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arXiv:1510.08123 · Journal of High Energy Physics

A holographic two-impurity Kondo model

Andy O’Bannon, Ioannis Papadimitriou, Jonas Probst

Published Jan 1, 2016• 25 citations

Abstract

We propose a model of a strongly-interacting two-impurity Kondo system based on the Anti-de Sitter/Conformal Field Theory (AdS/CFT) correspondence, also known as holography. In a Landau Fermi Liquid, the single-impurity Kondo effect is the screening of an impurity spin at low temperature T . The two-impurity Kondo model then describes the competition between the Kondo interaction and the Heisenberg interaction between two impurity spins, also called the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. For spin-1/2 impurities, that competition leads to a quantum phase transition from a Kondo-screened phase to a phase in which the two impurity spins screen one another. Our holographic model is based on a (1 + 1)-dimensional CFT description of the two-impurity Kondo model, reliable for two impurities with negligible separation in space. We consider only impurity spins in a totally anti-symmetric representation of an SU(N ) spin symmetry. We employ a large-N limit, in which both Kondo and RKKY couplings are double-trace, and both Kondo and inter-impurity screening appear as condensation of single-trace operators at the impurities’ location. We perform the holographic renormalization of our model, which allows us to identify the Kondo and RKKY couplings as boundary conditions on fields in AdS. We numerically compute the phase diagram of our model in the plane of RKKY coupling versus T , finding evidence for a quantum phase transition from a trivial phase, with neither Kondo nor inter-impurity screening, to a non-trivial phase, with both Kondo and anti-ferromagnetic inter-impurity screening. More generally we show, just using SU(N ) representation theory, that ferromagnetic correlations must be absent at leading order in the large-N limit. Our holographic model may be useful for studying many open problems involving strongly-interacting quantum impurities, including for example the Kondo lattice, relevant for describing the heavy fermion compounds.

DOI: 10.1007/jhep01(2016)103

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We propose a model of a strongly-interacting two-impurity Kondo system based on the Anti-de Sitter/Conformal Field Theory (AdS/CFT) correspondence, also known as holography. In a Landau Fermi Liquid, the single-impurity Kondo effect is the screening of an impurity spin at low temperature T . The two-impurity Kondo model then describes the competition between the Kondo interaction and the Heisenberg interaction between two impurity spins, also called the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction. For spin-1/2 impurities, that competition leads to a quantum phase transition from a Kondo-screened phase to a phase in which the two impurity spins screen one another. Our holographic model is based on a (1 + 1)-dimensional CFT description of the two-impurity Kondo model, reliable for two impurities with negligible separation in space. We consider only impurity spins in a totally anti-symmetric representation of an SU(N ) spin symmetry. We employ a large-N limit, in which both Kondo and RKKY couplings are double-trace, and both Kondo and inter-impurity screening appear as condensation of single-trace operators at the impurities’ location. We perform the holographic renormalization of our model, which allows us to identify the Kondo and RKKY couplings as boundary conditions on fields in AdS. We numerically compute the phase diagram of our model in the plane of RKKY coupling versus T , finding evidence for a quantum phase transition from a trivial phase, with neither Kondo nor inter-impurity screening, to a non-trivial phase, with both Kondo and anti-ferromagnetic inter-impurity screening. More generally we show, just using SU(N ) representation theory, that ferromagnetic correlations must be absent at leading order in the large-N limit. Our holographic model may be useful for studying many open problems involving strongly-interacting quantum impurities, including for example the Kondo lattice, relevant for describing the heavy fermion compounds.

We propose that real-space properties of the two-impurity Kondo model can be obtained from an effective spin model where two single-impurity Kondo spin chains are joined via an Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between the two impurity spins. We then use a density matrix renormalization group approach, valid in all ranges of parameters, to study its features using two complementary quantum-entanglement measures, the negativity and the von Neumann entropy. This nonperturbative approach enables us to uncover the precise dependence of the spatial extent ξ(K) of the Kondo screening cloud with the Kondo and RKKY couplings. Our results reveal an exponential suppression of the Kondo temperature T(K)~1/ξ(K) with the size of the effective impurity spin in the limit of large ferromagnetic RKKY coupling, a striking display of "Kondo resonance narrowing" in the two-impurity Kondo model. We also show how the antiferromagnetic RKKY interaction produces an effective decoupling of the impurities from the bulk already for intermediate strengths of this interaction, and, furthermore, exhibit how the non-Fermi liquid quantum critical point is signaled in the quantum entanglement between various parts of the system.

The competition between the Kondo screening and indirect magnetic exchange in systems with two magnetic impurities coupled to a conventional

s

-wave superconductor gives rise to a nontrivial ground-state phase diagram. Here, we utilize the density matrix renormalization group (DMRG) method and exploit the non-Abelian spin-SU(2) symmetry to study the phase diagram for two quantum spin-

\frac{1}{2}

impurities locally exchange coupled to large one-dimensional chains. The nonlocal interimpurity exchange is treated as an emergent Ruderman-Kittel-Kasuya-Yosida (RKKY) coupling. We find qualitatively different phase diagrams for impurity spins coupled to sites with odd or even distances

d

on the chain and a partial Kondo-screened spin-doublet phase that extends over the whole range of local exchange couplings

J

in the limit of weak superconducting pairing strength $\mathrm{\ensuremath{\Delta}}$. Our numerical DMRG studies are complemented by exact diagonalization of small (quantum-box) systems and by perturbative-in-

J

computations of the

d

- and $\mathrm{\ensuremath{\Delta}}$-dependent RKKY interaction. It is thereby demonstrated that the specific system geometry is essential for our understanding of magnetic impurity interactions in superconducting hosts, and thus for insights into the control of quantum-state properties in nanoparticle systems and topological superconductivity.

In order to quantify quantum entanglement in two-impurity Kondo systems, we calculate the concurrence, negativity, and von Neumann entropy. The entanglement of the two Kondo impurities is shown to be determined by two competing many-body effects, namely the Kondo effect and the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction,

I

. Due to the spin-rotational invariance of the ground state, the concurrence and negativity are uniquely determined by the spin-spin correlation between the impurities. It is found that there exists a critical minimum value of the antiferromagnetic correlation between the impurity spins which is necessary for entanglement of the two impurity spins. The critical value is discussed in relation with the unstable fixed point in the two-impurity Kondo problem. Specifically, at the fixed point there is no entanglement between the impurity spins. Entanglement will only be created [and quantum information processing (QIP) will only be possible] if the RKKY interaction exchange energy,

I

, is at least several times larger than the Kondo temperature,

{T}_{K}

. Quantitative criteria for QIP are given in terms of the impurity spin-spin correlation.

Competition between the Kondo effect and Ruderman-Kittel-Kasuya-Yosida interaction in the two-impurity Kondo problem can be phenomenologically described by the Rasul-Schlottmann spin model. We revisit this model from the quantum entanglement perspective by calculating both the inter-impurity entanglement and the local Kondo entanglement, the latter being the entanglement between a local magnetic impurity and its spatially nearby conduction electron. A groundstate phase diagram is derived and a discontinuous breakdown of the local Kondo entanglement is found at the singular point, associated concomitantly with a jump in the inter-impurity entanglement. An entanglement monogamy holds in the whole phase diagram. Our results identify the important role of the frustrated cross-coupling and demonstrate the local characteristic of the quantum phase transition in the two-impurity Kondo problem. The implications of these results for Kondo lattices and quantum information processing are also briefly discussed.

The problem of two magnetic impurities in a normal metal exposes the two opposite tendencies in the formation of a singlet ground state, driven respectively by the single-ion Kondo effect with conduction electrons to screen impurity spins or the Ruderman-Kittel-Kasuya-Yosida interaction between the two impurities to directly form impurity spin singlet. However, whether the competition between these two tendencies can lead to a quantum critical point has been debated over more than two decades. Here, we study this problem by applying the newly proposed natural orbitals renormalization group method to a lattice version of the two-impurity Kondo model with a direct exchange

K

between the two impurity spins. The method allows for unbiased access to the ground state wave functions and low-lying excitations for sufficiently large system sizes. We demonstrate the existence of a quantum critical point, characterized by the power-law divergence of impurity staggered susceptibility with critical exponent $\ensuremath{\gamma}=0.60(1)$, on the antiferromagnetic side of

K

when the interimpurity distance

R

is even lattice spacing, while a crossover behavior is recovered when

R

is odd lattice spacing. These results have ultimately resolved the long-standing discrepancy between the numerical renormalization group and quantum Monte Carlo studies, confirming a link of this two-impurity Kondo critical point to a hidden particle-hole symmetry predicted by the local Fermi liquid theory.

We study non-equilibrium dynamics and quantum quenches in a recent gauge/gravity duality model for a strongly coupled system interacting with a magnetic impurity with SU(N ) spin. At large N , it is convenient to write the impurity spin as a bilinear in Abrikosov fermions. The model describes an RG flow triggered by the marginally relevant Kondo operator. There is a phase transition at a critical temperature, below which an operator condenses which involves both an electron and an Abrikosov fermion field. This corresponds to a holographic superconductor in AdS2 and models the impurity screening. We quench the Kondo coupling either by a Gaussian pulse or by a hyperbolic tangent, the latter taking the system from the condensed to the uncondensed phase or vice-versa. We study the time dependence of the condensate induced by this quench. The timescale for equilibration is generically given by the leading quasinormal mode of the dual gravity model. This mode also governs the formation of the screening cloud, which is obtained as the decrease of impurity degrees of freedom with time. In the condensed phase, the leading quasinormal mode is imaginary and the relaxation of the condensate is over-damped. For quenches whose final state is close to the critical point of the large N phase transition, we study the critical slowing down and obtain the combination of critical exponents zν = 1. When the final state is exactly at the phase transition, we find that the exponential ringing of the quasinormal modes is replaced by a power-law behaviour of the form ∼ t −a sin(b log t). This indicates the emergence of a discrete scale invariance.