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arXiv:1007.0922 · Physical Review A

Atom-light crystallization of Bose-Einstein condensates in multimode cavities: Nonequilibrium classical and quantum phase transitions, emergent lattices, supersolidity, and frustration

Sarang Gopalakrishnan, Benjamin Lev, Paul M. Goldbart

Published Oct 18, 2010• 108 citations
arXivHTMLPDF

Abstract

The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity. In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms. The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity. We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory. At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition. We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry. In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.

DOI
10.1103/physreva.82.043612

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The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity. In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms. The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity. We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory. At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition. We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry. In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
The self-organization of a Bose-Einstein condensate (BEC) in a transversely pumped optical cavity is a process akin to crystallization: when pumped by a laser of sufficient intensity, the coupled matter and light fields evolve, spontaneously, into a spatially modulated pattern, or crystal, whose lattice structure is dictated by the geometry of the cavity.In cavities having multiple degenerate modes, the quasicontinuum of possible lattice arrangements, and the continuous symmetry breaking associated with the adoption of a particular lattice arrangement, give rise to phenomena such as phonons, defects, and frustration, which have hitherto been unexplored in ultracold atomic settings involving neutral atoms.The present work develops a nonequilibrium field-theoretic approach to explore the self-organization of a BEC in a pumped, lossy optical cavity.We find that the transition is well described, in the regime of primary interest, by an effective equilibrium theory.At nonzero temperatures, the self-organization occurs via a fluctuation-driven first-order phase transition of the Brazovskii class; this transition persists to zero temperature and crosses over into a quantum phase transition.We make further use of our field-theoretic description to investigate the role of nonequilibrium fluctuations in the self-organization transition, as well as to explore the nucleation of ordered-phase droplets, the nature and energetics of topological defects, supersolidity in the ordered phase, and the possibility of frustration controlled by the cavity geometry.In addition, we discuss the range of experimental parameters for which we expect the phenomena described here to be observable, along with possible schemes for detecting ordering and fluctuations via either atomic correlations or the correlations of the light emitted from the cavity.
"Spatially modulated ordered states, such as crystals, liquid crystals, and antiferromagnets, are ubiquitous in nature but relatively difficult to realize in ultracold atomic systems. In the present work, we present a scheme for generating controllable cavity-mediated interactions between atoms, and show that these interactions give rise to a crystallization transition in the case of a transversely pumped optical cavity. We focus on the case of multimode cavities, in which the interactions are relatively local and the range of possible ordered configurations (and consequently of low-energy fluctuations) is large; as we show, the crystallization transition for a Bose-Einstein condensate in a multimode cavity is driven first-order by fluctuations, through the Brazovskii effect. The ordered state to which this crystallization transition gives rise is a ""supersolid,"" possessing both superfluid and solid order. We address the crystallization transition and the properties of the ordered state, discuss the experimental feasibility of observing these, and finally show how ordering in layered systems of atoms is geometrically frustrated. We then introduce a more straightforward realization of frustrated cavity-mediated interactions, viz. systems of randomly-positioned spins in multimode cavities. We show by means of a mapping to a variant of the Hopfield associative-memory model that such systems exhibit a spin-glass phase. Finally, we consider a different ultracold-atomic setting---that of spin-orbit-coupled Bose gases---in which the Brazovskii effect has a profound influence on the low-temperature phases, leading to a universal preference for stripe-like ordering at zero temperature and bosonic pair condensation at nonzero temperatures."
Coherent scattering of light from ultracold atoms involves an exchange of energy and momentum introducing a wealth of nonlinear dynamical phenomena.As a prominent example, particles can spontaneously form stationary periodic configurations that simultaneously maximize the light scattering and minimize the atomic potential energy in the emerging optical lattice.Such self-ordering effects resulting in periodic lattices via bimodal symmetry breaking have been experimentally observed with cold gases and Bose-Einstein condensates (BECs) inside an optical resonator.Here, we study a new regime of periodic pattern formation for an atomic BEC in free space, driven by far off-resonant counterpropagating and noninterfering lasers of orthogonal polarization.In contrast to previous works, no spatial light modes are preselected by any boundary conditions and the transition from homogeneous to periodic order amounts to a crystallization of both light and ultracold atoms breaking a continuous translational symmetry.In the crystallized state the BEC acquires a phase similar to a supersolid with an emergent intrinsic length scale whereas the light field forms an optical lattice allowing phononic excitations via collective backscattering, which are gapped due to the infinte-range interactions.The system we study constitutes a novel configuration allowing the simulation of synthetic solid-state systems with ultracold atoms including long-range phonon dynamics.
Atoms in transversely pumped optical cavities ``self-organize'' by forming a density wave and emitting superradiantly into the cavity mode(s). For a single-mode cavity, the properties of this self-organization transition are well characterized both theoretically and experimentally. Here, we explore the self-organization of a Bose-Einstein condensate in the presence of two cavity modes---a system that recently was realized experimentally [L\'eonard et al., Nature (London) 543, 87 (2017)]. We argue that this system can exhibit a ``vestigially ordered'' phase in which neither cavity mode exhibits superradiance but the cavity modes are mutually phase locked by the atoms. We argue that this vestigially ordered phase should generically be present in multimode cavity geometries.
We present a novel cavity QED system in which a Bose–Einstein condensate (BEC) is trapped within a high-finesse optical cavity whose length may be adjusted to access both single-mode and multimode configurations. We demonstrate the coupling of an atomic ensemble to the cavity in both configurations and measure that the single-atom, -mode cooperativity exceeds unity. The atoms are confined either within an intracavity far-off-resonance optical dipole trap or a crossed optical dipole trap via transversely oriented lasers. Multimode cavity QED provides fully emergent and dynamical optical lattices for intracavity BECs, in that the process of atomic self-organization may be described as a continuous symmetry breaking phase transition resulting in the emergence of a compliant lattice with phonon-like excitations. Such systems will enable explorations of quantum soft matter, including superfluid smectics, superfluid glasses, and spin glasses as well as neuromorphic associative memory.
We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.