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arXiv:quant-ph/0509207 · Physical Review A

Quantum entanglement in the two-impurity Kondo model

Sam Young Cho, Ross H. McKenzie

Published Jan 19, 2006• 63 citations
arXivHTMLPDF

Abstract

In order to quantify quantum entanglement in two-impurity Kondo systems, we calculate the concurrence, negativity, and von Neumann entropy. The entanglement of the two Kondo impurities is shown to be determined by two competing many-body effects, namely the Kondo effect and the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction, $I$. Due to the spin-rotational invariance of the ground state, the concurrence and negativity are uniquely determined by the spin-spin correlation between the impurities. It is found that there exists a critical minimum value of the antiferromagnetic correlation between the impurity spins which is necessary for entanglement of the two impurity spins. The critical value is discussed in relation with the unstable fixed point in the two-impurity Kondo problem. Specifically, at the fixed point there is no entanglement between the impurity spins. Entanglement will only be created [and quantum information processing (QIP) will only be possible] if the RKKY interaction exchange energy, $I$, is at least several times larger than the Kondo temperature, ${T}_{K}$. Quantitative criteria for QIP are given in terms of the impurity spin-spin correlation.

DOI
10.1103/physreva.73.012109

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In order to quantify quantum entanglement in two-impurity Kondo systems, we calculate the concurrence, negativity, and von Neumann entropy. The entanglement of the two Kondo impurities is shown to be determined by two competing many-body effects, namely the Kondo effect and the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction, III. Due to the spin-rotational invariance of the ground state, the concurrence and negativity are uniquely determined by the spin-spin correlation between the impurities. It is found that there exists a critical minimum value of the antiferromagnetic correlation between the impurity spins which is necessary for entanglement of the two impurity spins. The critical value is discussed in relation with the unstable fixed point in the two-impurity Kondo problem. Specifically, at the fixed point there is no entanglement between the impurity spins. Entanglement will only be created [and quantum information processing (QIP) will only be possible] if the RKKY interaction exchange energy, III, is at least several times larger than the Kondo temperature, TK{T}_{K}TK​. Quantitative criteria for QIP are given in terms of the impurity spin-spin correlation.
We propose that real-space properties of the two-impurity Kondo model can be obtained from an effective spin model where two single-impurity Kondo spin chains are joined via an Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between the two impurity spins. We then use a density matrix renormalization group approach, valid in all ranges of parameters, to study its features using two complementary quantum-entanglement measures, the negativity and the von Neumann entropy. This nonperturbative approach enables us to uncover the precise dependence of the spatial extent ξ(K) of the Kondo screening cloud with the Kondo and RKKY couplings. Our results reveal an exponential suppression of the Kondo temperature T(K)~1/ξ(K) with the size of the effective impurity spin in the limit of large ferromagnetic RKKY coupling, a striking display of "Kondo resonance narrowing" in the two-impurity Kondo model. We also show how the antiferromagnetic RKKY interaction produces an effective decoupling of the impurities from the bulk already for intermediate strengths of this interaction, and, furthermore, exhibit how the non-Fermi liquid quantum critical point is signaled in the quantum entanglement between various parts of the system.
Competition between the Kondo effect and Ruderman-Kittel-Kasuya-Yosida interaction in the two-impurity Kondo problem can be phenomenologically described by the Rasul-Schlottmann spin model. We revisit this model from the quantum entanglement perspective by calculating both the inter-impurity entanglement and the local Kondo entanglement, the latter being the entanglement between a local magnetic impurity and its spatially nearby conduction electron. A groundstate phase diagram is derived and a discontinuous breakdown of the local Kondo entanglement is found at the singular point, associated concomitantly with a jump in the inter-impurity entanglement. An entanglement monogamy holds in the whole phase diagram. Our results identify the important role of the frustrated cross-coupling and demonstrate the local characteristic of the quantum phase transition in the two-impurity Kondo problem. The implications of these results for Kondo lattices and quantum information processing are also briefly discussed.
We study the ground-state entanglement properties of nanostructured Kondo systems consisting of a pair of impurity spins coupled to a background of confined electrons. The competition between the Ruderman-Kittel-Kasuya-Yosida-like coupling and the Kondo effect determines the development of quantum correlations between the different parts of the system. A key element is the electronic filling due to confinement. An even electronic filling leads to results similar to those found previously for extended systems, where the properties of the reduced impurity spin subsystem are uniquely determined by the spin-correlation function defining a one-dimensional phase space. An odd filling, instead, breaks spin rotation symmetry unfolding a two-dimensional phase space showing rich entanglement characteristics as, e.g., the requirement of a larger amount of entanglement for the development of nonlocal correlations between impurity spins. We illustrate these results by numerical simulations of elliptic quantum corrals with magnetic impurities at the foci as a case study.
We propose a model of a strongly-interacting two-impurity Kondo system based on the Anti-de Sitter/Conformal Field Theory (AdS/CFT) correspondence, also known as holography. In a Landau Fermi Liquid, the single-impurity Kondo effect is the screening of an impurity spin at low temperature T . The two-impurity Kondo model then describes the competition between the Kondo interaction and the Heisenberg interaction between two impurity spins, also called the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. For spin-1/2 impurities, that competition leads to a quantum phase transition from a Kondo-screened phase to a phase in which the two impurity spins screen one another. Our holographic model is based on a (1 + 1)-dimensional CFT description of the two-impurity Kondo model, reliable for two impurities with negligible separation in space. We consider only impurity spins in a totally anti-symmetric representation of an SU(N ) spin symmetry. We employ a large-N limit, in which both Kondo and RKKY couplings are double-trace, and both Kondo and inter-impurity screening appear as condensation of single-trace operators at the impurities’ location. We perform the holographic renormalization of our model, which allows us to identify the Kondo and RKKY couplings as boundary conditions on fields in AdS. We numerically compute the phase diagram of our model in the plane of RKKY coupling versus T , finding evidence for a quantum phase transition from a trivial phase, with neither Kondo nor inter-impurity screening, to a non-trivial phase, with both Kondo and anti-ferromagnetic inter-impurity screening. More generally we show, just using SU(N ) representation theory, that ferromagnetic correlations must be absent at leading order in the large-N limit. Our holographic model may be useful for studying many open problems involving strongly-interacting quantum impurities, including for example the Kondo lattice, relevant for describing the heavy fermion compounds.
We study the two-impurity Kondo model (TIKM) in two dimensions with spin-orbit coupled conduction electrons. In the first part of the paper we analyze how spin-orbit interactions of Rashba as well as Dresselhaus type influence the Kondo and Ruderman-Kittel-Kasuya-Yoshida (RKKY) interactions in the TIKM, generalizing results obtained by H. Imamura et al. [Phys. Rev. B 69, 121303(R) (2004)] and J. Malecki [J. Stat. Phys. 129, 741 (2007)]. Using our findings we then explore the effect from spin-orbit interactions on the non-Fermi-liquid quantum critical transition between the RKKY-singlet and Kondo-screened RKKY-triplet states. We argue that spin-orbit interactions under certain conditions produce a line of critical points exhibiting the same leading scaling behavior as that of the ordinary TIKM. In the second part of the paper we shift focus and turn to the question of how spin-orbit interactions affect the entanglement between two localized RKKY-coupled spins in the parameter regime where the competition from the direct Kondo interaction can be neglected. Using data for a device with two spinful quantum dots patterned in a gated InAs heterostructure we show that a gate-controlled spin-orbit interaction may drive a maximally entangled state to one with vanishing entanglement or vice versa (as measured by the concurrence). This has important implications for proposals using RKKY interactions for nonlocal control of qubit entanglement in semiconductor heterostructures.
We investigate the equilibrium and real-time properties of the spin-correlation function $\ensuremath{\langle}{\stackrel{P\vec}{S}}_{1}{\stackrel{P\vec}{S}}_{2}\ensuremath{\rangle}$ in the two-impurity Kondo model for different distances RRR between the two-impurity spins. It is shown that the competition between the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction and the Kondo effect governs the amplitude of $\ensuremath{\langle}{\stackrel{P\vec}{S}}_{1}{\stackrel{P\vec}{S}}_{2}\ensuremath{\rangle}$. For distances RRR exceeding the Kondo length scale, the Kondo effect also has a profound effect on the sign of the correlation function. For ferromagnetic Heisenberg couplings JJJ between the impurities and the conduction band, the Kondo effect is absent and the correlation function only decays for distances beyond a certain length scale introduced by finite temperature. The real-time dynamics after a sudden quench of the system reveals that correlations propagate through the conduction band with Fermi velocity. We identify two distinct timescales for the long-time behavior, which reflects that for small JJJ the system is driven by the RKKY interaction while for large JJJ the Kondo effect dominates. Interestingly, we find that at certain distances a one-dimensional dispersion obeying $\ensuremath{\epsilon}(k)=\ensuremath{\epsilon}(\ensuremath{-}k)$ may lead to a local parity conservation of the impurities such that $\ensuremath{\langle}{\stackrel{P\vec}{S}}_{1}{\stackrel{P\vec}{S}}_{2}\ensuremath{\rangle}$ becomes a conserved quantity for long times and does not decay to its equilibrium value.