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Physical Review A

Population dynamics in a metastable neon magneto-optical trap

R. D. Glover, James Calvert, Robert T. Sang

Published Feb 20, 2013• 6 citations
Publisher

Abstract

We observe the population dynamics within a metastable neon magneto-optical trap (MOT) through the measurement of the average squared Clebsch-Gordan coefficient ${C}^{2}$ over a range of laser detunings. The magnitude of ${C}^{2}$ is dependent on the internal quantum state of an atom interacting with the light field and is found to show a strong dependence on the applied laser detuning. Previously it has been reported [Townsend et al., Phys. Rev. A 52, 1423 (1995)] that trapped atoms in a MOT are pumped towards the states that interact most strongly with the local field and therefore the measured value of ${C}^{2}$ is larger than the average over all possible transitions. For the ${}^{3}{P}_{2}$-to-${}^{3}{D}_{3}$ cooling transition in metastable neon the average ${C}^{2}$ value is equal to 0.46; however, we have measured $0.29\ifmmode\pm\else\textpm\fi{}0.03<{C}^{2}<0.73\ifmmode\pm\else\textpm\fi{}0.09$. We explain this range of values for ${C}^{2}$ by considering the possible transition rates between the different magnetic sublevels in the system. This result has significant consequences when trap populations are measured via fluorescence in a MOT.

DOI
10.1103/physreva.87.023415

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We observe the population dynamics within a metastable neon magneto-optical trap (MOT) through the measurement of the average squared Clebsch-Gordan coefficient C2{C}^{2}C2 over a range of laser detunings. The magnitude of C2{C}^{2}C2 is dependent on the internal quantum state of an atom interacting with the light field and is found to show a strong dependence on the applied laser detuning. Previously it has been reported [Townsend et al., Phys. Rev. A 52, 1423 (1995)] that trapped atoms in a MOT are pumped towards the states that interact most strongly with the local field and therefore the measured value of C2{C}^{2}C2 is larger than the average over all possible transitions. For the 3P2{}^{3}{P}_{2}3P2​-to-3D3{}^{3}{D}_{3}3D3​ cooling transition in metastable neon the average C2{C}^{2}C2 value is equal to 0.46; however, we have measured 0.29\ifmmode±\else\textpm\fi0.03<C2<0.73\ifmmode±\else\textpm\fi0.090.29\ifmmode\pm\else\textpm\fi{}0.03<{C}^{2}<0.73\ifmmode\pm\else\textpm\fi{}0.090.29\ifmmode±\else\textpm\fi0.03<C2<0.73\ifmmode±\else\textpm\fi0.09. We explain this range of values for C2{C}^{2}C2 by considering the possible transition rates between the different magnetic sublevels in the system. This result has significant consequences when trap populations are measured via fluorescence in a MOT.
This thesis presents an in-depth study into the characterization and enhancement of a metastable neon laser cooled and trapped atomic beam. The apparatus consists of a standard Zeeman slowed atomic beam loaded into a magneto-optical trap and was designed for applications to electron scattering experiments and photoionization. The efficiency of the metastable neon atomic source was investigated to determine the ideal cathode type for maximum metastable production and optimal atomic beam velocity haracteristics. A series of characterization measurements were performed on the MOT, and the trap volume and population were investigated for a range of trapping and slowing laser intensities and detunings, together with the MOT and Zeeman slower magnetic fields. The volume measurements were compared to standard Doppler theory and it was found that the Doppler model inadequately explained the trap behaviour. It was found that the MOT population characteristics were governed by two processes: two-body losses that limit the trap population at high densities, and the efficiency of the atom capture process which limits the operational range of the MOT over the various parameters. The trap temperature was determined to be 1.3mK via a time-of-flight technique. This was nearly twice that predicted by Doppler theory and the lack of agreement once again suggests the inadequacies in the Doppler theory to correctly model the experiment. The application of the MOT to the photoionization cross-section measurement of the (2p53p)3D3 state of neon was investigated. The MOT decay technique was utilized to measure cross-section values of o351 = 2.9+0.2 -0.3 x 10 -18cm2 and o363 = 3.1 +0.3 -0.4 x 10-18cm2 at the wavelengths of 351nm and 363nm respectively. This is an increase in accuracy of around a factor of five from previous measurements and it was found that the results agreed well with the values predicted by current theories.
We have constructed a magneto-optical trap (MOT) for metastable triplet helium atoms utilizing the $2{}^{3}{S}_{1}\ensuremath{\rightarrow}3{}^{3}{P}_{2}$ line at 389 nm as the trapping and cooling transition. The far-red-detuned MOT (detuning $\ensuremath{\Delta}=\ensuremath{-}41\mathrm{MHz})$ typically contains few times 107{10}^{7}107 atoms at a relatively high $(\ensuremath{\sim}{10}^{9}{\mathrm{cm}}^{\ensuremath{-}3})$ density, which is a consequence of the large momentum transfer per photon at 389 nm and a small two-body loss rate coefficient $(2\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}10}{\mathrm{cm}}^{3}/\mathrm{s}<\ensuremath{\beta}<1.0\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}9}{\mathrm{cm}}^{3}/\mathrm{s}).$ The two-body loss rate is more than five times smaller than in a MOT on the commonly used $2{}^{3}{S}_{1}\ensuremath{\rightarrow}2{}^{3}{P}_{2}$ line at 1083 nm. Furthermore, laser cooling at 389 nm results in temperatures somewhat lower than those achieved using 1083 nm. The 389-nm MOT exhibits small losses due to two-photon ionization, which have been investigated as well.
We present results for controlled optical collisions of cold, metastable Ne atoms in a magneto-optical trap. The modification of the ionizing collision rate is demonstrated using a control laser tuned close to the (3s)3P2 to (3p)3D3 cooling transition. The measured ionization spectrum does not contain resonances due to the formation of photoassociated molecules connected to the omega = 5 excited state potential as predicted by Doery et al (1998 Phys. Rev. A 57 3603-20). Instead, we observe a broad unresolvable ionization spectrum that is well described by established theory (Gallagher and Pritchard 1989 Phys. Rev. Lett. 63 957). In order to induce collisions between pairs of trapped metastables, a control laser is tuned to the red of the transition where we measure a factor of 4 increase in the rate for ionizing collisions. We also investigate the effect of optical shielding by tuning the laser to the blue of the transition and observe a factor of 5 suppression in the ionization rate.
In this thesis, the study of cold gases of neon atoms in different metastable states is described. It contains measurements of the collisional parameters for both the 3s[3/2]2 and the 3s'[1/2]0 metastable state and the dependence of the inelastic loss on external fields. Furthermore, the investigation of frequency dependent laser-induced collisions, and the possibility to excite photoassociation resonances is presented. Based on previous measurements we have selected 22Ne for evaporative cooling. Although, we can experimentally achieve an increase in phase-space density with evaporative cooling, the relatively high inelastic collision parameters prevent the realization of a Bose-Einstein condensate in neon. For the measurements described here, neon atoms have been confined in a magneto-optical trap, in a magnetostatic trap, or in an optical dipole trap, respectively. By laser cooling inside the magnetic trap, atomic samples with more than 95 percent occupation of the magnetic substate m=+2 could be prepared. They have a typical temperature of 0.5 mK, central densities up to 1e11 cm^-3, and a central phase-space density of up to 2.2e-7. After loading the optical dipole trap from the magnetic trap, 2.5e6 atoms with typical temperatures of 0.1 mK, and central densities up to 5e10 cm^-3 were trapped. By evaporative cooling of the atoms in the magnetic trap we could increase the phase-space density by a factor of 200 to 5e-5. Also simulations of optimized evaporation for our experimental parameters show clearly that we are limited to a phase-space density on the order of 1e-5. From these simulations it became clear that a 5-fold increase in the good-to-bad ratio for evaporative cooling suffices to reach the quantum degenerate regime. Investigating the frequency dependence of laser-induced collisions did not reveal an experimental signature for the excitation of photoassociation resonances. For the 3D3 line a frequency dependence of laser enhanced Penning ionization was observed, which is interesting in itself. The absence of the collisional enhancement effect by laser light for the transition to the 3D2 line is intriguing and for an explanation calculations are required. Measurement of the two-body loss coefficient as function of the magnetic field showed a field dependence of the inelastic loss. These losses increase towards both small and large offset fields. In the magnetic trap, we are limited to offset fields < 50 G. In this range of fields, the two-body losses are too large to achieve a Bose-Einstein condensate of magnetically trapped metastable neon. The implementation of an optical dipole trap allowed us to trap the 3P0 metastable state. From the trap loss measurements we determined the two-body loss coefficient of the 3P0 metastable state for both bosonic isotopes 20Ne and 22Ne. For 20Ne we obtained s=6(+5,-4)e-10 cm^3/s and for 22Ne s=11(+7,-6)e-10 cm^3/s. These large two-body losses make it extremely unlikely to reach degeneracy with this metastable state. Nevertheless it is important that the 3P0 metastable state can be trapped to investigate other interesting physical effects. For example, it is essential to apply the STIRAP technique for trapped atoms and to realize the proposed coherent control of collisions. There is also a large interest in a precise determination of the lifetime of this metastable state, which is of importance for the verification of QED. We can also trap neon atoms in their energetically lowest magnetic substate 3P2(m=-2) with the perspective of reducing inelastic collisions in the energetically lowest state.
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