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arXiv:physics/0501033

Anharmonic mixing in a magnetic trap

Ralf Gommers, BJ Bert Claessens, C. J. Hawthorn, Herman C. W. Beijerinck, Ejd Edgar Vredenbregt

Published Jan 7, 2005• 0 citations
arXivHTMLPDF

Abstract

We have experimentally observed re-equilibration of a magnetically trapped cloud of metastable neon atoms after it was put in a non-equilibrium state. Using numerical simulations we show that anharmonic mixing, equilibration due to the collisionless dynamics of atoms in a magnetic trap, is the dominant process in this equilibration. We determine the dependence of its time on trap parameters and atom temperature. Furthermore we observe in the simulations a resonant energy exchange between the radial and axial trap dimensions at a ratio of trap frequencies ω_r / ω_z = 3/2. This resonance is explained by a simple oscillator model.

DOI
10.48550/arxiv.physics/0501033

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We have experimentally observed re-equilibration of a magnetically trapped cloud of metastable neon atoms after it was put in a non-equilibrium state. Using numerical simulations we show that anharmonic mixing, equilibration due to the collisionless dynamics of atoms in a magnetic trap, is the dominant process in this equilibration. We determine the dependence of its time on trap parameters and atom temperature. Furthermore we observe in the simulations a resonant energy exchange between the radial and axial trap dimensions at a ratio of trap frequencies ω_r / ω_z = 3/2. This resonance is explained by a simple oscillator model.
We describe an experiment in which cold rubidium atoms, confined in an elongated magnetic trap, are excited by transverse oscillation of the trap center. The temperature after excitation exhibits resonance as a function of the driving frequency. We measure these resonances at several different trap frequencies. In order to interpret the experiments, we develop a simple model that incorporates both collisions between atoms and the anharmonicity of the real three-dimensional trapping potential. As well as providing a precise connection between the transverse harmonic oscillation frequency and the temperature resonance frequency, this model gives insight into the heating and loss mechanisms and into the dynamics of driven clouds of cold trapped atoms.
In this thesis, the study of cold gases of neon atoms in different metastable states is described. It contains measurements of the collisional parameters for both the 3s[3/2]2 and the 3s'[1/2]0 metastable state and the dependence of the inelastic loss on external fields. Furthermore, the investigation of frequency dependent laser-induced collisions, and the possibility to excite photoassociation resonances is presented. Based on previous measurements we have selected 22Ne for evaporative cooling. Although, we can experimentally achieve an increase in phase-space density with evaporative cooling, the relatively high inelastic collision parameters prevent the realization of a Bose-Einstein condensate in neon. For the measurements described here, neon atoms have been confined in a magneto-optical trap, in a magnetostatic trap, or in an optical dipole trap, respectively. By laser cooling inside the magnetic trap, atomic samples with more than 95 percent occupation of the magnetic substate m=+2 could be prepared. They have a typical temperature of 0.5 mK, central densities up to 1e11 cm^-3, and a central phase-space density of up to 2.2e-7. After loading the optical dipole trap from the magnetic trap, 2.5e6 atoms with typical temperatures of 0.1 mK, and central densities up to 5e10 cm^-3 were trapped. By evaporative cooling of the atoms in the magnetic trap we could increase the phase-space density by a factor of 200 to 5e-5. Also simulations of optimized evaporation for our experimental parameters show clearly that we are limited to a phase-space density on the order of 1e-5. From these simulations it became clear that a 5-fold increase in the good-to-bad ratio for evaporative cooling suffices to reach the quantum degenerate regime. Investigating the frequency dependence of laser-induced collisions did not reveal an experimental signature for the excitation of photoassociation resonances. For the 3D3 line a frequency dependence of laser enhanced Penning ionization was observed, which is interesting in itself. The absence of the collisional enhancement effect by laser light for the transition to the 3D2 line is intriguing and for an explanation calculations are required. Measurement of the two-body loss coefficient as function of the magnetic field showed a field dependence of the inelastic loss. These losses increase towards both small and large offset fields. In the magnetic trap, we are limited to offset fields < 50 G. In this range of fields, the two-body losses are too large to achieve a Bose-Einstein condensate of magnetically trapped metastable neon. The implementation of an optical dipole trap allowed us to trap the 3P0 metastable state. From the trap loss measurements we determined the two-body loss coefficient of the 3P0 metastable state for both bosonic isotopes 20Ne and 22Ne. For 20Ne we obtained s=6(+5,-4)e-10 cm^3/s and for 22Ne s=11(+7,-6)e-10 cm^3/s. These large two-body losses make it extremely unlikely to reach degeneracy with this metastable state. Nevertheless it is important that the 3P0 metastable state can be trapped to investigate other interesting physical effects. For example, it is essential to apply the STIRAP technique for trapped atoms and to realize the proposed coherent control of collisions. There is also a large interest in a precise determination of the lifetime of this metastable state, which is of importance for the verification of QED. We can also trap neon atoms in their energetically lowest magnetic substate 3P2(m=-2) with the perspective of reducing inelastic collisions in the energetically lowest state.
A combined gravitomagnetic trap was used to measure how the anharmonicity of a trapping potential affects the dynamics of a cold atomic cloud. A displacement of the effective potential minimum as a function of the ensemble temperature was observed. The effect is a direct consequence of the thermal nature of the atomic sample. The results of both a theory approach to the dynamical evolution of the atomic cloud and a numerical simulation are in very good agreement with the experimental observations. The effect can be exploited to devise a novel measurement technique for the temperature of a trapped atomic cloud, as well as to separate thermal and condensed phases in Bose-Einstein condensation experiments.
Ludwig Boltzmann made tremendously important contributions to the problem of connecting macroscopic, empirical phenomena with microscopic, atomistic dynamics. At the end of the nineteenth century, Boltzmann was confronted with various strong objections to his work. For example, Boltzmann's atomistic explanations presuppose the reality of atoms, a notion that was vigorously rejected in some circles [14, 38]. Then too, there was the critique by Loschmidt that Boltzmann's H-theorem, put forth as a microscopic explanation for the Second Law of Thermodynamics, could hardly account for irreversible physics when the individual two-atom collisions were each reversible [18, 42]. Still intriguing today is the existence of special cases of the Boltzmann equation in which time-varying distributions of atoms resist the imperative of equilibration, even in the presence of collisions. Boltzmann discussed such situations in a paper dedicated to responding to Loschmidt's critique [7, 4]. Perhaps Boltzmann's motivation was to enumerate special cases where his famous H value does not relax as it should, and by enumerating them, point out their nonnaturalness, their artificiality. Damping, or relaxation to equilibrium, of a time-invariant phase-space distribution, is an all-but universal result predicted by the Boltzmann equation.\nSuch improbable systems of atoms have only very recently been realized experimentally. Kinoshita et al. [36] experimentally confirmed that atoms constrained to move in a quasi one-dimensional potential, an atomistic Newtons cradle, exhibit vastly suppressed relaxation. Chevy et al. [15] observed long-lived breathe-mode oscillations in highly elongated but still 3D geometries. Perhaps one of the more interesting cases is the vanishing damping of the monopole breathe-mode oscillation in a spherically symmetric harmonic oscillator [29], where a cloud of atoms experiences undamped temperature oscillations, causing the cloud to expand and contract as if it were breathing. Until now, this phenomenon has been experimentally inaccessible due to the difficulty in generating isotropic harmonic confinement. This thesis discusses a new magnetic trap capable of producing spherical confinement and presents the first experimental realization of this historically significant oddity using a magnetically trapped gas of 87Rb atoms.
We observe the population dynamics within a metastable neon magneto-optical trap (MOT) through the measurement of the average squared Clebsch-Gordan coefficient C2{C}^{2}C2 over a range of laser detunings. The magnitude of C2{C}^{2}C2 is dependent on the internal quantum state of an atom interacting with the light field and is found to show a strong dependence on the applied laser detuning. Previously it has been reported [Townsend et al., Phys. Rev. A 52, 1423 (1995)] that trapped atoms in a MOT are pumped towards the states that interact most strongly with the local field and therefore the measured value of C2{C}^{2}C2 is larger than the average over all possible transitions. For the 3P2{}^{3}{P}_{2}3P2​-to-3D3{}^{3}{D}_{3}3D3​ cooling transition in metastable neon the average C2{C}^{2}C2 value is equal to 0.46; however, we have measured $0.29\ifmmode\pm\else\textpm\fi{}0.03<{C}^{2}<0.73\ifmmode\pm\else\textpm\fi{}0.09$. We explain this range of values for C2{C}^{2}C2 by considering the possible transition rates between the different magnetic sublevels in the system. This result has significant consequences when trap populations are measured via fluorescence in a MOT.