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arXiv:1508.06606 · Physical Review A

Thermodynamics and dynamics of atomic self-organization in an optical cavity

Stefan Schütz, Simon B. Jäger, Giovanna Morigi

Published Dec 7, 2015• 29 citations
arXivHTMLPDF

Abstract

Pattern formation of atoms in high-finesse optical resonators results from the mechanical forces of light associated with superradiant scattering into the cavity mode. It occurs when the laser intensity exceeds a threshold value such that the pumping processes counteract the losses. We consider atoms driven by a laser and coupling with a mode of a standing-wave cavity and describe their dynamics with a Fokker-Planck equation, in which the atomic motion is semiclassical but the cavity field is a full quantum variable. The asymptotic state of the atoms is a thermal state, whose temperature is solely controlled by the detuning between the laser and the cavity frequency and by the cavity loss rate. From this result we derive the free energy and show that in the thermodynamic limit self-organization is a second-order phase transition. The order parameter is the field inside the resonator to which one can associate a magnetization in analogy to ferromagnetism, the control field is the laser intensity, but the steady state is intrinsically out of equilibrium. In the symmetry-broken phase, quantum noise induces jumps of the spatial density between two ordered patterns: We characterize the statistical properties of this temporal behavior at steady state and show that the thermodynamic properties of the system can be extracted by detecting the light at the cavity output. The results of our analysis are in full agreement with previous studies; we extend them by deriving a self-consistent theory which is valid also when the cavity field is in the shot-noise limit and elucidate the nature of the self-organization transition.

DOI
10.1103/physreva.92.063808

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Pattern formation of atoms in high-finesse optical resonators results from the mechanical forces of light associated with superradiant scattering into the cavity mode. It occurs when the laser intensity exceeds a threshold value such that the pumping processes counteract the losses. We consider atoms driven by a laser and coupling with a mode of a standing-wave cavity and describe their dynamics with a Fokker-Planck equation, in which the atomic motion is semiclassical but the cavity field is a full quantum variable. The asymptotic state of the atoms is a thermal state, whose temperature is solely controlled by the detuning between the laser and the cavity frequency and by the cavity loss rate. From this result we derive the free energy and show that in the thermodynamic limit self-organization is a second-order phase transition. The order parameter is the field inside the resonator to which one can associate a magnetization in analogy to ferromagnetism, the control field is the laser intensity, but the steady state is intrinsically out of equilibrium. In the symmetry-broken phase, quantum noise induces jumps of the spatial density between two ordered patterns: We characterize the statistical properties of this temporal behavior at steady state and show that the thermodynamic properties of the system can be extracted by detecting the light at the cavity output. The results of our analysis are in full agreement with previous studies; we extend them by deriving a self-consistent theory which is valid also when the cavity field is in the shot-noise limit and elucidate the nature of the self-organization transition.
Photons mediate long-range optomechanical forces between atoms in high-finesse resonators, which can induce the formation of ordered spatial patterns. When a transverse laser drives the atoms, the system undergoes a second-order phase transition that separates a uniform spatial density from a Bragg grating maximizing scattering into the cavity and is controlled by the laser intensity. Starting from a Fokker-Planck equation describing the semiclassical dynamics of the NNN-atom distribution function, we systematically develop a mean-field model and analyze its predictions for the equilibrium and out-of-equilibrium dynamics. The validity of the mean-field model is tested by comparison with the numerical simulations of the NNN-body Fokker-Planck equation and by means of a Bogoliubov-Born-Green-Kirkwood-Yvon (BBGKY) hierarchy. The mean-field theory predictions well reproduce several results of the NNN-body Fokker-Planck equation for sufficiently short times and are in good agreement with existing theoretical approaches based on field-theoretical models. The mean field, on the other hand, predicts thermalization time scales which are at least one order of magnitude shorter than the ones predicted by the NNN-body dynamics. We attribute this discrepancy to the fact that the mean-field ansatz discards the effects of the long-range incoherent forces due to cavity losses.
Atoms can spontaneously form spatially ordered structures in optical resonators when they are transversally driven by lasers. This occurs when the laser intensity exceeds a threshold value and results from the mechanical forces on the atoms associated with superradiant scattering into the cavity mode. We treat the atomic motion semiclassically and show that, while the onset of spatial ordering depends on the intracavity-photon number, the stationary momentum distribution is a Gaussian function whose width is determined by the rate of photon losses. Above threshold, the dynamics is characterized by two time scales: after a violent relaxation, the system slowly reaches the stationary state over time scales exceeding the cavity lifetime by several orders of magnitude. In this transient regime the atomic momenta form non-Gaussian metastable distributions, which emerge from the interplay between the long-range dispersive and dissipative mechanical forces of light. We argue that the dynamics of self-organization of atoms in cavities offers a test bed for studying the statistical mechanics of long-range interacting systems.
The semiclassical dynamics of atoms, when the atoms are confined inside a standing-wave high-finesse resonator, is theoretically studied. The atoms are cooled by scattering processes in which the photons of a transverse laser are coherently scattered into the cavity mode. We derive a Fokker-Planck equation for the atomic center-of-mass variables which allows us to determine the equations of motion in the semiclassical limit for any value of the intensity of the laser field. We extract its prediction for the dynamics when the resonator is essentially in the vacuum state and the atoms are cooled by scattering photons into the cavity mode, which then decays. Its predictions for the stationary atomic distribution are compared with the ones of the Fokker-Planck equation by Domokos et al. [J. Phys. B 34, 187 (2001)], which has been derived under different assumptions. We find full agreement in the considered parameter regime.
Active atomic clocks are predicted to provide far better short-term stability and robustness against thermal fluctuations than typical feedback-based optical atomic clocks. However, continuous laser operation using an ensemble of clock atoms still remains an experimentally challenging task. We study spatial self-organization in a transversely driven ensemble of clock atoms inside an optical resonator and coherent light emission from the cavity. We focus on the spectral properties of the emitted light in the narrow atomic linewidth regime, where the phase coherence providing frequency stability is stored in the atomic dipoles rather than the cavity field. The atoms are off-resonantly driven by a standing-wave coherent laser transversely to the cavity axis, allowing for atomic motion along the cavity axis as well as along the pump. In order to treat larger atom numbers we employ a second-order cumulant expansion which allows us to calculate the spectrum of the cavity light field. We identify the self-organization threshold where the atoms align themselves in a checkerboard pattern, thus maximizing light scattering into the cavity, which simultaneously induces cooling. For a larger driving intensity, more atoms are transferred to the excited state, reducing cooling but increasing light emission from the excited atoms. This can be enhanced via a second cavity mode at the atomic frequency spatially shifted by a quarter wavelength. For large enough atom numbers we observe laser-like emission close to the bare atomic transition frequency.
When atoms scatter photons from a transverse laser into a high-finesse optical cavity, they form crystalline structures which maximize the intracavity light field and trap the atoms in the ordered array. Stable organization occurs when the laser field amplitude exceeds a certain threshold. For planar single-mode cavities there exist two equivalent possible atomic patterns, which determine the phase of the intracavity light field. Under these premises, we show that the effect of an additional laser pumping the cavity makes one pattern more favorable than the other and that it can dynamically force the system into a predetermined configuration. This is an instance of pattern formation and seeding in a nonlinear quantum-optical system.
We study a transversely pumped atomic Bose-Einstein condensate coupled to a single-mode optical cavity, where effective atom-atom interactions are mediated by pump and cavity photons. A number of experiments and theoretical works have shown the formation of a superradiant state in this setup, where interference of pump and cavity light leads to an optical lattice in which atoms self-consistently organize. This self-organization has been extensively studied using the approximate Dicke model (truncating to two momentum states), as well as through numerical Gross-Pitaevskii simulations in one and two dimensions. Here, we perform a full mean-field analysis of the system, including all relevant atomic momentum states and the cavity field. We map out the steady-state phase diagram vs pump strength and cavity detuning, and provide an in-depth understanding of the instabilities that are linked to the emergence of spatiotemporal patterns. We find and describe parameter regimes where the mean field predicts bistability, regimes where the dynamics form chaotic trajectories, instabilities caused by resonances between normal mode excitations, and states with atomic dynamics but vanishing cavity field.