length scales at which crystalline order can emerge. In addition to the formation of regular crystals with simple periodic patterns due to the softening of one of the rotons, we find that both rotons can also soften simultaneously, resulting in the formation of exotic, complex periodic, or aperiodic density patterns. We also demonstrate dynamic state-preparation schemes for achieving all the crystalline ground states found for experimentally relevant and feasible parameter regimes.
Matter waves inside periodic potentials are well known from solid-state physics, where electrons interacting with a crystal lattice are considered. Atomic Bose-Einstein condensates inside light-induced periodic potentials (optical lattices) share many features with electrons in solids, but also with light waves in nonlinear materials and other nonlinear systems. Generally, atom-atom interactions in Bose-Einstein condensates lead to rich and interesting nonlinear effects. Furthermore, the experimental control over the parameters of the periodic potential and the condensate make it possible to enter regimes inaccessible in other systems. In this review, an introduction to the physics of ultracold bosonic atoms in optical lattices is given and an overview of the theoretical and experimental advances to date.
Self-structuring via symmetry breaking is a prominent collective phenomenon occurring in cold and ultracold atoms coupled to optical fields [1] . Experimental realizations by means of trapped dipolar gases and optical cavities have shed light onto supersolidity and crystallization in out-of-equilibrium atomic systems [2] , [3] . Recent work demonstrated the occurrence of structural phase transitions between hexagonally coordinated supersolid phases in dipolar condensates [4] . In this work, we address 2D structural transitions occurring in an ensemble of cold thermal atoms with effective optomechanical interactions mediated by a coherent beam retro-reflected by means of a feedback mirror. The feedback loop scheme is represented in Fig. 1(a) , where the dipole potential induces atomic density structures which, in turn, scatter photons into side-band modes enhancing the potential itself and leading to transverse light-atom self-structuring, sharing similarities with an effective-Kerr nonlinear medium [5] .