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arXiv:1205.4393 · Physical Review B

Quantum correlations in nanostructured two-impurity Kondo systems

Marco Nizama, Diego Frustaglia, K. Hallberg

Published Aug 6, 2012• 7 citations
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Abstract

We study the ground-state entanglement properties of nanostructured Kondo systems consisting of a pair of impurity spins coupled to a background of confined electrons. The competition between the Ruderman-Kittel-Kasuya-Yosida-like coupling and the Kondo effect determines the development of quantum correlations between the different parts of the system. A key element is the electronic filling due to confinement. An even electronic filling leads to results similar to those found previously for extended systems, where the properties of the reduced impurity spin subsystem are uniquely determined by the spin-correlation function defining a one-dimensional phase space. An odd filling, instead, breaks spin rotation symmetry unfolding a two-dimensional phase space showing rich entanglement characteristics as, e.g., the requirement of a larger amount of entanglement for the development of nonlocal correlations between impurity spins. We illustrate these results by numerical simulations of elliptic quantum corrals with magnetic impurities at the foci as a case study.

DOI
10.1103/physrevb.86.075413

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We study the ground-state entanglement properties of nanostructured Kondo systems consisting of a pair of impurity spins coupled to a background of confined electrons. The competition between the Ruderman-Kittel-Kasuya-Yosida-like coupling and the Kondo effect determines the development of quantum correlations between the different parts of the system. A key element is the electronic filling due to confinement. An even electronic filling leads to results similar to those found previously for extended systems, where the properties of the reduced impurity spin subsystem are uniquely determined by the spin-correlation function defining a one-dimensional phase space. An odd filling, instead, breaks spin rotation symmetry unfolding a two-dimensional phase space showing rich entanglement characteristics as, e.g., the requirement of a larger amount of entanglement for the development of nonlocal correlations between impurity spins. We illustrate these results by numerical simulations of elliptic quantum corrals with magnetic impurities at the foci as a case study.
In order to quantify quantum entanglement in two-impurity Kondo systems, we calculate the concurrence, negativity, and von Neumann entropy. The entanglement of the two Kondo impurities is shown to be determined by two competing many-body effects, namely the Kondo effect and the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction, III. Due to the spin-rotational invariance of the ground state, the concurrence and negativity are uniquely determined by the spin-spin correlation between the impurities. It is found that there exists a critical minimum value of the antiferromagnetic correlation between the impurity spins which is necessary for entanglement of the two impurity spins. The critical value is discussed in relation with the unstable fixed point in the two-impurity Kondo problem. Specifically, at the fixed point there is no entanglement between the impurity spins. Entanglement will only be created [and quantum information processing (QIP) will only be possible] if the RKKY interaction exchange energy, III, is at least several times larger than the Kondo temperature, TK{T}_{K}TK​. Quantitative criteria for QIP are given in terms of the impurity spin-spin correlation.
We propose that real-space properties of the two-impurity Kondo model can be obtained from an effective spin model where two single-impurity Kondo spin chains are joined via an Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between the two impurity spins. We then use a density matrix renormalization group approach, valid in all ranges of parameters, to study its features using two complementary quantum-entanglement measures, the negativity and the von Neumann entropy. This nonperturbative approach enables us to uncover the precise dependence of the spatial extent ξ(K) of the Kondo screening cloud with the Kondo and RKKY couplings. Our results reveal an exponential suppression of the Kondo temperature T(K)~1/ξ(K) with the size of the effective impurity spin in the limit of large ferromagnetic RKKY coupling, a striking display of "Kondo resonance narrowing" in the two-impurity Kondo model. We also show how the antiferromagnetic RKKY interaction produces an effective decoupling of the impurities from the bulk already for intermediate strengths of this interaction, and, furthermore, exhibit how the non-Fermi liquid quantum critical point is signaled in the quantum entanglement between various parts of the system.
Competition between the Kondo effect and Ruderman-Kittel-Kasuya-Yosida interaction in the two-impurity Kondo problem can be phenomenologically described by the Rasul-Schlottmann spin model. We revisit this model from the quantum entanglement perspective by calculating both the inter-impurity entanglement and the local Kondo entanglement, the latter being the entanglement between a local magnetic impurity and its spatially nearby conduction electron. A groundstate phase diagram is derived and a discontinuous breakdown of the local Kondo entanglement is found at the singular point, associated concomitantly with a jump in the inter-impurity entanglement. An entanglement monogamy holds in the whole phase diagram. Our results identify the important role of the frustrated cross-coupling and demonstrate the local characteristic of the quantum phase transition in the two-impurity Kondo problem. The implications of these results for Kondo lattices and quantum information processing are also briefly discussed.
We study the two-impurity Kondo model (TIKM) in two dimensions with spin-orbit coupled conduction electrons. In the first part of the paper we analyze how spin-orbit interactions of Rashba as well as Dresselhaus type influence the Kondo and Ruderman-Kittel-Kasuya-Yoshida (RKKY) interactions in the TIKM, generalizing results obtained by H. Imamura et al. [Phys. Rev. B 69, 121303(R) (2004)] and J. Malecki [J. Stat. Phys. 129, 741 (2007)]. Using our findings we then explore the effect from spin-orbit interactions on the non-Fermi-liquid quantum critical transition between the RKKY-singlet and Kondo-screened RKKY-triplet states. We argue that spin-orbit interactions under certain conditions produce a line of critical points exhibiting the same leading scaling behavior as that of the ordinary TIKM. In the second part of the paper we shift focus and turn to the question of how spin-orbit interactions affect the entanglement between two localized RKKY-coupled spins in the parameter regime where the competition from the direct Kondo interaction can be neglected. Using data for a device with two spinful quantum dots patterned in a gated InAs heterostructure we show that a gate-controlled spin-orbit interaction may drive a maximally entangled state to one with vanishing entanglement or vice versa (as measured by the concurrence). This has important implications for proposals using RKKY interactions for nonlocal control of qubit entanglement in semiconductor heterostructures.
Quantum dots exhibit a variety of strongly correlated effects, e.g., when tuned to emulate localized magnetic impurities that form a Kondo singlet with their surrounding environment. Interestingly, in double-dots setups, the magnetic impurities couple to each other by direct Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction, which wins over the Kondo physics. In this work, we investigate a double-dot device where the dots are coupled via off-resonant ballistic whispering gallery modes, dubbed electronic cavity modes. Within this cavity-double-dot system, we study, using variational matrix product state techniques, the competition between Kondo formation and the coherent RKKY-like interaction that the cavity facilitates. Specifically, we find that (i) Kondo can win and form on each dot individually, or (ii) the cavity can win and mediate between the two dots either a singlet or a novel nonlocal Kondo-like effect phase, which we call "cat Kondo". We systematically study the quantum phase transitions between the different many-body states. Our discoveries lay the foundation for the experimental observation of unconventional nonlocal magnetic impurities.
In order to study the interplay between Kondo and Ruderman-Kittel-Kasuya-Yosida interaction, we calculate the spin-spin correlation functions between two Kondo impurities coupled to different sites of a half-filled open Hubbard chain. Using the density-matrix renormalization group (DMRG), we reexamine the exponents for the power-law decay of the correlation function between the two impurity spins as a function of the antiferromagnetic coupling JJJ, the Hubbard interaction UUU, and the distance RRR between the impurities. The exponents for finite systems obtained in this work deviate from previously published DMRG calculations. We furthermore show that the long-distance behavior of the exponents is the same for impurities coupled to the bulk or to both ends of the chain. We note that a universal exponent for the asymptotic behavior can not be extracted from these finite-size systems with open boundary conditions.